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Large-scale Monte Carlo simulations of a phase-separating colloid-polymer mixture are performed and compared to recent experiments. The approach is based on effective interaction potentials in which the central monomers of self-avoiding…

软凝聚态物质 · 物理学 2007-05-23 R. L. C. Vink , A. Jusufi , J. Dzubiella , C. N. Likos

The properties of a system of charged particles on a 2D lattice, subject to an anisotropic Jahn-Teller-type interaction and 3D Coulomb repulsion are investigated. In the mean-field approximation without Coulomb interaction, the system…

强关联电子 · 物理学 2008-11-19 T. Mertelj , V. V. Kabanov , D. Mihailovic

Properties of polyelectrolytes in tetravalent salt solutions are intensively investigated by a coarse-grained model. The concentration of salt and the size of tetravalent counterions are found playing a decisive role on chain properties. If…

软凝聚态物质 · 物理学 2009-09-29 Pai-Yi Hsiao

We consider the response of an adsorbed polymer that is pulled by an AFM within a simple geometric framework. We separately consider the cases of i) fixed polymer-surface contact point, ii) sticky case where the polymer is peeled off from…

软凝聚态物质 · 物理学 2009-11-11 Andreas Serr , Roland R. Netz

We use the worm-like chain model to analytically calculate the linear response of a grafted semiflexible polymer to a uniform force field. The result is a function of the bending stiffness, the temperature, the total contour length, and the…

软凝聚态物质 · 物理学 2009-11-10 Panayotis Benetatos , Erwin Frey

The effective interaction between charged colloidal particles confined between two planar like-charged walls is investigated using computer simulations of the primitive model describing asymmetric electrolytes. In detail, we calculate the…

软凝聚态物质 · 物理学 2016-08-15 E. Allahyarov , I. D'Amico , H. Löwen

The influence of long-range correlated surface and decaying near surface disorder with quenched defects is studied. We consider a correlation function for the defects of the form $\frac{e^{-z/\xi}}{r^{a}}$, where $a<d-1$ and $z$ being the…

软凝聚态物质 · 物理学 2009-10-08 Z. Usatenko , J. -U. Sommer

Brownian Dynamics simulations are carried out to understand the effect of temperature and dielectric constant of the medium on microphase separation of charged-neutral diblock copolymer systems. For different dielectric media, we focus on…

软凝聚态物质 · 物理学 2011-07-20 Monojoy Goswami , Rajeev Kumar , Bobby G. Sumpter , Jimmy Mays

The folding transition of single, long semiflexible polymers was studied with special emphasis on the chain length effect using Monte Carlo simulations. While a relatively short chain (10-25 Kuhn segments) undergoes a large discrete…

软凝聚态物质 · 物理学 2008-05-06 Yuji Higuchi , Takahiro Sakaue , Kenichi Yoshikawa

We propose that several mechanisms contribute to friction in a polymer melt adsorbed at a structured surface. The first one is the well known disentanglement of bulk polymer chains from the surface layer. However, if the surface is ideal at…

软凝聚态物质 · 物理学 2007-05-23 X. Zhou , D. Andrienko , L. Delle Site , K. Kremer

Surface properties of mixtures of charged platelike colloids and salt in contact with a charged planar wall are studied within density functional theory. The particles are modeled by hard cuboids with their edges constrained to be parallel…

软凝聚态物质 · 物理学 2011-09-14 Markus Bier , Ludger Harnau , S. Dietrich

We consider the thermodynamics of a uniformly charged polyelectrolyte with harmonic bonds. For such a system there is at high temperatures an approximate scaling of global properties like the end-to-end distance and the interaction energy…

chem-ph · 物理学 2016-08-15 Carsten Peterson , Ola Sommelius , Bo Söderberg

We consider a polymer brush grafted to a surface (acting as an electrode) and bearing a charged group at its free end. Using a second distant electrode, the brush is subject to a constant electric field. Based on a coarse-grained continuum…

软凝聚态物质 · 物理学 2012-01-31 Yoav Tsori , David Andelman , Jean-François Joanny

The stretching of brushes of long polymers grafted to a planar surface is investigated byMonte Carlo simulations in the limit of very high grafting densities, as achieved in recent experiments. The monomer density profiles are shown to…

软凝聚态物质 · 物理学 2009-11-13 Ivan Coluzza , Jean-Pierre Hansen

The behavior of mesoscopic particles dissolved in a dilute solution of long, flexible, and nonadsorbing polymer chains is studied by field-theoretic methods. For spherical and cylindrical particles the solvation free energy for immersing a…

软凝聚态物质 · 物理学 2009-10-31 A. Hanke , E. Eisenriegler , S. Dietrich

We investigate the localization of a hydrophobic - polar (HP) - regular copolymer at a selective solvent-solvent interface with emphasis on the impact of block length $M$ on the copolymer behavior. The considerations are based on simple…

软凝聚态物质 · 物理学 2007-05-23 Andrea Corsi , Andrey Milchev , Vakhtang G. Rostiashvili , Thomas A. Vilgis

We develop Monte Carlo simulations for uniformly charged polymers and machine learning algorithm to interpret the intra-polymer structure factor of the charged polymer system, which can be obtained from small-angle scattering experiments.…

软凝聚态物质 · 物理学 2025-11-21 Lijie Ding , Chi-Huan Tung , Jan-Michael Y. Carrillo , Wei-Ren Chen , Changwoo Do

We study a solution of long polyanions (PA) with shorter polycations (PC) and focus on the role of Coulomb interaction. A good example is solutions of DNA and PC which are widely studied for gene therapy. In the solution, each PA attracts…

软凝聚态物质 · 物理学 2025-02-11 Rui Zhang , B. I. Shklovskii

We present a set of molecular dynamics (MD) simulations of strongly charged, flexible polyelectrolyte chains under poor solvent conditions in a salt free solution. Structural properties of the chains and of the solutions are reported. By…

软凝聚态物质 · 物理学 2007-05-23 Uwe Micka , Christian Holm , Kurt Kremer

We consider forces acting on objects immersed in, or attached to, long fluctuating polymers. The confinement of the polymer by the obstacles results in polymer-mediated forces that can be repulsive (due to loss of entropy) or attractive (if…

统计力学 · 物理学 2017-08-28 Yacov Kantor , Mehran Kardar