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We study the adsorption-desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the…

软凝聚态物质 · 物理学 2016-10-05 Sidney J. de Carvalho , Ralf Metzler , Andrey G. Cherstvy

We study the interaction between heterogeneously charged surfaces in an electrolyte solution by employing classical Density Functional Theory (cDFT) and Monte Carlo simulations. We observe a consistent behavior between cDFT and Monte Carlo…

软凝聚态物质 · 物理学 2023-07-11 Shiqi Zhou , Amin Bakhshandeh

We report results from a molecular dynamics (MD) simulation on the conformations of a long flexible polyelectrolyte complexed to a charged sphere, \textit{both negatively charged}, in the presence of neutralizing counterions in the strong…

软凝聚态物质 · 物理学 2009-11-07 Rene Messina , Christian Holm , Kurt Kremer

Taking into account the well known correspondence between the field theoretical O(n)-vector model in the limit $n\to 0$ and the behavior of long-flexible polymer chains in a good solvent the investigation of ideal polymer chains adsorption…

软凝聚态物质 · 物理学 2012-09-25 Zoryana Usatenko

The results of a study that helps understand the mechanisms of adsorption of polyelectrolytes on particles, using numerical simulation methods, specifically the one known as dissipative particle dynamics are reported here. The adsorption of…

软凝聚态物质 · 物理学 2016-08-24 M. A. Balderas Altamirano , R. Camacho , E. Pérez , A. Gama Goicochea

Structure and dynamics of an active polymer on a smooth cylindrical surface are studied by Brownian dynamics simulations. The effect of active force on the polymer adsorption behavior and the combined effect of chain mobility, length N,…

软凝聚态物质 · 物理学 2024-08-21 Chen Shen , Chao-ran Qin , Tian-liang Xu , Kang Chen , Wen-de Tian

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

化学物理 · 物理学 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller

Polyampholytes (PA) are charged polymers composed of positively and negatively charged monomers along their backbone. The sequence of the charged monomers and the bending of the chain significantly influence the conformation and dynamical…

软凝聚态物质 · 物理学 2024-08-29 Rakesh Palariya , Sunil P. Singh

We analyze the structural behavior of a single polymer chain grafted to an attractive, flexible surface. Our model is composed of a coarse-grained bead-and-spring polymer and a tethered membrane. By means of extensive parallel tempering…

软凝聚态物质 · 物理学 2011-09-26 Steffen Karalus , Wolfhard Janke , Michael Bachmann

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

软凝聚态物质 · 物理学 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

We study analytically a model of a two dimensional, partially directed, flexible or semiflexible polymer, attached to an attractive wall which is perpendicular to the preferred direction. In addition, the polymer is stretched by an…

统计力学 · 物理学 2015-05-13 Pui-Man Lam , Yi Zhen , Haijun Zhou , Jie Zhou

The influence of monomer-monomer interactions on the scaling exponents and shape characteristics of a single polymer chain in a selective solvent is investigated using Langevin dynamics simulations. By systematically increasing the…

软凝聚态物质 · 物理学 2025-04-01 K. Haydukivska

Experiments using the Surface Force Apparatus (SFA) have found anomalously long-ranged interactions between charged surfaces in concentrated salt solutions. Ion clustering have been suggested as a possible origin of this behaviour. In this…

软凝聚态物质 · 物理学 2025-08-05 David Ribar , Clifford E. Woodward , Jan Forsman

The adsorption of a single ideal polymer chain on energetically heterogeneous and rough surfaces is investigated using a variational procedure introduced by Garel and Orland (Phys. Rev. B 55 (1997), 226). The mean polymer size is calculated…

统计力学 · 物理学 2009-10-31 Gregor Huber , Thomas A. Vilgis

Charged colloidal monolayers at the interface between water and air (or oil) are used in a large number of chemical, physical and biological applications. Although a considerable experimental and theoretical effort has been devoted in the…

软凝聚态物质 · 物理学 2018-12-03 Aviv Karnieli , Tomer Markovich , David Andelman

Equilibrium adsorption of disk-like particles on patterned adhesive surfaces is studied using Monte Carlo simulations. The surface is represented as a two-dimensional plane with circular adhesive domains arranged either regularly or…

软凝聚态物质 · 物理学 2026-05-05 Nazar Kukarkin , Taras Patsahan

Mean-field theory and scaling arguments are presented to model polyelectrolyte adsorption from semi-dilute solutions onto charged surfaces. Using numerical solutions of the mean-field equations, we show that adsorption exists only for…

软凝聚态物质 · 物理学 2009-11-10 A. Shafir , D. Andelman , R. R. Netz

Forced desorption of a semiflexible polymer chain on a solid substrate is theoretically investigated. The pulling force versus displacement is studied for different adsorption energy and persistence length P. It is found that the…

统计力学 · 物理学 2015-06-19 Pui-Man Lam , Yi Zhen

The adsorption of a bottle-brush polymer end-grafted with one chain end of its backbone to a flat substrate surface is studied by Monte Carlo simulation of a coarse-grained model, that previously has been characterized in the bulk, assuming…

软凝聚态物质 · 物理学 2010-10-13 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

We discuss in this paper the phase diagram of a diblock polyampholyte solution in the limit of high ionic strength as a function of concentration and charge asymmetry. This system is shown to be very similar to solutions of so-called…

软凝聚态物质 · 物理学 2009-11-07 Martin Castelnovo , J. F. Joanny