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Charged soft-matter systems--such as colloidal dispersions and charged polymers--are dominated by attractive forces between constituent like-charged particles when neutralizing counterions of high charge valency are introduced. Such…

软凝聚态物质 · 物理学 2009-11-11 Ali Naji , Swetlana Jungblut , Andre G. Moreira , Roland R. Netz

In the study of colloidal, biological and electrochemical systems, it is customary to treat surfaces, macromolecules and electrodes as homogeneously charged. This simplified approach is proven successful in most cases, but fails to describe…

软凝聚态物质 · 物理学 2022-08-04 Ram M. Adar , David Andelman , Haim Diamant

Soft matter materials, such as polymers, membranes, proteins, are often electrically charged. This makes them water soluble, which is of great importance in technological application and a prerequisite for biological function. We discuss a…

软凝聚态物质 · 物理学 2007-05-23 H. Boroudjerdi , Y. -W. Kim , A. Naji , R. R. Netz , X. Schlagberger , A. Serr

Electrostatic interactions provide a convenient way to modulate interactions between nanoparticles, colloids, and biomolecules because they can be adjusted by the solution pH or salt concentration. While the presence of salt provides an…

软凝聚态物质 · 物理学 2019-09-04 Sawyer S. Hopkins , Amitabha Chakrabarti , Jeremy D. Schmit

The complexity of biomolecular interactions necessitates advanced methodologies to accurately capture their behavior in solution. In this work, we focus on monoclonal antibodies and adopt a multi-scale coarse-graining strategy for their…

Recently synthesized colloids and biological systems such as proteins, viruses and monoclonal antibodies are heterogeneously charged, i.e., different regions of their surfaces carry different amount of positive or negative charge. Because…

计算物理 · 物理学 2024-06-24 Daniele Notarmuzi , Emanuela Bianchi

We predict the nature (attractive or repulsive) and range (exponentially screened or long-range power law) of the electrostatic interactions of oppositely charged and planar plates as a function of the salt concentration and surface charge…

软凝聚态物质 · 物理学 2012-01-31 Dan Ben-Yaakov , Yoram Burak , David Andelman , S. A. Safran

Electrostatic interactions play an important role in numerous self-assembly phenomena, including colloidal aggregation. Although colloids typically have a dielectric constant that differs from the surrounding solvent, the effective…

软凝聚态物质 · 物理学 2018-09-17 Kipton Barros , Erik Luijten

In solution, electrically like-charged particles can experience a strong and long-ranged attraction that leads to the formation of stable, slowly reorganizing clusters. The attractive force underpinning this spontaneous organization process…

软凝聚态物质 · 物理学 2026-01-14 Sida Wang , Angela Le , Rowan Walker-Gibbons , Madhavi Krishnan

Electrostatic interactions fundamentally govern the structure, stability, and dynamics of charged (bio)matter, yet the impact of heterogeneous and anisotropic charge distributions on the behavior of protein solutions remains elusive. Here,…

Electrostatic correlations play an important role in physics, chemistry and biology. In plasmas they lead to thermodynamic instability similar to the liquid-gas phase transition of simple molecular fluids. For charged colloidal suspensions…

软凝聚态物质 · 物理学 2009-11-07 Yan Levin

Polymer chains adsorbed onto oppositely charged spherical colloidal particles can significantly modify the particle-particle interactions. For sufficient amounts of added polymers, the original electrostatic repulsion can even turn into an…

软凝聚态物质 · 物理学 2015-05-13 D. Truzzolillo , F. Bordi , F. Sciortino , C. Cametti

A multiple-image method is developed to accurately calculate the electrostatic interaction between neutral dielectric particles and a uniformly charged dielectric substrate. The difference in dielectric constants between the particle and…

软凝聚态物质 · 物理学 2024-12-18 Xin Li , Changhao Li , Xiangui Chen , Zaixin Wang , Sun Min , Decai Huang

Charge-stabilized colloidal spheres dispersed in deionized water are supposed to repel each other. Instead, artifact-corrected video microscopy measurements reveal an anomalous long-ranged like-charge attraction in the interparticle pair…

软凝聚态物质 · 物理学 2009-11-11 Marco Polin , David G. Grier , Yilong Han

We present an overview of our understanding of electrostatic interactions between charged macromolecular surfaces mediated by mobile counter- and coions. The dichotomy between the weak and the strong coupling regimes is described in detail…

软凝聚态物质 · 物理学 2016-12-21 Ali Naji , Matej Kanduc , Roland R. Netz , Rudolf Podgornik

Electrostatic interactions involving proteins depend not just on the ionic charges involved but also on their chemical identities. Here we examine the origins of incompletely understood differences in the strength of association of…

化学物理 · 物理学 2023-08-15 Chase E. Herman , Arjun Valiya Parambathu , D. N. Asthagiri , Abraham M. Lenhoff

Electrostatic polarization is important in many nano-/micro-scale physical systems such as colloidal suspensions, biopolymers, and nanomaterials assembly. The calculation of polarization potential requires an efficient algorithm for solving…

软凝聚态物质 · 物理学 2015-06-11 Zhenli Xu

As proteins typically have charges of around 10, they will interact strongly with charged surfaces. We calculate the electrostatic contribution to the interaction of crystals of protein with charged surfaces. The surfaces repel like-charged…

软凝聚态物质 · 物理学 2009-11-10 Richard P. Sear

As is well known in electrolyte theory, electrostatic fields are attenuated by the presence of mobile charges in the solution. This seems to limit the possibility of an electrostatic repulsion model of biological interactions such as cell…

生物物理 · 物理学 2012-01-04 Eshel Faraggi

Field induced assembly of reconfigurable structures with complex hierarchical configurations has recently become an area of intense research with the promise for exciting applications in programmable self-assembly and nano/microstructure…

软凝聚态物质 · 物理学 2026-01-14 Indira Barros , Sayanth Ramachandran , Indrani Chakraborty
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