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Optical conductivity spectra of cubic pyrochlore $Y_{2-x} Bi_x Ru_2 O_7$ (0.0$\leq ${\it x}$\leq $2.0) compounds are investigated. As a metal-insulator transition (MIT) occurs around {\it x}$=$0.8, large spectral changes are observed. With…

强关联电子 · 物理学 2009-11-11 J. S. Lee , S. J. Moon , T. W. Noh , T. Takeda , R. Kanno , S. Yoshii , M. Sato

The filling-controlled metal-insulator transition (MIT) in a two-dimensional Mott-Hubbard system La1.17-xPbxVS3.17 has been studied by photoemission spectroscopy. With Pb substitution x, chemical potential mu abruptly jumps by ~ 0.07 eV…

强关联电子 · 物理学 2009-11-10 A. Ino , T. Okane , S. -I. Fujimori , A. Fujimori , T. Mizokawa , Y. Yasui , T. Nishikawa , M. Sato

Carrier doping to the Mott insulator is essential to produce highly correlated metals with emergent properties. Pyrochlore ruthenates, Pr$_{2}$Ru$_{2}$O$_{7}$ (Ru-$4d$ electron number, $n=4$) and Ca$_{2}$Ru$_{2}$O$_{7}$ ($n=3$), are a Mott…

Insulator-to-metal transition in Ca$_{2}$RuO$_{4}$ has drawn keen attention because of its sensitivity to various stimulation and its potential controllability. Here, we report a direct observation of Fermi surface, which emerges upon…

Eu2Ir2O7, a candidate Weyl semimetal, shows an insulator-to-metal transition as a function of Bi substitution at the Eu site. In this work, we investigate the (Eu_1-xBi_x)2Ir2O7 series via Hard X-ray Photoemission Spectroscopy (HAXPES),…

强关联电子 · 物理学 2021-01-29 Prachi Telang , Kshiti Mishra , Rabindranath Bag , A. Gloskovskii , Yu. Matveyev , Surjeet Singh

First principles density functional calculations within the local spin density approximation (LSDA) and the generalized gradient approximation (GGA) are reported for pyrochlore Cd$_2$Os$_2$O$_7$ and Cd$_{2}$Re$_{2}$O$_7$. The transition…

凝聚态物理 · 物理学 2009-11-07 D. J. Singh , P. Blaha , K. Schwarz , J. O. Sofo

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

We conduct a comprehensive \textit{ab initio} investigation of electron-electron interactions within the pyrochlore structures of R$_2$Ru$_2$O$_7$, R$_2$Ir$_2$O$_7$, Ca$_2$Ru$_2$O$_7$, and Cd$_2$Ru$_2$O$_7$, where R denotes a rare-earth…

强关联电子 · 物理学 2024-09-04 Jianyu Li , Ji Liu , Mingjun Han , Waqas Haider , Yusuke Nomura , Ho-Kin Tang

La-doped and Y-doped Bi2Sr2CaCu2O8+d (Bi2212) compounds Bi2Sr2-xLax(Ca,Y)Cu2O8+d, which range from the insulator to the deeply underdoped superconductor, have been studied by angle-resolved photoemission spectroscopy. We have observed that…

超导电性 · 物理学 2010-04-12 K. Tanaka , T. Yoshida , K. M. Shen , D. H. Lu , W. S. Lee , H. Yagi , A. Fujimori , Z. -X. Shen , Risdiana , T. Fujii , I. Terasaki

We have studied the chemical potential shift in the high-temperature superconductor Bi$_2$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ({\it R} = Pr, Er), where the hole concentration is varied from 0.025 to 0.17 per Cu, by precise…

超导电性 · 物理学 2009-11-07 N. Harima , A. Fujimori , T. Sugaya , I. Terasaki

Single crystals of the perovskite-type $3d^{1}$ metallic alloy system Ca$_{1-x}$Sr$_x$VO$_3$ were synthesized in order to investigate metallic properties near the Mott transition. The substitution of a Ca$^{2+}$ ion for a Sr$^{2+}$ ion…

强关联电子 · 物理学 2009-10-31 I. H. Inoue , O. Goto , H. Makino , N. E. Hussey , M. Ishikawa

We investigated the electronic structures of the bandwidth-controlled ruthenates, Y$_{2}$Ru$_{2}$O$_{7}$, CaRuO$_{3}$, SrRuO$_{3}$, and Bi$_{2}$Ru$% _{2}$O$_{7}$, by optical conductivity analysis in a wide energy region of 5 meV $\sim $ 12…

强关联电子 · 物理学 2009-11-07 J. S. Lee , Y. S. Lee , T. W. Noh , K. Char , Jonghyurk Park , S. -J. Oh , J. -H. Park , C. B. Eom , T. Takeda , R. Kanno

We investigated the electronic structures of the 5$d$ Ruddlesden-Popper series Sr$_{n+1}$Ir$_{n}$O$_{3n+1}$ ($n$=1, 2, and $\infty$) using optical spectroscopy and first-principles calculations. As 5$d$ orbitals are spatially more extended…

强关联电子 · 物理学 2009-11-13 S. J. Moon , H. Jin , K. W. Kim , W. S. Choi , Y. S. Lee , J. Yu , G. Cao , A. Sumi , H. Funakubo , C. Bernhard , T. W. Noh

Numerical studies on Mott transitions caused by the control of the ratio between bandwidth and electron-electron interaction ($U$) are reported. By using the recently proposed path-integral renormalization group(PIRG) algorithm, physical…

强关联电子 · 物理学 2007-05-23 Tsuyoshi Kashima , Masatoshi Imada

In the two-dimensional organic charge-transfer salts kappa-(BEDT-TTF)2Cu[N(CN)2]Br{x}Cl{1-x} a systematic variation of the Br content from x = 0 to 0.9 allows us to tune the Mott transition by increasing the bandwidth. At temperatures below…

We report on the evolution of the thermal metal-insulator transition in polycrystalline samples of Nd$_2$Ir$_2$O$_7$ upon hole-doping via substitution of Ca$^{2+}$ for Nd$^{3+}$. Ca substitution mediates a filling-controlled Mott-like…

We investigate the nature and origin of the metal-insulator transition in Sr2Ru1-xTixO4 as a function of increasing Ti content (x). Employing detailed core, valence, and conduction band studies with x-ray and ultraviolet photoelectron…

强关联电子 · 物理学 2009-11-11 Sugata Ray , D. D. Sarma , R. Vijayaraghavan

NiS$_2$ has been widely regarded as a model system to study the bandwidth-controlled Mott transition, as enabled by isovalent Se chemical substitution on the S sites. Motivated by advances in electrolyte gating, we theoretically investigate…

强关联电子 · 物理学 2023-03-15 Ezra Day-Roberts , Rafael M. Fernandes , Turan Birol

We report a study of magnetic, thermal, and transport properties of La(3+) substituted Sr2RuO4, performed in order to investigate the effects of additional electron doping in this correlated metal. A gradual enhancement of the electronic…

强关联电子 · 物理学 2007-05-23 N. Kikugawa , C. Bergemann , A. P. Mackenzie , Y. Maeno

We have investigated the electronic structure of polycrystalline Ca$_2$FeReO$_6$ using photoemission spectroscopy and band-structure calculations within the local-density approximation+$U$ (LDA+$U$) scheme. In valence-band photoemission…

强关联电子 · 物理学 2009-11-10 H. Iwasawa , T. Saitoh , Y. Yamashita , D. Ishii , H. Kato , N. Hamada , Y. Tokura , D. D. Sarma
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