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New Raman and incoherent neutron scattering data at various temperatures and molecular dynamic simulations in amorphous silica, are compared to obtain the Raman coupling coefficient $C(\omega)$ and, in particular, its low frequency limit.…

无序系统与神经网络 · 物理学 2009-10-31 A. Fontana , R. Dell'Anna , M. Montagna , F. Rossi , G. Viliani , G. Ruocco , M. Sampoli , U. Buchenau , A. Wischnewski

Low-frequency Raman coupling coefficient of 11 different glasses is evaluated. It is found that the coupling coefficient demonstrates a universal linear frequency behavior near the boson peak maximum and a superlinear behavior at very low…

材料科学 · 物理学 2009-11-07 N. V. Surovtsev , A. P. Sokolov

The effects of plasticization of poly(methyl methacrylate) glass on the boson peaks observed by Raman and neutron scattering are compared. In plasticized glass the cohesion heterogeneities are responsible for the neutron boson peak and…

凝聚态物理 · 物理学 2007-05-23 E. Duval , L. Saviot , A. Mermet , L. David , S. Etienne , V. Bershtein , A. J. Dianoux

We show that a {\em vibrational instability} of the spectrum of weakly interacting quasi-local harmonic modes creates the maximum in the inelastic scattering intensity in glasses, the Boson peak. The instability, limited by anharmonicity,…

无序系统与神经网络 · 物理学 2009-11-07 V. L. Gurevich , D. A. Parshin , H. R. Schober

Inelastic light scattering is an intensively used tool in the study of electronic properties of solids. Triggered by the discovery of high temperature superconductivity in the cuprates and by new developments in instrumentation, light…

强关联电子 · 物理学 2009-11-11 T. P. Devereaux , R. Hackl

Hyper-Raman scattering spectra of vitreous B$_2$O$_3$ are reported and compared to Raman scattering results. The main features are indexed in terms of vibrations of structural units. Particular attention is given to the low frequency boson…

无序系统与神经网络 · 物理学 2009-11-11 G. Simon , B. Hehlen , E. Courtens , E. Longueteau , R. Vacher

We use the symmetry constrained low energy effective Hamiltonian of iron based superconductors to study the Raman scattering in the normal state of underdoped iron-based superconductors. The incoming and scattered Raman photons couple…

强关联电子 · 物理学 2015-07-01 M. Khodas , A. Levchenko

In this Letter we analyze theoretically how the emergence of collective strong coupling between vibrational excitations and confined cavity modes affects Raman scattering processes. This work is motivated by recent experiments [Shalabney et…

介观与纳米尺度物理 · 物理学 2016-11-10 Javier del Pino , Johannes Feist , F. J. García-Vidal

Strong coupling between cavity photons and molecular vibrations can lead to the formation of vibron-polaritons. In a recent experiment with PVAc molecules in a metal-metal microcavity [A.Shalabney et al., Ang.Chem.Int.Ed. 54 7971 (2015)],…

光学 · 物理学 2016-08-31 Artem Strashko , Jonathan Keeling

Resonant inelastic (Raman) light scattering off neutral GaAs quantum dots which contain a mean number, N=42, of electron-hole pairs is computed. We find Raman amplitudes corresponding to strongly collective final states (charge-density…

介观与纳米尺度物理 · 物理学 2009-11-07 Alain Delgado , Augusto Gonzalez , Eduardo Menendez-Proupin

Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

The Raman response of the metallic glass Ni$_{67}$Zr$_{33}$ is measured as a function of polarization and temperature and analyzed theoretically. Unexpectedly, the intensity in the range up to 300\wn increases upon cooling, which is…

无序系统与神经网络 · 物理学 2015-05-20 B. Muschler , I. Tüttő , A. Zawadowski , J. Balogh , R. Hackl

We use dynamical mean field theory to find an exact solution for inelastic light scattering in strongly correlated materials such as those near a quantum-critical metal-insulator transition. We evaluate the results for $\textbf{q}=0$…

强关联电子 · 物理学 2009-11-10 A. M. Shvaika , O. Vorobyov , J. K. Freericks , T. P. Devereaux

Anelastic light scattering is computed numerically for model disordered systems (linear chains and 2-dimensional site and bond percolators), with and without electrical disorder. A detailed analysis of the vibrational modes and of their…

凝聚态物理 · 物理学 2015-06-25 P. Benassi , W. Frizzera , M. Montagna , G. Viliani , V. Mazzacurati , G. Ruocco , G. Signorelli , .

Incoherent neutron scattering experiments are simulated for simple dynamic models: a glass (with a smooth distribution of harmonic vibrations) and a viscous liquid (described by schematic mode-coupling equations). In most situations…

软凝聚态物质 · 物理学 2009-10-31 Joachim Wuttke

A consistent calculation of resonant inelastic (Raman) scattering amplitudes for relatively large quantum dots, which takes account of valence-band mixing, discrete character of the spectrum in intermediate and final states, and…

介观与纳米尺度物理 · 物理学 2009-11-10 Alain Delgado , Augusto Gonzalez

Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…

无序系统与神经网络 · 物理学 2009-10-31 L. Saviot , E. Duval , J. F. Jal , A. J. Dianoux

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

介观与纳米尺度物理 · 物理学 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller

The scaling behavior of the so-called boson peak in glass-formers and its relation to the elastic properties of the system remains a source of controversy. Here, the boson peak in a binary reactive mixture is measured by Raman scattering…

软凝聚态物质 · 物理学 2013-08-06 Silvia Corezzi , Silvia Caponi , Flavio Rossi , Daniele Fioretto

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

光学 · 物理学 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran
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