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The assembly of colloidal cubic diamond is a challenging process since the shape and interaction parameters and the thermodynamic conditions where this structure is stable are elusive. The simultaneous use of shape-anisotropic particles and…

软凝聚态物质 · 物理学 2024-06-12 Susana Marín-Aguilar , Fabrizio Camerin , Marjolein Dijkstra

Microfluidic chips provide unparalleled control over droplets and jets, which have advanced all natural sciences. However, microfluidic applications could be vastly expanded by increasing the per-channel throughput and directly exploiting…

流体动力学 · 物理学 2020-02-06 Claas Willem Visser , Tom Kamperman , Lisanne P. Karbaat , Detlef Lohse , Marcel Karperien

Colloids are abundant in nature, science and technology, with examples ranging from milk to quantum dots and the "colloidal atom" paradigm. Similarly, liquid crystal ordering is important in contexts ranging from biological membranes to…

软凝聚态物质 · 物理学 2017-12-29 Ivan I. Smalyukh

We demonstrate a novel route of spatially organizing the colloid arrangements on the polymer-grafted substrate by use of self-consistent field and density functional theories. We find that grafting of polymers onto a substrate can…

软凝聚态物质 · 物理学 2007-05-23 Kang Chen , Yu-qiang Ma

The directed self-assembly of colloidal nanoparticles (NPs) using external fields guides the formation of sophisticated hierarchical materials but becomes less effective with decreasing particle size. As an alternative, electron-beam-driven…

软凝聚态物质 · 物理学 2024-09-13 Jonathan G. Raybin , Ethan J. Dunsworth , Veronica Guo , Naomi S. Ginsberg

We exploit the long-ranged elastic fields inherent to confined nematic liquid crystals to assemble colloidal particles trapped at the liquid crystal interface into reconfigurable structures with complex symmetries and packings. Spherical…

Anisotropy at the level of the inter-particle interaction provides the particles with specific instructions for the self-assembly of target structures. The ability to synthesize non-spherical colloids, together with the possibility of…

软凝聚态物质 · 物理学 2020-01-03 Carina Karner , Christoph Dellago , Emanuela Bianchi

Building structures with hierarchical order through the self-assembly of smaller blocks is not only a prerogative of nature, but also a strategy to design artificial materials with tailored functions. We explore in simulation the…

软凝聚态物质 · 物理学 2020-02-17 Santi Prestipino , Domenico Gazzillo , Gianmarco Munaò , Dino Costa

Organic capping ligands can selectively bind to crystal facets to modulate growth kinetics and are important in chemical synthesis of inorganic nanocrystals. Using the capping ligands for shape-controlled growth of colloidal crystals is…

软凝聚态物质 · 物理学 2025-11-11 Rui Huang , Jordan Austin-Frank Wilson , Allen Sun , Artemis Harlow , Zhiwei Li

Hierarchical self-assembly consisting of local associations of simple building-blocks for the formation of complex structures widely exists in nature, while the essential role of local assembly remains unknown. In this work, by using…

软凝聚态物质 · 物理学 2017-10-18 Qun-li Lei , Kunn Hadinoto , Ran Ni

Colloidal systems find important applications ranging from fabrication of photonic crystals to direct probing of phenomena typically encountered in atomic crystals and glasses. New applications - such as nanoantennas, plasmonic sensors, and…

软凝聚态物质 · 物理学 2016-12-30 Rahul P. Trivedi , Ivan I. Klevets , Bohdan Senyuk , Taewoo Lee , Ivan I. Smalyukh

Understanding the out-of equilibrium behaviour of point defects in crystals, yields insights into the nature and fragility of the ordered state, as well as being of great practical importance. In some rare cases defects are spontaneously…

软凝聚态物质 · 物理学 2013-10-14 William T. M. Irvine , Mark J. Bowick , Paul M. Chaikin

Using controlled spinodal decomposition, we have created a fluid-bicontinuous structure stabilized by colloidal particles. We present confocal microscopy studies of these structures and their variation with kinetic pathway. Our studies…

We present confocal microscopy studies of novel particle-stabilized emulsions. The novelty arises because the immiscible fluids have an accessible upper critical solution temperature. The emulsions have been created by beginning with…

软凝聚态物质 · 物理学 2009-11-11 P. S. Clegg , E. M. Herzig , A. B. Schofield , T. S. Horozov , B. P. Binks , M. E. Cates , W. C. K. Poon

Colloidal particles with appropriate wetting properties can become very strongly trapped at an interface between two immiscible fluids. We have harnessed this phenomenon to create a new class of soft materials with intriguing and…

软凝聚态物质 · 物理学 2009-11-13 K. A. White , A. B. Schofield , B. P. Binks , P. S. Clegg

Crystalline films offer various physical properties based on the modulation of their thicknesses and atomic structures. The layer-by-layer assembly of atomically thin crystals provides powerful means to arbitrarily design films at the…

Two-dimensional (2D) layered materials, demonstrating significantly different properties from their bulk counterparts, offer a materials platform with potential applications from energy to information processing devices. Although some…

介观与纳米尺度物理 · 物理学 2021-07-13 Georgios A. Tritsaris , Stephen Carr , Gabriel R. Schleder

We report observations of the self-assembly of coated droplets into regular clusters at the sudden expansion of a microfluidic channel. A double emulsion consisting of a regular train of coated microdroplets was created upstream of the…

软凝聚态物质 · 物理学 2020-10-19 Kerstin Schirrmann , Gabriel Cáceres-Aravena , Anne Juel

Self-assembly is traditionally described as the process through which an initially disordered system relaxes towards an equilibrium ordered phase only driven by local interactions between its building blocks. However, This definition is too…

软凝聚态物质 · 物理学 2015-06-15 Lorenzo Di Michele , Francesco Varrato , Jurij Kotar , Simon H. Nathan , Giuseppe Foffi , Erika Eiser

Colloidal particles trapped at an interface between two fluids can form a wide range of different structures. Replacing one of the fluid with a liquid crystal increases the complexity of interactions and results in a greater range of…

软凝聚态物质 · 物理学 2014-03-20 Anne Claire Pawsey , Juho Lintuvuori