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Density functional methods were developed, in which the Coulomb electron-electron interaction is split into a long- and a short-range part. In such methods, one term is calculated using traditional density functional approximations, like…

化学物理 · 物理学 2007-05-23 Julien Toulouse , Andreas Savin

We calculate the ground state energies of a system of two dipolar fermions trapped in a harmonic oscillator potential. The dipoles are assumed to be aligned parallel to each other. We perform the calculations of ground state energy as a…

原子与分子团簇 · 物理学 2014-10-09 Amit K. Das , Arup Banerjee

We re-adapt a spectral renormalization method, introduced in nonlinear optics, to solve the Kohn-Sham (KS) equations of density functional theory (DFT), with a focus on functionals based on the strictly-correlated electrons (SCE) regime,…

强关联电子 · 物理学 2020-04-23 Juri Grossi , Ziad H. Musslimani , Michael Seidl , Paola Gori-Giorgi

One key issue in the probability density function (PDF) approach for disperse two-phase turbulent flows is to close the diffusion term in the phase space. This study aimed to derive a kinetic equation for particle dispersion in turbulent…

统计力学 · 物理学 2020-07-15 De-yu Zhong , Guang-qian Wang , Tie-jian Li , Ming-xi Zhang , You Xia

We consider density functionals for exchange and correlation energies in two-dimensional systems. The functionals are constructed by making use of exact constraints for the angular averages of the corresponding exchange and correlation…

强关联电子 · 物理学 2010-02-25 E. Rasanen , S. Pittalis

Modern extensions of density functional theory such as the density functional theory plus U and the density functional theory plus dynamical mean-field theory require choices, including selection of variable (charge vs spin density) for the…

强关联电子 · 物理学 2015-05-04 Hyowon Park , Andrew J. Millis , Chris A. Marianetti

We put forward a general procedure to obtain an approximate free energy density functional for any hard-core lattice gas, regardless of the shape of the particles, the underlying lattice or the dimension of the system. The procedure is…

统计力学 · 物理学 2007-05-23 Luis Lafuente , Jose A. Cuesta

This work presents a microscopic study of dissipation in fission dynamical evolutions with the time-dependent Hartree-Fock+BCS method in terms of energy dependence and pairing dependence. The friction coefficients and dissipation energies…

核理论 · 物理学 2021-11-24 Yu Qiang , Junchen Pei

Coupled-cluster calculations of static electronic dipole polarizabilities for 145 organic molecules are performed to create a reference data set. The molecules are composed from carbon, hydrogen, nitrogen, oxygen, fluorine, sulfur,…

化学物理 · 物理学 2015-07-28 Taozhe Wu , Yulia N. Kalugina , Ajit J. Thakkar

Coordinate scaling of each spin density separately is considered in spin density functional theory. A virial theorem relates the spin-scaled correlation energy to the spin-scaled correlation potentials. An adiabatic connection formula…

材料科学 · 物理学 2009-11-07 R. J. Magyar , T. K. Whittingham , K. Burke

Stochastic density functional theory is applied to analyze the conductivity of strong two species electrolytes at arbitrary field strengths. The corresponding stochastic equations for the density of the electrolyte species are solved by…

统计力学 · 物理学 2016-05-04 Vincent Démery , David S Dean

Standard density functional approximations often give questionable results for odd-electron radical complexes, with the error typically attributed to self-interaction. In density corrected density functional theory (DC-DFT), certain classes…

化学物理 · 物理学 2015-06-19 Min-Cheol Kim , Eunji Sim , Kieron Burke

The functional renormalization group method is used to take into account the vacuum polarization around localized bound states generated by external potential. The application to Atomic Physics leads to improved Hartree-Fock and Kohn-Sham…

强关联电子 · 物理学 2007-05-23 Janos Polonyi

In the framework of density functional theory, scaling and the virial theorem are essential tools for deriving exact properties of density functionals. Preexisting mathematical difficulties in deriving the virial theorem via scaling for…

其他凝聚态物理 · 物理学 2014-06-18 H. Mirhosseini , A. Cangi , T. Baldsiefen , A. Sanna , C. R. Proetto , E. K. U. Gross

By introducing a set of auxiliary equations representing a many-body system, we have derived an extension of the Kohn-Sham scheme for the density functional theory. These equations consist of a Kohn-Sham-type equation determining…

材料科学 · 物理学 2009-11-07 Koichi Kusakabe

Projected Hartree-Fock theory provides an accurate description of many kinds of strong correlations but does not properly describe weakly-correlated systems. On the other hand, single-reference methods such as configuration interaction or…

强关联电子 · 物理学 2022-04-06 Ruiheng Song , Thomas M. Henderson , Gustavo E. Scuseria

We present a numerical study of a trapped binary Bose-condensed gas by solving the corresponding Hartree-Fock equations. The density profile of the binary Bose gas is solved with a harmonic trapping potential as a function of temperature in…

软凝聚态物质 · 物理学 2015-06-25 P. Ohberg , S. Stenholm

We calculate the Hartree-Fock energy of a density-wave in a spin polarized two-dimensional electron gas using a short-range repulsive interaction. We find that the stable ground state for a short-range potential is always either the…

强关联电子 · 物理学 2009-11-10 Juana Moreno , D. C. Marinescu

An atom placed inside a cavity of finite dimension offers many interesting features, and thus has been a topic of great current activity. This work proposes a density functional approach to pursue both ground and excited states of a…

量子物理 · 物理学 2022-05-20 Sangita Majumdar , Amlan K. Roy

A bivariate perspective on Kohn-Sham density functional theory is proposed, treating potential and density as simultaneous independent variables, and used to make fruitful connection between Lieb's rigorous foundational framework and…

材料科学 · 物理学 2020-07-07 Paul E. Lammert
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