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We study the electronic properties of DNA by way of a tight-binding model applied to four particular DNA sequences. The charge transfer properties are presented in terms of localisation lengths, crudely speaking the length over which…

基因组学 · 定量生物学 2007-05-23 Daphne Klotsa , Rudolf A. Roemer , Matthew S. Turner

Charge migration along DNA molecules has attracted scientific interest for over half a century. Reports on possible high rates of charge transfer between donor and acceptor through the DNA, obtained in the last decade from solution…

材料科学 · 物理学 2009-11-10 Danny Porath , Gianaurelio Cuniberti , Rosa Di Felice

We study electronic transport in long DNA chains using the tight-binding approach for a ladder-like model of DNA. We find insulating behavior with localizaton lengths xi ~ 25 in units of average base-pair seperation. Furthermore, we observe…

软凝聚态物质 · 物理学 2007-05-23 Antonio Rodriguez , Rudolf A. Roemer , Matthew S. Turner

Quantum transport for DNA conduction has widely studied with interest in application as a candidate in making nanowires as well as interest in the scientific mechanism. In this paper, we review recent works with concerning the electronic…

无序系统与神经网络 · 物理学 2015-03-13 Hiroaki Yamada , Kazumoto Iguchi

Measurements of electron transfer rates as well as of charge transport characteristics in DNA produced a number of seemingly contradictory results, ranging from insulating behaviour to the suggestion that DNA is an efficient medium for…

软凝聚态物质 · 物理学 2007-05-23 R. Bulla , R. Gutierrez , G. Cuniberti

A theoretical study is presented to quantitatively analyze the transport experiment through individual DNA molecules reported recently by Porath {\it et al.} [Nature {\bf 403}, 635 (2000)]. A variety of valuable quantities are identified by…

介观与纳米尺度物理 · 物理学 2009-11-07 Xin-Qi Li , YiJing Yan

The rapid progress in the field of molecular electronics has led to an increasing interest on DNA oligomers as possible components of electronic circuits at the nanoscale. For this, however, an understanding of charge transfer and transport…

软凝聚态物质 · 物理学 2007-05-23 R. Gutierrez , G. Cuniberti

Charge transfer can take place along double helical DNA over distances as long as 30 nanometers. However, given the active role of the thermal environment surrounding charge carriers in DNA, physical mechanisms driving the transfer process…

介观与纳米尺度物理 · 物理学 2020-12-04 Roman Korol , Dvira Segal

Nucleic acids and proteins are not only biologically important polymers: They have recently been recognized as novel functional materials surpassing in many aspects the conventional ones. Although Herculean efforts have been undertaken to…

软凝聚态物质 · 物理学 2010-06-17 Waleed Shinwari , Jamal Deen , Evgeni Starikov , Gianaurelio Cuniberti

Long range charge transfer experiments in DNA oligomers and the subsequently measured -- and very diverse -- transport response of DNA wires in solid state experiments exemplifies the need for a thorough theoretical understanding of charge…

基因组学 · 定量生物学 2015-05-13 G. Cuniberti , E. Macia , A. Rodriguez , R. A. Römer

The bias-dependent transport properties of short poly(G)-poly(C) A-DNA strands attached to Au electrodes are investigated with first principles electronic transport methods. By using the non- equilibrium Green's function approach combined…

介观与纳米尺度物理 · 物理学 2015-05-19 C. D. Pemmaraju , I. Rungger , X. Chen , A. R. Rocha , S. Sanvito

The complex mechanisms governing charge migration in DNA oligomers reflect the rich structural and electronic properties of the molecule of life. Controlling the mechanical stability of DNA nanowires in charge transport experiments is a…

介观与纳米尺度物理 · 物理学 2015-05-13 Bo Song , Marcus Elstner , Gianaurelio Cuniberti

In the field of DNA nanotechnology, it is common wisdom that charge transport occurs through the {\pi} stacked bases of double-stranded DNA. However, recent experimental findings by Zhuravel et. al. [Nat. Nanotech. 15, 836 (2020)] suggest…

介观与纳米尺度物理 · 物理学 2024-12-31 Sourav Kundu , Siddhartha Lal

We report theoretical studies of charge transport in single-stranded DNA in the direction perpendicular to the backbone axis. We find that, if the electrodes which sandwich the DNA have the appropriate spatial width, each nucleotide carries…

其他凝聚态物理 · 物理学 2010-11-03 Michael Zwolak , Massimiliano Di Ventra

Microscopic mechanisms of positive charge transfer in DNA remain unclear. A quantum state of electron hole in DNA is determined by the competition of a pi-stacking interaction $b$ smearing a charge between different base pairs and…

软凝聚态物质 · 物理学 2008-03-15 D. B. Uskov , A. L. Burin

Charge diffusion through desoxyribonucleic acid (DNA) is a physico-chemical phenomenon that on the one hand is being explored for technological purposes, on the other hand is applied by nature for various informational processes in life.…

生物物理 · 物理学 2024-07-22 Mirko Rossini , Ole Ammerpohl , Reiner Siebert , Joachim Ankerhold

An 1d model with time-dependent random hopping is proposed to describe charge transport in DNA. It admits to investigate both diffusion of electrons and their tunneling between different sites in DNA. The tunneling appears to be strongly…

软凝聚态物质 · 物理学 2009-11-07 E. I. Kats , V. V. Lebedev

We present a short review of various experiments that measure charge transfer and charge transport in DNA. Some general comments are made on the possible connection between 'chemistry-style' charge transfer experiments that probe…

无序系统与神经网络 · 物理学 2009-11-10 N. P. Armitage , M. Briman , G. Gruner

The electrical properties of DNA molecules are investigated by charge injection and electric force microscopy experiments. Prior to injection, DNA molecules exhibit a weak positively charged state. We probe the electrical behaviour of DNA…

材料科学 · 物理学 2009-11-10 Thomas Heim , Thierry Melin , Dominique Deresmes , Dominique Vuillaume

By resorting to a model inspired to the standard Davydov and Holstein-Fr\"ohlich models, in the present paper we study the motion of an electron along a chain of heavy particles modelling a sequence of nucleotides proper to a DNA fragment.…

生物物理 · 物理学 2021-08-17 Elham Faraji , Roberto Franzosi , Stefano Mancini , Marco Pettini
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