相关论文: Igniting homogeneous nucleation
Classical nucleation theory (CNT), linking rare nucleation events to the free energy landscape of a growing nucleus, is central to understanding phase-change kinetics in passive fluids. Nucleation in non-equilibrium systems is much harder…
Recent very large molecular dynamics simulations of homogeneous nucleation with $(1-8) \cdot 10^9$ Lennard-Jones atoms [Diemand et al. J. Chem. Phys. {\bf 139}, 074309 (2013)] allow us to accurately determine the formation free energy of…
A dissipation rate, which grows faster than any power of the wave number in Fourier space, may be scaled to lead a hydrodynamic system {\it actually} or {\it potentially} converge to its Galerkin truncation. Actual convergence we name for…
Understanding the pathways to crystallization during the deposition of a vapor phase on a cold solid substrate is of great interest in industry, e.g., for the realization of electronic devices made of crystallites-free glassy materials, as…
Detailed measurements of the cosmic microwave background indicate the large-scale homogeneity of the universe. On very small scales, we observe however inhomogeneities such as galaxies, stars, planets and ourselves. In the context of hot…
The phase diagram of the monoaxial chiral helimagnet as a function of temperature (T ) and magnetic field with components perpendicular (H x ) and parallel (H z ) to the chiral axis is theoretically studied via the variational mean field…
The task of a first principles theoretical calculation of the rate of gas to liquid nucleation has remained largely incomplete despite the existence of reliable results from unbiased simulation studies at large supersaturation. Although the…
We propose a new model for the nature of the nucleation of solid from the superfluid phases of $^4$He and $^3$He. Unique to the superfluid phases the solid nucleation involves an extremely fast solidification front. This results in a local…
Nanoparticle agglomeration in a quiescent fluid is simulated by solving the Langevin equations of motion of a set of interacting monomers in the continuum regime. Monomers interact via a radial, rapidly decaying intermonomer potential. The…
The basic notion of percolation in physics assumes the emergence of a giant connected (percolation) cluster in a large disordered system when the density of connections exceeds some critical value. Until recently, the percolation phase…
Statistical aspects of the dynamics of chaotic scattering in the classical model of $\alpha$-cluster nuclei are studied. It is found that the dynamics governed by hyperbolic instabilities which results in an exponential decay of the…
Strongly first-order phase transitions, i.e., those with a large order parameter, are characterized by a considerable supercooling and high velocities of phase transition fronts. A very strong phase transition may have important…
We study the dynamical formation of disoriented chiral condensates in very high energy nucleus-nucleus collisions using Bjorken hydrodynamics and relativistic nucleation theory. It is the dynamics of the first order confinement phase…
This work addresses nucleation rates in systems with strong initial recombination. Initial (or `geminate') recombination is a process where a dissociated structure (anion, vortex, kink etc.) recombines with its twin brother (cation,…
One possible way in which phase transitions in the early universe may have ocurred is via nucleation of bubbles of the new phase (true vacuum) in the old phase (false vacuum). The technique most widely used to compute the probability of…
We develop a theory of various kinds of large-scale clustering of inertial particles in a rotating density stratified or inhomogeneous turbulent fluid flows. The large-scale particle clustering occurs in scales which are much larger than…
Motivated by recent time domain experiments on ultrafast atom ionization, we analyze the transients and timescales that characterize, besides the relatively long lifetime, the decay by tunneling of a localized state. While the tunneling…
There are not many kinetic models where it is possible to prove bifurcation phenomena for any value of the Knudsen number. Here we consider a binary mixture over a line with collisions and long range repulsive interaction between different…
We introduce and analyse a variant of the Becker-D{\"o}ring equations that models the growth of clusters through the gain or loss of monomers. Motivated by enzymatic reactions in biology, this model incorporates irreversible fragmentation…
The familiar process of bubbles generated via breaking waves in the ocean is foundational to many natural and industrial applications. In this process, large pockets of entrained gas are successively fragmented by the ambient turbulence…