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In this review, we address the issue of the electrostatic complexation between charged-neutral diblock copolymers and oppositely charged nanocolloids. We show that nanocolloids such as surfactant micelles and iron oxide magnetic…

软凝聚态物质 · 物理学 2011-02-01 J. -F. Berret

We report on the formation and the structural properties of supermicellar aggregates also called electrostatic complexes, made from mineral nanoparticles and polyelectrolyte-neutral block copolymers in aqueous solutions. The mineral…

软凝聚态物质 · 物理学 2007-09-10 Jean-Francois Berret , Kazuhiko Yokota , Mikel Morvan , Ralf Schweins

When polyelectrolyte-neutral block copolymers are mixed in aqueous solutions with oppositely charged species, stable complexes are found to form spontaneously. The mechanism is based on electrostatics, and on the compensation between the…

During the last 3 years, our group has investigated extensively the complexation mechanism between neutral-polyelectrolyte block copolymers with oppositely charged species. These species are surfactant micelles, multivalent counterions and…

软凝聚态物质 · 物理学 2007-05-23 J. -F. Berret , P. Herve , M. Morvan , K. Yokota , M. Destarac , J. Oberdisse , I. Grillo , R. Schweins

We report on the complexation between charged-neutral block copolymers and oppositely charged surfactants studied by small-angle neutron scattering. Two block copolymers/surfactant systems are investigated, poly(acrylic…

软凝聚态物质 · 物理学 2007-05-23 Jean-Francois Berret

We report on the formation of colloidal complexes resulting from the electrostatic self-assembly of polyelectrolyte-neutral block copolymers and oppositely charged surfactants. The copolymers investigated are asymmetric and characterized by…

软凝聚态物质 · 物理学 2007-05-23 Jean-Francois Berret , Pascal Herve , Isabelle Grillo

We report the presence of a correlation between the bulk and interfacial properties of electrostatic coacervate complexes. Complexes were obtained by co-assembly between cationic-neutral diblocks and oppositely charged surfactant micelles…

软凝聚态物质 · 物理学 2007-10-12 Ling Qi , Jean-Paul Chapel , Jean-Christophe Castaing , Jerome Fresnais , Jean-Francois Berret

Polypeptide-based diblock copolymers forming either well-defined self-assembled micelles or vesicles after direct dissolution in water or in dichloromethane, have been studied combining light and neutron scattering with electron microscopy…

During the past years we have investigated the complexation between nanocolloids and oppositely charged polymers. The nanocolloids examined were ionic surfactant micelles and inorganic oxide nanoparticles. For the polymers, we used…

软凝聚态物质 · 物理学 2007-05-23 Jean-Francois Berret , Regis Cartier

We report the co-assembly and adsorption properties of coacervate complexes made from polyelectrolyte-neutral block copolymers and oppositely charged nanocolloids. The nanocolloids put under scrutiny were ionic surfactant micelles and…

We report on the structural properties of mixed aggregates made from rare-earth inorganic nanoparticles (radius 20 Angstroms) and polyelectrolyte-neutral block copolymers in aqueous solutions. Using scattering experiments and Monte Carlo…

软凝聚态物质 · 物理学 2021-09-27 K. Yokota , M. Morvan , J. -F. Berret , J. Oberdisse

The complexation between charged-neutral block copolymers and oppositely charged surfactants was investigated by light scattering experiments and by isothermal titration calorimetry (ITC). The copolymer was poly(sodium…

材料科学 · 物理学 2011-07-27 J. Courtois , J. -F. Berret

We investigate by scattering techniques the structure of water-based soft composite materials comprising a crystal made of Pluronic block-copolymer micelles arranged in a face-centered cubic lattice and a small amount (at most 2% by volume)…

软凝聚态物质 · 物理学 2012-06-07 Elisa Tamborini , Neda Ghofraniha , Julian Oberdisse , Luca Cipelletti , Laurence Ramos

We report on the electrostatic complexation between oppositely charged polymers and inorganic nanoparticles investigated by static and dynamical light scattering. The nanoparticles put under scrutiny were citrate-coated nanocrystals of…

软凝聚态物质 · 物理学 2007-09-10 J. -F. Berret

A novel type of hybrid colloids is presented, based on the association of several polymeric systems and ferrofluids. On the one hand, we use inorganic nanoparticles made of magnetic iron oxide prepared at the LI2C, which response to a…

We report the synthesis of complex salts made from the cationic surfactant dodecyltrimethyl-ammonium and diblock copolymers poly(acrylic acid)-block-poly(acrylamide) of different molecular weights. In water, the complex salts self-assemble…

材料科学 · 物理学 2013-10-29 Leticia Vitorazi , Jean-Francois Berret , Watson Loh

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

软凝聚态物质 · 物理学 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

We report the formation of colloidal complexes resulting from the electrostatic co-assembly between anionic surfactants and cationic polyelectrolytes or block copolymers. Combining light and x-ray scattering experiments with cryogenic…

软凝聚态物质 · 物理学 2009-04-01 J. -F. Berret

Engineered nanoparticles made from noble metals, rare-earth oxides or semiconductors are emerging as the central constituents of future nanotech developments. In this review, a survey of the complexing strategies between nanoparticles and…

材料科学 · 物理学 2011-08-25 J. -P. Chapel , J. -F. Berret

We report on the electrostatic complexation between polyelectrolyte-neutral copolymers and oppositely charged 6 nm-crystalline nanoparticles. For two different dispersions of oxide nanoparticles, the electrostatic complexation gives rise to…

软凝聚态物质 · 物理学 2007-09-10 J. -F. Berret , A. Sehgal , M. Morvan , O. Sandre , A. Vacher , M. Airiau
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