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Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

无序系统与神经网络 · 物理学 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

Based on experimental evidences we present a phenomenological description of the thermal glass transition as a dynamical phase transition. Different susceptibilities calculated on the basis of this description are in good qualitative…

无序系统与神经网络 · 物理学 2016-08-16 J. K. Krüger , J. Petersson , J. Baller , M. Henkel

A core-softened model of a glass forming fluid is numerically studied in the limit of very low temperatures. The model shows two qualitatively different behaviors depending on the strength of the attraction between particles. For no or low…

统计力学 · 物理学 2009-11-07 E. A. Jagla

The thermodynamic and kinetic anomalies of supercooled liquids are analyzed from the perspective of energy landscapes. A mean field model, a generalized random energy model of liquids is developed, which exhibits a dynamical transition of…

软凝聚态物质 · 物理学 2009-11-10 Masaki Sasai

We analyse numerically thermal fluctuations of the static overlap between equilibrium configurations in a glass-forming liquid approaching the glass transition. We find that the emergence of slow dynamics near the onset temperature…

统计力学 · 物理学 2013-08-23 Ludovic Berthier

We review the available experimental information on the thermodynamic properties of supercooled ordinary and heavy water and demonstrate the possibility of modeling these thermodynamic properties on a theoretical basis. We show that by…

化学物理 · 物理学 2013-02-25 V. Holten , C. E. Bertrand , M. A. Anisimov , J. V. Sengers

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

软凝聚态物质 · 物理学 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

The description of molecular motion by macroscopic hydrodynamics has a long and continuing history. The Stokes-Einstein relation between the diffusion coefficient of a solute and the solvent viscosity predicted using macroscopic continuum…

无序系统与神经网络 · 物理学 2007-05-23 Xiaoyu Xia , Peter G. Wolynes

The fragility, that controls the temperature-dependent viscous properties of liquids as the glass transition is approached, in various glass-forming liquids with different atomic interactions and densities is investigated by molecular…

软凝聚态物质 · 物理学 2016-08-03 Lijin Wang , Pengfei Guan , W. H. Wang

In this paper, we discuss theoretically the behavior of the four point nonlinear susceptibility and its associated correlation length for supercooled liquids close to the Mode Coupling instability temperature $T_c$. We work in the…

无序系统与神经网络 · 物理学 2009-10-31 Silvio Franz , Giorgio Parisi

We present a mean-field theory of a coarse-grained model of a super-cooled liquid in which relaxation occurs via local plastic rearrangements. Local relaxation can be induced by thermal fluctuations or by the long-range elastic consequences…

软凝聚态物质 · 物理学 2023-12-07 Joseph W. Baron , Giulio Biroli

The dynamics of supercooled liquid and glassy systems are usually studied within the Lagrangian representation, in which the positions and velocities of distinguishable interacting particles are followed. Within this representation,…

无序系统与神经网络 · 物理学 2009-09-28 Claudio Chamon , Leticia F. Cugliandolo , Gabriel Fabricius , Jose Luis Iguain , Eric R. Weeks

We introduce the ideal Gaussian glass-forming system as a model to describe the thermodynamics and dynamics of supercooled liquids on a local scale in terms of the properties of the potential energy landscape (PEL). The first ingredient is…

材料科学 · 物理学 2009-11-13 A. Heuer , A. Saksaengwijit

In this work, we study the nature of transitions between inherent structures of a two-dimensional model supercooled liquid. We demonstrate that these transitions occur predominately along a small number of directions on the energy…

统计力学 · 物理学 2013-03-12 Glen M. Hocky , David R. Reichman

The transition from a flowing to a static state in a granular material is studied using large-scale, 3D particle simulations. Similar to glasses, this transition is manifested in the development of a plateau in the contact normal force…

统计力学 · 物理学 2007-05-23 L. E. Silbert , D. Ertas , G. S. Grest , T. C. Halsey , D. Levine

We use light microscopy to investigate the aging dynamics of a glass made of closely packed soft spheres, following a rapid transition from a fluid to a solid-like state. By measuring time-resolved, coarse-grained displacements fields, we…

软凝聚态物质 · 物理学 2009-11-13 Sylvain Mazoyer , Luca Cipelletti , Laurence Ramos

As one increases the concentration of a colloidal suspension, the system exhibits a dramatic increase in viscosity. Structurally, the system resembles a liquid, yet motions within the suspension are slow enough that it can be considered…

软凝聚态物质 · 物理学 2012-05-22 Gary L. Hunter , Eric R. Weeks

As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this…

When a liquid is cooled below its melting temperature it usually crystallizes. However, if the quenching rate is fast enough, it is possible that the system remains in a disordered state, progressively losing its fluidity upon further…

无序系统与神经网络 · 物理学 2009-11-10 Tullio Scopigno , Giancarlo Ruocco , Francesco Sette , Giulio Monaco

We study the dynamical melting of "hot" one-dimensional many-body localized systems. As disorder is weakened below a critical value these non-thermal quantum glasses melt via a continuous dynamical phase transition into classical thermal…

无序系统与神经网络 · 物理学 2015-09-23 Andrew C. Potter , Romain Vasseur , S. A. Parameswaran