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We present a Monte Carlo approach to incorporating the effect of thermal fluctuations in field theories of polymeric fluids. This method is applied to a field-theoretic model of a ternary blend of AB diblock copolymers with A and B…

材料科学 · 物理学 2009-11-10 Dominik Düchs , Venkat Ganesan , Glenn H. Fredrickson , Friederike Schmid

The structure of lamellar phases of symmetric $AB$ diblock copolymers in a thin film is investigated. We quantitatively compare the composition profiles and profiles of individual segments in self-consistent field calculations with Monte…

统计力学 · 物理学 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

统计力学 · 物理学 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

Double emulsion formation in a hierarchical flow-focusing channel is systematically investigated using a free energy ternary lattice Boltzmann model. A three dimensional formation regime diagram is constructed based on the capillary numbers…

软凝聚态物质 · 物理学 2020-06-24 Ningning Wang , Ciro Semprebon , Haihu Liu , Chuhua Zhang , Halim Kusumaatmaja

The structure of polymer coils near interfaces between coexisting phases of symmetrical polymer mixtures (AB) is discussed, as well as the structure of symmetric diblock copolymers of the same chain length N adsorbed at the interface. The…

软凝聚态物质 · 物理学 2015-06-25 K. Binder , M. Mueller , F. Schmid , A. Werner

We have carried out extensive Monte Carlo simulations of the fusion of tense apposed bilayers formed by amphiphilic molecules within the framework of a coarse grained lattice model. The fusion pathway differs from the usual stalk mechanism.…

软凝聚态物质 · 物理学 2016-08-31 M. Mueller , K. Katsov , M. Schick

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

化学物理 · 物理学 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller

The interfacial profile between coexisting phases of a binary mixture (A,B) in a thin film of thickness D and lateral linear dimensions L depends sensitively on both linear dimensions and on the nature of boundary conditions and statistical…

统计力学 · 物理学 2009-10-30 Andreas Werner , Friederike Schmid , Marcus Mueller , Kurt Binder

Amphiphilic block copolymer solutions form various micellar structures including micelles and vesicles. We applied the density functional theory for block copolymers which we have proposed to amphiphilic block copolymer systems. The 3…

软凝聚态物质 · 物理学 2007-05-23 Takashi Uneyama , Masao Doi

We investigate the phase behaviour of random copolymers melts via large scale Monte Carlo simulations. We observe macrophase separation into A and B--rich phases as predicted by mean field theory only for systems with a very large…

软凝聚态物质 · 物理学 2009-11-07 J. Houdayer , M. Mueller

Reactions at a strongly segregated interface of a symmetric binary polymer blend are investigated via Monte Carlo simulations. End functionalized homopolymers of different species interact at the interface instantaneously and irreversibly…

统计力学 · 物理学 2009-10-30 Marcus Mueller

The phase separation of a simple binary mixture of incompatible linear polymers in solution is investigated using an extension of the sedimentation equilibrium method, whereby the osmotic pressure of the mixture is extracted from the…

软凝聚态物质 · 物理学 2009-09-29 Chris I. Addison , Pierre-Arnaud Artola , Jean-Pierre Hansen , Ard A. Louis

Spontaneous liquid-liquid phase separation is commonly understood in terms of phenomenological mean-field theories. These theories correctly predict the structural features of the fluid at sufficiently long time scales and wavelengths.…

软凝聚态物质 · 物理学 2019-07-11 Charley Schaefer , Stefan Paquay , Tom C. B. McLeish

To explain the appearance of heterogeneities in the plasma membrane, I propose a hypothesis which begins with the observation that fluctuations in the membrane curvature are coupled to the difference between compositions in one leaf and the…

软凝聚态物质 · 物理学 2017-08-23 M. Schick

Formation of the intermediate phase patterns in the thin-film co-deposition process is simulated using the Stochastic Kinetic Mean-Field method and Monte Carlo. Three basic morphologies of the 2D sections are distinguished: (1) spots…

材料科学 · 物理学 2024-12-05 Serhii Abakumov , Andriy Gusak

The self-assembly behaviour of a diblock copolymer-diblock copolymer mixture under an oscillating shear field is investigated via cell dynamics simulation. The results indicate that the macrophase separation of the composite system is…

软凝聚态物质 · 物理学 2024-07-02 Y. Guo , H. He , X. Fu

The formation of various bicontinuous phases from binary blends of linear AB diblock copolymers (DBCPs) is studied using the polymeric self-consistent field theory. The theoretical study predicts that the double-diamond and the "plumber's…

软凝聚态物质 · 物理学 2021-09-01 Chi To Lai , An-Chang Shi

This paper represents a model for microstructure formation in metallic foams based on the multi-phase-field (MPF) approach. By the use of a no-coalescence boundary condition within this MPF-framework, it is possible to completely prevent…

计算物理 · 物理学 2020-07-13 Samad Vakili , Ingo Steinbach , Fathollah Varnik

We study a two-component mixture of fermionic dipoles in two dimensions at zero temperature, interacting via a purely repulsive $1/r^3$ potential. This model can be realized with ultracold atoms or molecules, when their dipole moments are…

The phase structure of self-avoiding polymerized membranes is studied by extensive Hybrid Monte Carlo simulations. Several folding transitions from the flat to a collapsed state are found. Using a suitable order parameter and finite size…

凝聚态物理 · 物理学 2009-10-28 Christian Münkel , Dieter W. Heermann
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