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We present an experimental determination of the isothermal magnetic susceptibility of the spin ice materials Dy2Ti2O7 and Ho2Ti2O7 in the temperature range 1.8-300 K. The use of spherical crystals has allowed the accurate correction for…

强关联电子 · 物理学 2013-09-02 L. Bovo , L. D. C. Jaubert , P. C. W. Holdsworth , S. T. Bramwell

Traditional magnetic sub-Kelvin cooling relies on the nearly free local moments in hydrate paramagnetic salts, whose utility is hampered by the dilute magnetic ions and low thermal conductivity. Here we propose to use instead fractional…

强关联电子 · 物理学 2024-08-06 Han Li , Enze Lv , Ning Xi , Yuan Gao , Yang Qi , Wei Li , Gang Su

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

无序系统与神经网络 · 物理学 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

We have studied spin freezing in the diluted spin ice compound Dy2-xYxTi2O7 where the non-magnetic Y ions replace the magnetic Dy ions on the frustrated pyrochlore lattice. Magnetic a.c. and d.c. susceptibility data are presented with an…

材料科学 · 物理学 2009-11-07 J. Snyder , J. S. Slusky , R. J. Cava , P. Schiffer

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

A detailed study of the structural and magnetic properties of the spin-$3/2$ hyperkagome lattice compound Li$_2$MgMn$_3$O$_8$ is reported. This material shows ferromagnetic response below $T_{\rm C} \simeq 20.6$ K, the temperature almost…

材料科学 · 物理学 2024-06-26 R. Kolay , A. Magar , A. A. Tsirlin , R. Nath

Using the experimental capability of the novel X-ray diffraction instrument available at the 25 Tesla Florida Split Coil Magnet at the NHMFL, Tallahassee we present an extensive investigation on the magnetostriction of polycrystalline…

We report the synthesis, characterization, low-temperature magnetic, and thermodynamic measurements of the novel milli-Kelvin adiabatic demagnetization refrigeration (mK-ADR) candidate material NaYbGeO$_4$ which exhibits a distorted square…

强关联电子 · 物理学 2023-12-12 U. Arjun , K. M. Ranjith , A. Jesche , F. Hirschberger , D. D. Sarma , P. Gegenwart

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

无序系统与神经网络 · 物理学 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas

We report the magnetic characterization of the frustrated transition metal pyrochlore NaCaCo$_2$F$_7$. This material has high spin Co$^{2+}$ in CoF$_6$ octahedra in a pyrochlore lattice, and disordered non-magnetic Na and Ca on the…

材料科学 · 物理学 2015-06-19 J. W. Krizan , R. J. Cava

We have synthesized the intermetallic YPrFe17 compound by arc-melting. X-ray and neutron powder diffraction show that the crystal structure is rhombohedral with View the MathML source space group (Th2Zn17-type). The investigated compound…

The Gd2Sn2O7 pyrochlore Heisenberg antiferromagnet displays a phase transition to a four sublattice Neel ordered state at a temperature near 1 K. Despite the seemingly conventional nature of the ordered state, the specific heat has been…

材料科学 · 物理学 2007-08-16 Adrian Del Maestro , Michel J. P. Gingras

A model for a Heisenberg antiferromagnet on a pyrochlore lattice with exchange and dipole-dipole interactions is studied via mean-field theory. In treating the dipoles by use of the Ewald method, a soft (critical) mode with a unique…

统计力学 · 物理学 2007-05-23 Matthew Enjalran , Michel J. P. Gingras

We report the ferroelectric property in Tb2Ti2O7 pyrochlore, prepared by a two-step solid-state reaction method. A concave P-E (polarisation vs electric field) loop observed from 382 K confirms ferroelectricity, below which the loop remains…

材料科学 · 物理学 2021-02-03 B. Santhosh Kumar , Rajesh Narayana Perumal , C. Venkateswaran

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

无序系统与神经网络 · 物理学 2009-11-07 A. L. Cornelius , J. S. Gardner

We have investigated the magnetocaloric effects in antiferromagnets and compared them with those in ferromagnets using Monte Carlo simulations. In antiferromagnets, the magnetic entropy reaches a maximum value at a finite magnetic field…

材料科学 · 物理学 2014-03-20 Ryo Tamura , Takahisa Ohno , Hideaki Kitazawa

The rich phase diagrams of magnetically frustrated pyrochlores have maintained a high level of interest over the past 20 years. To experimentally explore these phase diagrams requires a means of tuning the relevant interactions. One…

强关联电子 · 物理学 2015-03-24 A. M. Hallas , A. M. Arevalo-Lopez , A. Z. Sharma , T. Munsie , J. P. Attfield , C. R. Wiebe , G. M. Luke

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

材料科学 · 物理学 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $\rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with…

强关联电子 · 物理学 2022-08-11 A. Scheie , M. Sanders , Yiming Qiu , T. R. Prisk , R. J. Cava , C. Broholm

The electron paramagnetic resonance is used to measure the single-ion anisotropy of Gd3+ ions in the pyrochlore structure of (Y{1-x}Gdx)2Ti2O7. A rather strong easy-plane type anisotropy is found. The anisotropy constant D is comparable to…