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We have studied the neutron diffuse scattering in the relaxor PMN. The diffuse scattering appears around the Burns temperature (~620K), indicating its origin from the polar nanoregions (PNR). While the relative diffuse intensities are…

材料科学 · 物理学 2009-11-07 K. Hirota , Z. -G. Ye , S. Wakimoto , P. M. Gehring , G. Shirane

Single crystals of a ternary relaxor ferroelectric system, 0.29Pb(In1/2Nb1/2)O3-0.45Pb(Mg1/3Nb2/3)O3-0.26PbTiO3, have been studied using triple-axis based elastic and inelastic neutron scattering. Elastic diffuse scattering confirms the…

材料科学 · 物理学 2022-08-10 Qian Li , Sergey Danilkin , Guochu Deng , Jian Wang , Zhengrong Li. Ray L. Withers , Zhuo Xu , Yun Liu

We have used neutron scattering techniques to characterize the diffuse scattering and lattice dynamics in single crystals of the relaxor PMN from 10K to 900K. We observed two distinct types of diffuse scattering. The first is weak,…

材料科学 · 物理学 2009-06-11 P. M. Gehring , H. Hiraka , C. Stock , S. -H. Lee , W. Chen , Z. -G. Ye , S. B. Vakhrushev , Z. Chowdhuri

We report neutron inelastic scattering measurements of the lowest-energy transverse optic (TO) phonon branch in the relaxor Pb(Mg_1/3Nb_2/3)O_3 from 400 to 1100 K. Far above the Burns temperature T_d ~ 620 K we observe well-defined…

材料科学 · 物理学 2009-11-07 P. M. Gehring , S. Wakimoto , Z. -G. Ye , G. Shirane

Diffuse neutron scattering is a valuable tool to obtain information about the size and orientation of the polar nanoregions that are a characteristic feature of relaxor ferroelectrics. In this paper, we present new diffuse scattering…

材料科学 · 物理学 2009-11-07 D. La-Orauttapong , J. Toulouse , Z. -G. Ye , R. Erwin , J. L. Robertson , W. Chen

Neutron elastic diffuse scattering experiments performed on Pb(Zn1/3Nb2/3)O3 (PZN) and on its solid solution with PbTiO3(PT), known as PZN-xPT, with x=4.5% and 9% around many reflections show that diffuse scattering is observed around…

材料科学 · 物理学 2009-11-07 D. La-Orauttapong , J. Toulouse , Z. -G. Ye , W. Chen , R. Erwin , J. L. Robertson

The low-energy part of the vibration spectrum in PbMg$_{1/3}$Nb$_{2/3}$O$_3$ (PMN) relaxor ferroelectric has been studied by neutron scattering above and below the Burns temperature, T$_d$. The transverse acoustic and the lowest transverse…

材料科学 · 物理学 2007-05-23 S N Gvasaliya , B Roessli , R A Cowley , P Hubert , S G Lushnikov

The complex interaction between transverse acoustic (TA) phonon, transverse optic (TO) phonon and polar nano-domains (PND) in the relaxor ferroelectric KTa1-xNbxO3 (KTN) is studied by means of high resolution diffuse and inelastic neutron…

介观与纳米尺度物理 · 物理学 2016-09-08 J. Toulouse , E. Iolin , B. Hennion , D. Petitgrand , G. Yong , R. Erwin

We report neutron inelastic scattering experiments on single crystal PbMg$_{1/3}$Nb$_{2/3}$O$_{3}$ doped with 32\% PbTiO$_{3}$, a relaxor ferroelectric that lies close to the morphotropic phase boundary. When cooled under an electric field…

材料科学 · 物理学 2016-01-06 John A. Schneeloch , Zhijun Xu , B. Winn , C. Stock , P. M. Gehring , R. J. Birgeneau , Guangyong Xu

We use neutron scattering to characterize the acoustic phonons in the relaxor PMN and demonstrate the presence of an anisotropic damping mechanism directly related to short-range, polar correlations. For a large range of temperatures above…

材料科学 · 物理学 2015-06-11 C. Stock , P. M. Gehring , H. Hiraka , I. Swainson , G. Xu , Z. -G. Ye , H. Luo , J. -F. Li , D. Viehland

We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with…

材料科学 · 物理学 2009-11-10 Guangyong Xu , G. Shirane , J. R. D. Copley , P. M. Gehring

Soft phonons and diffuse scattering in insulating La$_{2-x}$Sr$_{x}$CuO$_4$ ($x=0.05$) have been studied by the neutron scattering technique. The X-point phonon softens from high temperature towards the structural transition temperature…

超导电性 · 物理学 2009-11-10 Shuichi Wakimoto , Seunghun Lee , Peter M. Gehring , Robert J. Birgeneau , Gen Shirane

We report measurements of the neutron diffuse scattering in a single crystal of the relaxor ferroelectric material 95.5%Pb(Zn$_{1/3}$Nb$_{2/3}$)O$_3$-4.5%PbTiO$_3$ (PZN-4.5%PT). Our results suggest that the nanometer scale structure in this…

材料科学 · 物理学 2010-11-10 Zhijun Xu , Jinsheng Wen , Guangyong Xu , C. Stock , J. S. Gardner , P. M. Gehring

We have characterized the dynamics of the polar nanoregions in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) through high-resolution neutron backscattering and spin-echo measurements of the diffuse scattering cross section. We find that the diffuse…

The damping ($\Gamma_a$) of the transverse acoustic (TA) phonon in single crystals of the relaxor $KTa_{1-x}Nb_xO_3$ with x=0.15-0.17 was studied by means of high resolution inelastic cold neutron scattering near the (200) B.Z. point where…

材料科学 · 物理学 2017-01-04 J. Toulouse , E. Iolin , B. Hennion , D. Petitgrand , R. Erwin

The intrinsic linewidth $\Gamma_{TA}$ of the transverse acoustic (TA) phonon observed in the relaxor ferroelectric compound Pb(Mg$_{1/3}$Nb$_{2/3})_{0.8}$Ti$_{0.2}$O$_3$ (PMN-20%PT) begins to broaden with decreasing temperature around 650…

材料科学 · 物理学 2009-11-07 T. -Y. Koo , P. M. Gehring , G. Shirane , V. Kiryukhin , G. Lee , S. -W. Cheong

We report measurements of the neutron diffuse scattering in a single crystal of the relaxor ferroelectric material 95.5%Pb(Zn1/3Nb2/3)O3-4.5%PbTiO3 (PZN-4.5%PT). We show that the diffuse scattering at high temperatures has a quasielastic…

材料科学 · 物理学 2013-01-10 Zhijun Xu , Jinsheng Wen , E. Mamontov , C. Stock , P. M. Gehring , Guangyong Xu

Neutron scattering techniques have been used to study the relaxor ferroelectric 0.68PbMg1/3Nb2/3O3-0.32PbTiO3 denoted in this paper as 0.68PMN-0.32PT. On cooling, these relaxor ferroelectrics have a long-range ordered ferroelectric phase…

材料科学 · 物理学 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. Kojima , S. G. Lushnikov

The relaxor ferroelectric PbMg1/Nb2/3O3 was investigated by means of broad-band dielectric and Fourier Transform Infrared (FTIR) transmission spectroscopy in the frequency range from 1 MHz to 15 THz at temperatures between 20 and 900 K…

材料科学 · 物理学 2009-11-10 S. Kamba , M. Kempa , V. Bovtun , J. Petzelt , K. Brinkman , N. Setter

The relaxor ferroelectric PbMg_1/3Ta_2/3O_3 was studied by single-crystal neutron and synchrotron x-ray diffraction and its detailed atomic structure has been modeled in terms of static Pb-displacements that lead to the formation of polar…

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