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Tetrahedral liquids such as water and silica-melt show unusual thermodynamic behavior such as a density maximum and an increase in specific-heat when cooled to low temperatures. There is a debate in the literature whether these phenomena…

统计力学 · 物理学 2011-08-10 Itamar Procaccia , Ido Regev

There has been long-standing debate about the physical state and possible phase transformations of confined liquids. In this report we show that a model confined liquid can behave both as a Newtonian liquid with very little change in its…

软凝聚态物质 · 物理学 2007-05-23 Shivprasad Patil , George Matei , Ahmet Oral , Peter M. Hoffmann

All phase transitions can be categorised into two different types: continuous and discontinuous phase transitions. Discontinuous phase transitions are normally accompanied with significant structural changes, and nearly all of them have the…

软凝聚态物质 · 物理学 2024-02-20 Yusheng Lei , Ran Ni

Gas hydrates are considered fundamental building blocks of giant icy planets like Neptune and similar exoplanets. The existence of these materials in the interiors of giant icy planets, which are subject to high pressures and temperatures,…

We investigate the properties of damped Ly{\alpha} absorption systems (DLAs) in semi-analytic models of galaxy formation, including partitioning of cold gas in galactic discs into atomic, molecular, and ionized phases with a molecular…

宇宙学与河外天体物理 · 物理学 2015-06-16 Michael Berry , Rachel S. Somerville , Marcel R. Haas , Eric Gawiser , Ari Maller , Gergo Popping , Scott C. Trager

This perspective article reviews arguments that glass-forming liquids are different from those of standard liquid-state theory, which typically have a viscosity in the mPa$\cdot$s range and relaxation times of order picoseconds. These…

软凝聚态物质 · 物理学 2024-02-13 Jeppe C. Dyre

We show that there can exist two liquid states in distinguishable helium-4 ($^4$He) obeying Boltzmann statistics by path integral centroid molecular dynamics (CMD) simulations. This is an indication of quantum liquid polyamorphism induced…

化学物理 · 物理学 2024-07-30 Momoko Tsujimoto , Kenichi Kinugawa

We show that the rate of separation of two phases of different densities (e.g. gas and solid) can be radically altered by the presence of a metastable intermediate phase (e.g. liquid). Within a Cahn-Hilliard theory we study the growth in…

软凝聚态物质 · 物理学 2016-08-31 R. M. L. Evans , W. C. K. Poon , M. E. Cates

In equilibrium liquid crystals, chirality leads to a variety of spectacular three-dimensional structures, but chiral and achiral phases with the same broken continuous symmetries have identical long-time, large-scale dynamics. In this…

软凝聚态物质 · 物理学 2021-06-23 S. J. Kole , Gareth P. Alexander , Sriram Ramaswamy , Ananyo Maitra

We propose and explore a new finite temperature phase of translationally invariant multi-component liquids which we call a "Quantum Disentangled Liquid" (QDL) phase. We contemplate the possibility that in fluids consisting of two (or more)…

强关联电子 · 物理学 2014-11-27 Tarun Grover , Matthew P. A. Fisher

Confinement can modify the dynamics, the thermodynamics and the structural properties of liquid water, the prototypical anomalous liquid. By considering a general anomalous liquid, suitable for globular proteins, colloids or liquid metals,…

软凝聚态物质 · 物理学 2015-06-19 Fabio Leoni , Giancarlo Franzese

Liquid $^3$He confined in low-density, highly porous random solids such as silica aerogel provides tuneable systems to study the effects of disorder and confinement on the properties of a quantum liquid. New superfluid phases result from…

超导电性 · 物理学 2018-12-13 W. P. Halperin , J. M. Parpia , J. A. Sauls

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

软凝聚态物质 · 物理学 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Experiments and computer simulations have established that liquid water's surfaces can deviate in important ways from familiar bulk behavior. Even in the simplest case of an air-water interface, distinctive layering, orientational biases,…

软凝聚态物质 · 物理学 2022-07-15 Nathan L. Odendahl , Phillip L. Geissler

Hydrogen is widely regarded as a cornerstone of future low-carbon energy technologies, yet the lack of safe, efficient, and reversible solid-state storage materials remains a major barrier to its large-scale deployment. Although porous…

Recent studies of the phase diagram for spherical, purely repulsive, active particles established the existence of a transition from a liquid-like to a solid-like phase analogous to the one observed in colloidal systems at thermal…

Damped Lyman-alpha systems (DLAs) are useful probes of star formation and galaxy formation at high redshift. We study the physical properties of DLAs and their relationship to Lyman-break galaxies using cosmological hydrodynamic simulations…

天体物理学 · 物理学 2008-11-26 Kentaro Nagamine

Beyond the snow line of protoplanetary discs and inside the dense core of molecular clouds, the temperature of gas is low enough for water vapour to condense into amorphous ices on the surface of preexisting refractory dust particles.…

The question of the local stability of the (replica-symmetric) amorphous solid state is addressed for a class of systems undergoing a continuous liquid to amorphous-solid phase transition driven by the effect of random constraints. The…

无序系统与神经网络 · 物理学 2009-10-31 Horacio E. Castillo , Paul M. Goldbart , Annette Zippelius

We examine the physical processes which are involved in the formation and stability of the anomalous states of water reported recently. The initial step of adding a small amount of ionic compound XY to pure water leads to the formation of…

化学物理 · 物理学 2007-05-23 Cheuk-Yin Wong , Shui-Yin Lo