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相关论文: Theory of Vibrationally Inelastic Electron Transpo…

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Vibrationally inelastic electron transport through a flexible molecular junction is investigated. The study is based on a mechanistic model for a biphenyl molecule between two metal electrodes. Employing methods from electron-molecule…

介观与纳米尺度物理 · 物理学 2023-07-26 Martin Cizek , Michael Thoss , Wolfgang Domcke

We theoretically analyzed inelastic effects in the electron transport through molecular junctions originating from electron-vibron interactions. The molecular bridge was simulated by a periodic chain of identical interacting hydrogen-like…

材料科学 · 物理学 2010-01-03 Natalya A. Zimbovskaya , Maija M. Kuklja

Currently, molecular tunnel junctions are recognized as important active elements of various nanodevices. This gives a strong motivation to study physical mechanisms controlling electron transport through molecules. Electron motion through…

介观与纳米尺度物理 · 物理学 2013-01-24 Natalya A. Zimbovskaya

We analyze various limits of vibrationally coupled resonant electron transport in single-molecule junctions. Based on a master equation approach, we discuss analytic and numerical results for junctions under a high bias voltage or weak…

介观与纳米尺度物理 · 物理学 2015-03-18 R. Härtle , M. Thoss

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , M. Thoss

We investigate the role of electronic-vibrational coupling in resonant electron transport through single-molecule junctions, taking into account that the corresponding coupling strengths may depend on the charge and excitation state of the…

介观与纳米尺度物理 · 物理学 2016-03-23 Andre Erpenbeck , Rainer Härtle , Michel Bockstedte , Michael Thoss

Using a model comprising a 2-level bridge connecting free electron reservoirs we show that coupling of a molecular bridge to electron-hole excitations in the leads can markedly effect the source-drain current through a molecular junction.In…

介观与纳米尺度物理 · 物理学 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

A time-dependent approach is used to explore inelastic effects during electron transport through few-level systems. We study a tight-binding chain with one and two sites connected to vibrations. This simple but transparent model gives…

介观与纳米尺度物理 · 物理学 2009-11-13 S. Monturet , N. Lorente

The thermoelectric transport through a molecular bridge is discussed, with an emphasis on the effects of inelastic processes of the transport electrons caused by the coupling to the vibrational modes of the molecule. In particular it is…

介观与纳米尺度物理 · 物理学 2015-03-17 O. Entin-Wohlman , Y. Imry , A. Aharony

We review studies of vibrational energy transfer in a molecular junction geometry, consisting of a molecule bridging two heat reservoirs, solids or large chemical compounds. This setup is of interest for applications in molecular…

介观与纳米尺度物理 · 物理学 2016-06-22 Dvira Segal , Bijay Kumar Agarwalla

The role of multimode vibrational dynamics in electron transport through single molecule junctions is investigated. The study is based on a generic model, which describes charge transport through a single molecule that is attached to metal…

介观与纳米尺度物理 · 物理学 2010-10-26 R. Härtle , C. Benesch , M. Thoss

The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

介观与纳米尺度物理 · 物理学 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

In this work we theoretically study steady state thermoelectric transport through a single-molecule junction with a long chain-like bridge. Electron transmission through the system is computed using a tight-binding model for the bridge. We…

介观与纳米尺度物理 · 物理学 2018-03-02 Natalya A. Zimbovskaya , Abraham Nitzan

We describe how to treat the interaction of travelling electrons with localised vibrational modes in nanojunctions. We present a multichannel scattering technique which can be applied to calculate the transport properties for realistic…

介观与纳米尺度物理 · 物理学 2007-05-23 H. Ness , A. J. Fisher

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

介观与纳米尺度物理 · 物理学 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

The effect of vibrational motion on resonant charge transport through single molecule junctions is investigated. The study is based on a combination of first-principles electronic structure calculations to characterize the system and…

其他凝聚态物理 · 物理学 2007-12-24 Claudia Benesch , Martin Cizek , Jiri Klimes , Michael Thoss , Wolfgang Domcke

Vibrational nonequilibrium effects in charge transport through single-molecule junctions are investigated. Focusing on molecular bridges with multiple electronic states, it is shown that electronic-vibrational coupling triggers a variety of…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , C. Benesch , M. Thoss

Experiments studying vibrational effects on electronic transport through single molecules have observed several seemingly inconsistent behaviors, ranging from up to 30 harmonics of a vibrational frequency in one experiment, to an absence of…

介观与纳米尺度物理 · 物理学 2007-05-23 Vivek Aji , J. E. Moore , C. M. Varma

The accuracy of the noninteracting electron approximation is examined for a model of vibrationally coupled electron transport in single molecule junction. In the absence of electronic-vibrational coupling, steady state transport in this…

介观与纳米尺度物理 · 物理学 2017-01-04 Haobin Wang , Michael Thoss

The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

介观与纳米尺度物理 · 物理学 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi
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