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In single-molecule transistors, we observe inelastic cotunneling features that correspond energetically to vibrational excitations of the molecule, as determined by Raman and infrared spectroscopy. This is a form of inelastic electron…

介观与纳米尺度物理 · 物理学 2007-05-23 L. H. Yu , Z. K. Keane , J. W. Ciszek , L. Cheng , M. P. Stewart , J. M. Tour , D. Natelson

We describe single electron tunneling through molecular structures under the influence of nano-mechanical excitations. We develop a full quantum mechanical model, which includes charging effects and dissipation, and apply it to the…

介观与纳米尺度物理 · 物理学 2009-10-31 Daniel Boese , Herbert Schoeller

We investigate vibron-assisted electron transport in single-molecule transistors containing an individual Fe4 Single-Molecule Magnet. We observe a strong suppression of the tunneling current at low bias in combination with vibron-assisted…

介观与纳米尺度物理 · 物理学 2016-06-09 E. Burzurí , Y. Yamamoto , M. Warnock , X. Zhong , K. Park , A. Cornia , H. S. J. van der Zant

Tunnel transport of interacting spin-polarized electrons through a single-level vibrating quantum dot in external magnetic field is studied. By using density matrix method, the current-voltage characteristics and the dependence of…

介观与纳米尺度物理 · 物理学 2021-03-23 A. D. Shkop , O. M. Bahrova , S. I. Kulinich , I. V. Krive

Transport through molecular devices with strong coupling to a single vibrational mode is considered in the case where the vibration is damped by coupling to the environment. We focus on the weak tunneling limit, for which a rate equation…

介观与纳米尺度物理 · 物理学 2007-05-23 Stephan Braig , Karsten Flensberg

Transport through molecular quantum dots coupled to a single vibration mode is studied in the case with strong coupling to the leads. We use an expansion in the correlation between electrons on the molecule and electrons in the leads and…

介观与纳米尺度物理 · 物理学 2009-11-10 Karsten Flensberg

We consider the electron-vibron coupling in suspended nanotube quantum dots. Modelling the tube as an elastic medium, we study the possible coupling mechanism for exciting the stretching mode in a single-electron-transistor setup. Both the…

介观与纳米尺度物理 · 物理学 2009-11-11 Karsten Flensberg

Single-molecule transistors provide a unique experimental tool to investigate the coupling between charge transport and the molecular degrees of freedom in individual molecules. One interesting class of molecules for such experiments are…

Effects of a coupling between the mechanical vibrations of a quantum dot placed between the two leads of a single electron transistor and coherent tunneling of electrons through a single level in the dot has been studied. We have found that…

介观与纳米尺度物理 · 物理学 2009-11-07 D. Fedorets , L. Y. Gorelik , R. I. Shekhter , M. Jonson

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

介观与纳米尺度物理 · 物理学 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin

The detection of vibrational excitations of individual molecules on surfaces by scanning tunneling spectroscopy does not obey strict selection rules but rather propensity rules. The experimental verification of these is challenging because…

We investigate transport through a mononuclear transition-metal complex with strong tunnel coupling to two electrodes. The ground state of this molecule is a singlet while the first excited state is a triplet. We show that a modulation of…

强关联电子 · 物理学 2007-05-23 K. Kikoin , M. N. Kiselev , M. R. Wegewijs

We present a microscopic study of single-electron tunneling in nanomechanical double-barrier tunneling junctions formed using a vibrating scanning nanoprobe and a metallic nanoparticle connected to a metallic substrate through a molecular…

介观与纳米尺度物理 · 物理学 2009-11-10 Yongqiang Xue , Mark A. Ratner

We present an experimental and theoretical study of a magnetic single-molecule transistor based on N@C60 connected to gold electrodes. Particular attention is paid to the regime of intermediate molecule-lead coupling, where cotunneling…

介观与纳米尺度物理 · 物理学 2015-05-27 Nicolas Roch , Romain Vincent , Florian Elste , Wolfgang Harneit , Wolfgang Wernsdorfer , Carsten Timm , Franck Balestro

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

介观与纳米尺度物理 · 物理学 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

We present a theory of single-electron tunneling transport through a ferromagnetic nanoparticle in which particle-hole excitations are coupled to spin collective modes. The model employed to describe the interaction between quasiparticles…

介观与纳米尺度物理 · 物理学 2009-11-11 L. Michalak , C. M. Canali , V. G. Benza

We theoretically examine the effect of the coupling of the transport electrons to a vibrational mode of the molecule on the ac linear-response conductance of molecular junctions. Representing the molecule by a single electronic state, we…

介观与纳米尺度物理 · 物理学 2015-05-27 A. Ueda , O. Entin-Wohlman , A. Aharony

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

介观与纳米尺度物理 · 物理学 2009-12-21 J. Mravlje , A. Ramsak

Graphene electrodes are promising candidates to improve reproducibility and stability in molecular electronics through new electrode-molecule anchoring strategies. Here we report sequential electron transport in few-layer graphene…

Understanding the influence of vibrational motion of the atoms on electronic transitions in molecules constitutes a cornerstone of quantum physics, as epitomized by the Franck-Condon principle of spectroscopy. Recent advances in building…

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