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We propose an explanation of the mid-infrared peak observed in the optical conductivity of the Bechgaard salt (TMTSF)$_2$PF$_6$ in terms of electronic excitations. It is based on a numerical calculation of the conductivity of the…

凝聚态物理 · 物理学 2009-10-28 Julien Favand , Frédéric Mila

The infrared response of the organic conductor (TMTSF)$_2$PF$_6$ and the Mott insulator (TMTTF)$_2$PF$_6$ are investigated as a function of temperature and pressure and for the polarization parallel and perpendicular to the molecular…

强关联电子 · 物理学 2015-05-14 A. Pashkin , M. Dressel , M. Hanfland , C. A. Kuntscher

We have measured the electrodynamic response in the metallic state of three highly anisotropic conductors, (TMTSF)_2 X, where X=PF_6, AsF_6, or ClO_4, and TMTSF is the organic molecule tetramethyltetraselenofulvalene. In all three cases we…

强关联电子 · 物理学 2009-10-31 A. Schwartz , M. Dressel , G. Gruner , V. Vescoli , L. Degiorgi , T. Giamarchi

The organic salt $\alpha$-(BEDT-TTF)$_2$I$_3$ is considered a model system for metal-insulator transition due to electronic charge ordering at $T_{\rm CO}=135$~K. The optical properties obtained from polarized reflection measurements above…

强关联电子 · 物理学 2016-03-25 T. Peterseim , M. Dressel

We studied the pressure dependence of the room-temperature infrared reflectivity of (TMTTF)_2AsF_6 along all three optical axes. This anisotropic organic compound consists of molecular stacks with orbital overlap along the a direction; due…

强关联电子 · 物理学 2007-05-23 A. Pashkin , M. Dressel , C. A. Kuntscher

The polarized optical reflectance spectra of the quasi two dimensional organic correlated electron system $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]$Y$, $Y =$ Br and Cl are measured in the infrared region. The former shows the…

超导电性 · 物理学 2007-05-23 T. Sasaki , I. Ito , N. Yoneyama , N. Kobayashi , N. Hanasaki , H. Tajima , T. Ito , Y. Iwasa

We present a group theoretical analysis of the superconducting state of the Bechgaard salts, e.g., (TMTSF)_2PF_6 or (TMTSF)_2ClO_6. We show that there are eight symmetry distinct superconducting states. Of these only the (fully gapped, even…

超导电性 · 物理学 2008-08-08 B. J. Powell

The electric conductivity which reveals the zero gap semiconducting (ZGS) state has been investigated as the function of temperature $T$ and life time $\tau$ in order to understand the ZGS state in quarter-filled…

材料科学 · 物理学 2009-11-11 Shinya Katayama , Akito Kobayashi , Yoshikazu Suzumura

We present a combined experimental and theoretical study on the quasi-one-dimensional organic conductor (TMTTF)$_2$PF$_6$, and elucidate the variation of its physical properties under pressure. We fully resolve the crystal structure by…

Numerical calculations of the kinetic energy of various extensions of the one-dimensional Hubbard model including dimerization and repulsion between nearest neighbours are reported. Using the sum rule that relates the kinetic energy to the…

凝聚态物理 · 物理学 2016-08-31 Frederic Mila

Optical reflection measurements within the highly conducting (a,b)-plane of the organic metal (BEDT-TTF)_4[Ni(dto)_2] reveal the gradual development of a sharp feature at around 200 cm as the temperature is reduced below 150 K. Below this…

凝聚态物理 · 物理学 2009-10-31 P. Haas , E. Griesshaber , B. Gorshunov , D. Schweitzer , M. Dressel , F. F. Assaad

We propose a quantitative estimate of the charge gap that opens in the one-dimensional dimerized Hubbard model at quarter-filling due to dimerization, which makes the system effectively half--filled, and to repulsion, which induces umklapp…

凝聚态物理 · 物理学 2009-02-27 K. Penc , F. Mila

We consider the optical conductivity $\sigma_1(\omega)$ in the metallic phase of the one-dimensional Hubbard model. Our results focus on the vicinity of half filling and the frequency regime around the optical gap in the Mott insulating…

We report a novel insulator-insulator transition arising from the internal charge degrees of freedom in the two-dimensional quarter-filled organic salt beta-(meso-DMBEDT-TTF)2PF6. The optical conductivity spectra above Tc = 70 K display a…

Conductivity and permittivity of the quasi-one-dimensionsional organic transfer salt (TMTTF)2PF6 have been measured at low frequencies (10^3-10^7 Hz) between room temperature down to below the temperature of transition into the spin-Peierls…

强关联电子 · 物理学 2009-10-31 F. Nad , P. Monceau , C. Carcel , J. M. Fabre

An exhaustive investigation of metallic electronic transport and superconductivity of organic superconductors (TMTSF)_2PF_6 and (TMTSF)_2ClO_4 in the Pressure-Temperature phase diagram between T=0 and 20 K and a theoretical description…

We investigated the electronic states of the quasi-one-dimensional organic conductors $\delta'_{P}$-(BPDT-TTF)$_2$ICl$_2$ and $\delta'_{C}$-(BPDT-TTF)$_2$ICl$_2$, both of which are insulating at room temperature owing to strong electron…

The low--energy excited states of a system of interacting one--dimensional fermions in a conducting state are collective charge and spin density oscillations. The unusual physical properties of such a system (called ``Luttinger liquid'')…

凝聚态物理 · 物理学 2007-05-23 H. J. Schulz

The quasi-1D organic Bechgaard salt (TMTSF)$_2$PF$_6$ displays spin-density-wave (SDW) order and superconductivity in close proximity in the temperature-pressure phase diagram. We have measured its normal-state electrical resistivity…

The infrared spectra of the quasi-two-dimensional organic conductors $\alpha$-(BEDT-TTF)$_2$$M$Hg(SCN)$_4$ ($M$ = NH$_4$, Rb, Tl) were measured in the range from 50 to 7000 \cm down to low temperatures in order to explore the influence of…

强关联电子 · 物理学 2015-06-25 N. Drichko , M. Dressel , C. A. Kuntscher , A. Pashkin , A. Greco , J. Merino , J. Schlueter
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