相关论文: Quadrupolar interactions in Pr compounds: PrFe4P12…
We describe the experimentally revealed by Sichelschmidt et al, Phys. Rev. Lett. 91 (2003) 156401, g tensor, g_perpendicular=3.561 and g_parallel=0.17, at 5 K by means of crystal field interactions of the 4f13 configuration of the Yb3+ ion…
The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…
Neutron diffraction measurements have been performed on the cubic compound PrPb3 in a [001] magnetic field to examine the quadrupolar ordering. Antiferromagnetic components with q=(1/2+-d 1/2 0), (1/2 1/2+-d 0) (d~1/8) are observed below…
Origin of the non-magnetic phase transition in PrTi$_2$Al$_{20}$, reported earlier in the macroscopic study, has been asserted microscopically using elastic and inelastic neutron scattering techniques. It has been shown spectroscopically…
Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior.…
In the external field slightly inclined to the $x$- or y-axis of the frustrated tetragonal atiferromagnet Pr2CuO4, a transition is discovered from the phase with orthogonal antiferromagnetic spin subsystems along [1,0,0] and [0,1,0] to the…
As a possible mechanism of the $\gamma-\alpha$ phase transition in pristine cerium a change of the electronic density from a disordered state with symmetry Fm-3m to an ordered state Pa-3 has been proposed. Here we include on-site and inter-…
A model for crystal field triplet ground states on rare earth or actinide ions with dipolar and quadrupolar couplings to conduction electrons is studied for the first time with renormalization group methods. The quadrupolar coupling leads…
We discuss the triple-$\vec{q}^X$ structures for the ordered cubic phase of NpO$_2$, which are $Pn{\bar 3}m$ and $Pa{\bar 3}$. A special care should be taken to discriminate between these two cases. We analyze the relevant structure-factor…
Characteristics of hybridization and multipole orders of $4f$-electrons in Pr skutterudites are explained in terms of a pseudo-quartet composed of crystalline electric field (CEF) singlet and the triplet. It is shown that the contrasting…
We propose novel triple-${\bm q}$ multipole orders as possible candidates for the two distinct low-temperature symmetry broken phases in quadrupolar system PrV$_2$Al$_{20}$. An analysis of the experiment under [111] magnetic fields…
A microscopic model is proposed for the scalar order in PrFe4P12 where f2 crystalline electric field (CEF) singlet and triplet states interact with two conduction bands. By combining the dynamical mean-field theory and the continuous-time…
Neutron scattering experiments have revealed a field-induced antiferroquadrupolar order parameter in the Pr-based heavy-fermion superconductor PrOs$_4$Sb$_{12}$. We observed the field-induced antiferromagnetic dipole moment with the…
Our single crystal study reveals that PrTr2Al20 (Tr = Ti and V) provides the first examples of a cubic {\Gamma}3 nonmagnetic ground doublet system that shows the Kondo effect including a -ln T dependent resistivity. The {\Gamma}3…
The recent experimental finding of large-amplitude antiferromagnetism induced by uniaxial strain shows that the "hidden" low-field order of URu2Si2 breaks time reversal invariance. We propose a new crystal field model which supports…
Double perovskites containing heavy transition metal ions are an important family of compounds for the study of the interplay between electron correlation and spin-orbit coupling. Here, by combining magnetic susceptibility, heat capacity,…
We have studied the low-temperature properties of Pr$_{x}$La$_{1-x}$Pb$_{3}$ with non-Kramers $\Gamma_{3}$ quadrupolar moments of the crystal-electric-field ground state, for a wide concentration range of Pr ions. For $x$$\le$0.05, the…
We report the results of 27Al-NMR measurements on a single crystal of PrTi2Al20. This compound shows a phase transition near 2 K associated with the quadrupole degree of freedom of Pr ions, for which the ground state of the crystalline…
Theoretical account is given of 4f-electron dynamics and multipole orders in Pr skutterudites with particular attention to (i) mechanism of the crystalline electric field (CEF) splitting leading to a pseudo-quartet ground state;(ii) Kondo…
We present neutron diffraction, magnetic susceptibility and specific heat data for a single-crystal sample of the cubic (Cu3Au structure) compound Pr3In. This compound is believed to have a singlet (Gamma1) groundstate and a low-lying…