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The effect of laser fields on the electron transport through a molecular wire being weakly coupled to two leads is investigated. The molecular wire acts as a coherent quantum ratchet if the molecule is composed of periodically arranged,…

介观与纳米尺度物理 · 物理学 2009-11-07 Jörg Lehmann , Sigmund Kohler , Peter Hänggi , Abraham Nitzan

The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…

量子物理 · 物理学 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

介观与纳米尺度物理 · 物理学 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi

We investigate the possibility of optical current control through single molecules which are weakly coupled to leads. A master equation approach for the transport through a molecule is combined with a Floquet theory for the time-dependent…

化学物理 · 物理学 2016-09-08 Jörg Lehmann , Sébastien Camalet , Sigmund Kohler , Peter Hänggi

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

无序系统与神经网络 · 物理学 2009-11-11 Florian Pump , Gianaurelio Cuniberti

New features of molecular wires can be observed when they are irradiated by laser fields. These effects can be achieved by periodically oscillating fields but also by short laser pulses. The theoretical foundation used for these…

介观与纳米尺度物理 · 物理学 2007-05-23 Sven Welack , Michael Schreiber , Ulrich Kleinekathoefer

The electron tunneling through a molecular junction modeled by a single site weakly coupled to two leads is studied in the presence of a time-dependent external field using a master equation approach. In the case of small bias voltages and…

介观与纳米尺度物理 · 物理学 2009-11-13 Guangqi Li , Michael Schreiber , Ulrich Kleinekathoefer

We investigate the influence of external laser excitations on the average current through bridged molecules. For the computation of the current, we use a numerically very efficient formalism that is based on the Floquet solutions of the…

化学物理 · 物理学 2007-05-23 Sigmund Kohler , Jörg Lehmann , Sébastien Camalet , Peter Hänggi

A molecular wire coupled to two electron reservoirs is investigated within a tight-binding approach including spin and Coulomb interaction. Under the assumption of weak coupling to the electron reservoirs a quantum master equation can be…

介观与纳米尺度物理 · 物理学 2007-08-28 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

The influence of Gaussian laser pulses on the transport through molecular wires is investigated within a tight-binding model for spinless electrons including correlation. Motivated by the phenomenon of coherent destruction of tunneling for…

介观与纳米尺度物理 · 物理学 2009-11-13 Ulrich Kleinekathoefer , GuangQi Li , Sven Welack , Michael Schreiber

We investigate transport through molecular wires whose energy levels are affected by environmental fluctuations. We assume that the relevant fluctuations are so slow that they, within a tight-binding description, can be described by…

介观与纳米尺度物理 · 物理学 2008-07-09 Franz J. Kaiser , Peter Hänggi , Sigmund Kohler

We introduce a theoretical approach based on scattering theory and total energy methods that treats transport non-linearities, conformational changes and charging effects in molecular wires in a unified way. We apply this approach to…

介观与纳米尺度物理 · 物理学 2009-11-07 Eldon Emberly , George Kirczenow

We consider several fundamental optical phenomena involving single molecules in biased metal-molecule-metal junctions. The molecule is represented by its highest occupied and lowest unoccupied molecular orbitals, and the analysis involves…

介观与纳米尺度物理 · 物理学 2007-05-23 Michael Galperin , Abraham Nitzan

Electrophoresis is a motion of charged dispersed particles relative to a fluid in a uniform electric field. The effect is widely used to separate macromolecules, to assemble colloidal structures, to transport particles in nano- and…

软凝聚态物质 · 物理学 2011-01-21 Oleg D. Lavrentovich , Israel Lazo , Oleg P. Pishnyak

We present a simple model of electrical transport through a metal-molecule-metal nanojunction that includes charging effects as well as aspects of the electronic structure of the molecule. The interplay of a large charging energy and an…

介观与纳米尺度物理 · 物理学 2007-05-23 Matthias H. Hettler , Herbert Schoeller , Wolfgang Wenzel

We explore heat transfer in molecular junctions between two leads in the absence of a finite net thermal bias. The application of an unbiased, time-periodic temperature modulation of the leads entails a dynamical breaking of reflection…

介观与纳米尺度物理 · 物理学 2009-12-18 Fei Zhan , Nianbei Li , Sigmund Kohler , Peter Hänggi

We develop a new general formulation to explore light-driven electron transport through a single-molecule device with multiple pathways. Three individual systems are proposed including (i) a two-terminal molecular junction based on…

介观与纳米尺度物理 · 物理学 2014-01-20 Liang-Yan Hsu , Herschel Rabitz

We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected…

量子物理 · 物理学 2009-11-13 Vyacheslav Shatokhin , Cord A. Müller , Andreas Buchleitner

The alternative to dynamic alignment explanation of experimental results on spatial-asymmetric dissociation of molecules in a laser field is proposed. The concept of geometrical alignment is sufficient for explanation of these results. In…

光学 · 物理学 2007-05-23 V. A. Kuz'menko

Charge transport through a rectangular vector potential barrier modulated by a continuum laser in monolayer phosphorene is studied theoretically in the ballistic regime along the line of Floquet formalism. Laser free transmission profile…

介观与纳米尺度物理 · 物理学 2019-06-12 R. Biswas , R. Dey , C. Sinha
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