相关论文: Spin dynamics and coherent tunnelling in the molec…
Quantum tunneling of nano-magnets finds a natural description in terms of intermediate spin. Periodic magnetic effects correspond to a change of flux by the flux quantum $\Phi_{0}$. Schr\"odinger cat states with different superpositions of…
A new approach is used that allows to describe the magnetic molecules main properties in a direct and simple way. Results obtained for the Fe8 cluster show good agreement with the experimental data.
Motivated by the intriguing properties of magnetic molecular wheels at field induced level crossings, we investigate the spin-Peierls instability of antiferromagnetic rings in a field by exact diagonalizations of a microscopic spin model…
We consider here the problem of a "central spin", with spin quantum number $S \gg 1$, interacting with a set of microscopic spins. Interactions between the microscopic spins are ignored. This model describes magnetic grains or magnetic…
The theory for the quantum tunneling of nano-magnets is developed within the intermediate spin framework. Periodic magnetic effects are seen to reflect that associated with a change of flux by a single flux quantum $\Phi_{0}$. Essential are…
Spin dynamics of nanomolecules and nanoclusters are analyzed. The nanosizes of these objects make it possible to consider them as single-domain magnets with a large total spin, where the motion of the spins of all atoms, composing a…
Molecular nanomagnets, besides promising to open new frontiers in technology, have attracted huge interest in the scientific community because they can exhibit the phenomenon known as quantum tunnelling of the magnetization, i.e. coherent…
We study the spin correlations of a few fermions in a quasi one-dimensional trap. Exact diagonalization calculations demonstrate that repulsive interactions between the two species drives ferromagnetic correlations. The ejection probability…
A new mechanism is proposed for the magnetization reversal of molecular nanomagnets such as \Fe8. In this process the spin tunnels from the lowest state near one easy direction to the first excited state near the opposite easy direction,…
The magnetic torque of the antiferromagnetic molecular wheel CsFe8 was studied down to 50 mK and in fields up to 28 T. Below ca. 0.5 K phase transitions were observed at the field-induced level-crossings (LCs). Intermolecular magnetic…
Antiferromagnetic spin rings represent prototypical realizations of highly correlated, low-dimensional systems. Here we theoretically show how the introduction of magnetic defects by controlled chemical substitutions results in a strong…
Magnetoelectric coupling in helical multiferroics allows to steer spin order with electric fields. Here we show theoretically that in a helical multiferroic chain quantum information processing as well as quantum phases are highly sensitive…
High-frequency ($f$ = 190 GHz) electron paramagnetic resonance (EPR) at magnetic fields up to 12 T as well as Q-band ($f$ = 34.1 GHz) EPR were performed on single crystals of the molecular wheel CsFe$_8$. In this molecule, eight Fe(III)…
Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the…
Hybrid elastic and spin waves hold promises for energy-efficient and versatile generation and detection of magnetic signals, with potentially long coherence times. Here we report on the combined elastic and magnetic dynamics in a…
The Landau Zener model has recently been used to measure very small tunnel splittings in molecular clusters of Fe8, which at low temperature behaves like a nanomagnet with a spin ground state of S = 10. The observed oscillations of the…
Coherent control of individual molecular spins in nano-devices is a pivotal prerequisite for fulfilling the potential promised by molecular spintronics. By applying electric field pulses during time-resolved electron spin resonance…
Single molecule magnets straddle the classical and quantum mechanical worlds, displaying many fascinating phenomena. They may have important technological applications in information storage and quantum computation. We review the physical…
The Landau Zener method allows to measure very small tunnel splittings \Delta in molecular clusters Fe_8. The observed oscillations of \Delta as a function of the magnetic field applied along the hard anisotropy axis are explained in terms…
Controlling quantum spins using electric rather than magnetic fields promises significant architectural advantages for developing quantum technologies. In this context, spins in molecular nanomagnets offer tunability of spin-electric…