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A consistent theory of electron energy-loss spectroscopy (EELS) includes two indispensable elements: (i) electronic response of the target system and (ii) quantum kinematics of probing electrons. While for the bulk materials and their…

介观与纳米尺度物理 · 物理学 2017-12-12 Vladimir U. Nazarov , Vyacheslav M. Silkin , Eugene E. Krasovskii

We have developed a spin-resolved resonant electron energy-loss spectroscopy (SR-rEELS) in the primary energy of 0.3--1.5 keV, which corresponds to the core excitations of $2p$-$3d$ absorption of transition metals and $3d$-$4f$ absorption…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

化学物理 · 物理学 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

We study the electron-energy loss spectra of strongly correlated electronic systems doped away from half-filling using dynamical mean-field theory ($d=\infty$). The formalism can be used to study the loss spectra in the optical (${\bf…

强关联电子 · 物理学 2009-10-31 Luis Craco , Mukul S. Laad

Using high-resolution angle-resolved photoemission, we observe a strong spin-dependent renormalization and lifetime broadening of the quasiparticle excitations in the electronic band structure of Ni(111) in an energy window of $\sim$0.3 eV…

强关联电子 · 物理学 2019-01-02 J. Sánchez-Barriga , R. Ovsyannikov , J. Fink

A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

原子物理 · 物理学 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Spin-conserving and spin-flip opaque reflections of electrons from a potential barrier in heterostructures are described. An electric field of the barrier is considered to be the only source of energy spin splitting in the presence of…

介观与纳米尺度物理 · 物理学 2023-07-19 Pawel Pfeffer , Wlodek Zawadzki

Inelastic scattering of electrons incident on a solid surface is determined by the two properties: (i) electronic response of the target system and (ii) the detailed quantum-mechanical motion of the projectile electron inside and in the…

材料科学 · 物理学 2016-01-06 V. U. Nazarov , V. M. Silkin , E. E. Krasovskii

The scattering theory of low-energy (slow) electrons has been developed by Evans and Mills [Phys. Rev. B 5, 4126 (1972)]. The formalism is merely based on the electrostatic Coulomb interaction of the scattering electrons with the…

强关联电子 · 物理学 2023-05-25 Khalil Zakeri , Christophe Berthod

Fast electrons spectromicroscopies enable to measure quantitatively the optical response of excitations with unrivaled spatial resolution. However, due to their inherently scalar nature, electron waves cannot access to polarization-related…

光学 · 物理学 2021-05-26 Hugo Lourenço-Martins , Davy Gérard , Mathieu Kociak

In the band theory of ferromagnetism there is a relative shift in the position of majority and minority spin bands due to the self-consistent field due to opposite spin electrons. In the simplest realization, the Stoner model, the majority…

强关联电子 · 物理学 2009-10-31 J. E. Hirsch

Probing optical excitations with high resolution is important for understanding their dynamics and controlling their interaction with other photonic elements. This can be done using state-of-the-art electron microscopes, which provide the…

材料科学 · 物理学 2021-10-13 Renwen Yu , Andrea Konečná , F. Javier García de Abajo

Recent experimental progress in creating and controlling singular electron beams that carry orbital angular momentum allows for new types of local spectroscopies. We theoretically investigate the twisted-electron energy loss spectroscopy…

介观与纳米尺度物理 · 物理学 2016-12-21 M. Schüler , J. Berakdar

Electron energy loss spectroscopy (EELS) has been established as a powerful analytical technique for investigating the oxidation state, band structure, and dielectric properties of materials with exceptional spatial resolution. Inspired by…

In this work we present a theoretical study of EELS (electron-energy-loss spectroscopy) experiments on the ${\rm C}_{60}$ molecule. Our treatment of the problem is based on the simple two-fluid model originally proposed for the description…

介观与纳米尺度物理 · 物理学 2009-10-31 D. A. Gorokhov , R. A. Suris , V. V. Cheianov

We propose a setup enabling electron energy loss spectroscopy to determine the density of the electrons accumulated by an electro-positive dielectric in contact with a plasma. It is based on a two-layer structure inserted into a recess of…

应用物理 · 物理学 2020-01-08 E. Thiessen , F. X. Bronold , H. Fehske

We perform a magneto-optical study of a two-dimensional electron systems (2DES) in the regime of the Stoner ferromagnetic instability for even quantum Hall filling factors on Mg$_x$Zn$_{1-x}$O/ZnO heterostructures. Under conditions of…

介观与纳米尺度物理 · 物理学 2017-12-06 A. B. Van'kov , B. D. Kaysin , I. V. Kukushkin

Van der Waals (vdW) materials exhibit intriguing structural, electronic and photonic properties. Electron Energy Loss Spectroscopy (EELS) within Scanning Transmission Electron Microscope (STEM) allows for nanoscale mapping of such…

A periodic arrangement of 2D conducting planes is known to host a (bulk) plasmon dispersion that interpolates between the typical, gapped behavior of 3D metals and a gapless, acoustic regime as a function of the out-of-plane wavevector. The…

强关联电子 · 物理学 2022-11-09 Christian Boyd , Luke Yeo , Philip W. Phillips

Over the last two decades, Electron Energy Loss Spectroscopy (EELS) imaging with a scanning transmission electron microscope (STEM) has emerged as a technique of choice for visualizing complex chemical, electronic, plasmonic, and phononic…

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