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Time-resolved multi-terahertz (THz) spectroscopy is used to observe an ultrafast, non-thermal electronic phase change in SnSe driven by interband photoexcitation with 1.55 eV pump photons. The transient THz photoconductivity spectrum is…

Ultrafast optical excitations trigger in materials a range of dynamics. An interesting range of dynamics is the ones that unfold within the picosecond timescale, corresponding to the THz frequency range. Within this short timescale, the…

光学 · 物理学 2023-09-27 Yingshu Yang , Stefano Dal Forno , Marco Battiato

Spintronic terahertz (THz) emitter provides the advantages such as apparently broader spectrum, significantly lower cost, and more flexibility in compared with the commercial THz emitters, and thus attracts great interests recently. In past…

介观与纳米尺度物理 · 物理学 2018-11-13 Zheng Feng , Rui Yu , Yu Zhou , Hai Lu , Wei Tan , Hu Deng , Quancheng Liu , Zhaohui Zhai , Liguo Zhu , Jianwang Cai , Bingfeng Miao , Haifeng Ding

Pumping n-type GaAs and InSb with ultrafast THz pulses having intensities higher than 150 MW/cm2 shows strong free carrier absorption saturation at temperatures of 300 K and 200 K respectively. If the energy imparted to the carriers exceeds…

材料科学 · 物理学 2009-06-17 Matthias C. Hoffmann , Janos Hebling , Harold Y. Hwang , Ka-Lo Yeh , Keith A. Nelson

A model for THz generation by optical rectification using tilted-pulse-fronts is developed. It simultaneously accounts for (i) the spatio-temporal distortions of the optical pump pulse, (ii) the nonlinear coupled interaction of THz and…

Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…

Terahertz (THz) radiation is a powerful probe of low-energy excitations in all phases of matter. However, it remains a challenge to find materials that efficiently generate THz radiation in a broad range of frequencies following optical…

Time-resolved multi-terahertz (THz) spectroscopy is used to observe pump fluence-dependent dynamics in the optical conductivity of photoexcited tin selenide (SnSe) over an ultrabroadband spectral range of 0.5 - 11 THz at fluences from 0.1 -…

We systematically study the pump-wavelength dependence of terahertz pulse generation in thin-film spintronic THz emitters composed of a ferromagnetic Fe layer between adjacent nonmagnetic W and Pt layers. We find that the efficiency of THz…

Mixing the fundamental ($\omega$) and the second harmonic (2$\omega$) waves in gas phase is a widely employed technique for emitting terahertz (THz) pulses. The THz generation driven by bi-chromatic fields can be described by the…

We propose an experimental technique to generate large amplitude coherent phonons with irradiation of THz-rate pump pulses and to study the dynamics of phase transition in GeTe ferroelectrics. When a single pump pulse irradiates the sample…

材料科学 · 物理学 2011-02-01 Muneaki Hase , Masahiro Kitajima , Shin-ichi Nakashima , Kohji Mizoguchi

Recent studies in spintronics have highlighted ultrathin magnetic metallic multilayers as a novel and very promising class of broadband terahertz radiation sources. Such spintronic multilayers consist of ferromagnetic (FM) and non-magnetic…

The relaxation dynamics of photoexcited quasiparticles of three-dimensional (3D) Dirac semimetals are vital towards their application in high performance electronic and optoelectronic devices. In this work, the relaxation dynamics of…

光学 · 物理学 2018-10-03 Wei Lu , Jiwei Ling , Faxian Xiu , Dong Sun

In stimulated Raman scattering, two incident optical waves induce a force oscillating at the difference of the two light frequencies. This process has enabled important applications such as the excitation and coherent control of phonons and…

材料科学 · 物理学 2017-09-27 Sebastian Maehrlein , Alexander Paarmann , Martin Wolf , Tobias Kampfrath

Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared…

仪器与探测器 · 物理学 2017-10-10 S. J. Zhang , Z. X. Wang , T. Dong , N. L. Wang

We characterize the terahertz (THz) generation of N-benzyl-2-methyl-4-nitroaniline (BNA), with crystals ranging in thickness from 123-700 {\mu}m. We compare excitation using 800-nm and 1250 to 1500-nm wavelengths. Pumping BNA with 800-nm…

The organic terahertz (THz) generation crystal BNA has recently gained traction as a valuable source to produce broadband THz pulses. Even when pumped with 800-nm light, thin BNA crystals can produce relatively high electric fields with…

Time-dependent femtosecond pump-probe spectroscopic ellipsometry studies on zincblende gallium-nitride (zb-GaN) are performed and analyzed between 2.9-3.7eV. An ultra-fast change of the absorption onset (3.23eV for zb-GaN) is observed by…

Phase-locked ultrashort pulses in the rich terahertz (THz) spectral range have provided key insights into phenomena as diverse as quantum confinement, first-order phase transitions, high-temperature superconductivity, and carrier transport…

介观与纳米尺度物理 · 物理学 2016-04-18 M. Eisele , T. L. Cocker , M. A. Huber , M. Plankl , L. Viti , D. Ercolani , L. Sorba , M. S. Vitiello , R. Huber

This study shows that a terahertz (THz) wave can be generated from the (001) surface of cleaved Bi$_{\textrm{2}}$Se$_{\textrm{3}}$ and Cu-doped Bi$_{\textrm{2}}$Se$_{\textrm{3}}$ single crystals using 800 nm femtosecond pulses. The…

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