相关论文: Direct three body dynamics govern ion atom recombi…
Three-body recombination, or ternary association, is a termolecular reaction in which three particles collide, forming a bound state between two, whereas the third escapes freely. Three-body recombination reactions play a significant role…
The recombination of halogen atoms has been a research topic in chemical physics for over a century. All theoretical descriptions of atom recombination depend on a two-step assumption, where two colliding atoms first form an unstable…
A very recently method for classical trajectory calculations for three-body collision [J. P\'{e}rez-R\'{i}os, S. Ragole, J. Wang and C. H. Greene, J. Chem. Phys. {\bf 140}, 044307 (2014)] has been applied to describe ion-neutral-neutral…
We present a detailed study about ion-atom-atom three-body recombination in hydrogen and deuterium plasmas based on classical trajectory calculations in hyperspherical coordinates. Our results, due to the predominant role of the long-range…
We investigate inelastic collision dynamics of a single cold ion in a Bose-Einstein condensate. We observe rapid ion-atom-atom three-body recombination leading to formation of weakly bound molecular ions followed by secondary two-body…
A classical approach based on hyperspherical coordinates is used to derive a first principle formulation of the the ion-neutral-neutral three-body recombination rate, A$^+$ + A + A $\rightarrow$ $\text{A}_2^+$ + A, in terms of the mass of…
We introduce a framework to investigate ab-initio the dynamics of rare thermally activated reactions. The electronic degrees of freedom are described at the quantum-mechanical level in the Born-Oppenheimer approximation, while the nuclear…
Novel physical mechanism is proposed for explanation of temperature-independent transition reactions in molecular systems. The mechanism becomes effective in the case of conformation transitions between quasi-isoenergetic molecular states.…
We show that a gas-to-liquid phase transition at zero temperature may occur in a coherent gas of bosons in the presence of competing nonlinear effects. This situation can take place both in atomic systems like Bose-Einstein Condensates in…
For many real physico-chemical complex systems detailed mechanism includes both reversible and irreversible reactions. Such systems are typical in homogeneous combustion and heterogeneous catalytic oxidation. Most complex enzyme reactions…
Interaction non-additivity in the chemical context means that binding of certain atom to a reference atom cannot be fully predicted from the interactions of these two atoms with other atoms. This constitutes one of key phenomena determining…
Chemical reactions at ultracold temperature provide an ideal platform to study chemical reactivity at the fundamental level, and to understand how chemical reactions are governed by quantum mechanics. Recent years have witnessed the…
Three-body recombination is a prime example of the fundamental interaction between three particles. Due to the complexity of this process it has resisted a comprehensive description. Experimental investigations have mainly focussed on the…
We propose generating long-range and nonreciprocal three-body interactions in quantum gases via optical feedback. By placing a quasi-two-dimensional Bose-Einstein condensate (BEC) in front of two reflecting mirrors and illuminating it with…
The shell correction is proposed in the improved isospin dependent quantum molecular dynamics (ImIQMD) model, which plays an important role in heavy-ion fusion reactions near Coulomb barrier. By using the ImIQMD model, the static and…
We investigate four-body nuclear reactions in stellar environments contributing to creation of light nuclei, exemplified by $^9$Be and $^{12}$C. The originally assumed process is radiative capture, where nuclear clusters combine into the…
Stable bound quantum states are ubiquitous in nature. Mostly, they result from the interaction of only pairs of particles, so called two-body interactions, even when large complex many-particle structures are formed. We show that…
We investigate the low-temperature reaction rates for radiative capture processes of three particles. We compare direct and sequential capture mechanisms and rates using realistic phenomenological parametrizations of the corresponding…
We discuss three-body recombination of ultra-cold atoms to a weakly bound $s$ level. In this case, characterized by large and positive scattering length $a$ for pair interaction, we find a repulsive effective potential for three-body…
Biomolecular condensates are small droplets forming spontaneously in biological cells via phase separation. They play a role in many cellular processes, but it is unclear how cells control them. Cellular regulation often relies on…