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We report on the crystallographic structure of penta-twinned gold nanoparticles. Although gold typically exhibits a face-centered cubic (fcc) lattice, other phases have been reported in some nanoscale systems. We show that the…

The competition between deformation twinning and dislocation slip underpins the evolution of mesoscale plasticity in face-centered cubic materials. While competition between these mechanisms is known to be related to the critical features…

材料科学 · 物理学 2025-09-18 Ritesh Jagatramka , Matthew Daly

Plasticity in body-centered cubic (BCC) nanocrystals is often associated with twin nucleation phenomena under extreme loading conditions. Here, we reveal unconventional twinning pathways that operate at the intersection of crystal…

High-density and nanosized deformation twins in face-centered cubic (fcc)materials can effectively improve the combination of strength and ductility. However, the microscopic dislocation mechanisms enabling a high twinnability remain…

材料科学 · 物理学 2021-05-13 Song Lu , Xun Sun , Xianghai An , Wei Li , Yujie Chen , Hualei Zhang , Levente Vitos

Plastic deformation of metallic alloys usually takes place through slip, but occasionally involves twinning. In particular, twinning is important in hexagonal close packed materials where the easy slip systems are insufficient to…

材料科学 · 物理学 2018-02-14 Dingyi Sun , Mauricio Ponga , Kaushik Bhattacharya , Michael Ortiz

Stacking defects in noble metal nanoparticles significantly impact their optical, catalytic, and electrical properties. While some mechanisms behind their formation have been studied, the ability to deliberately manipulate nanoparticle bulk…

材料科学 · 物理学 2024-09-04 Ilia Smirnov , Zbigniew Kaszkur , Riccardo Ferrando

Gold nanoclusters have been the focus of numerous computational studies but an atomistic understanding of their structural and dynamical properties at finite temperature is far from satisfactory. To address this deficiency, we investigate…

介观与纳米尺度物理 · 物理学 2018-11-13 Diego Guedes-Sobrinho , Weiqi Wang , Ian Hamilton , Juarez L. F. Da Silva , Luca M. Ghiringhelli

The impact of twin boundaries (TBs) on the microstructure evolution and plastic deformation mechanisms of face-centered cubic (FCC) metals has been extensively studied since the discovery that nanotwinned materials exhibit a favorable…

材料科学 · 物理学 2026-01-28 DeAn Wei , Michael Zaiser , Jing Tang , Xu Zhang

Controlling the self-assembly of surface-adsorbed molecules into nanostructures requires understanding physical mechanisms that act across multiple length and time scales. By combining scanning tunneling microscopy with hierarchical ab…

介观与纳米尺度物理 · 物理学 2014-04-04 Thomas K. Haxton , Hui Zhou , Isaac Tamblyn , Daejin Eom , Zonghai Hu , Jeffrey B. Neaton , Tony F. Heinz , Stephen Whitelam

While nanoalloys are of paramount scientific and practical interests, the main processes leading to their formation are still poorly understood. Key structural features in the alloy systems, including crystal phase, chemical ordering, and…

The freezing behavior of gold nanoclusters was studied by employing molecular dynamics simulations based on a semi-empirical embedded-atom method. Investigations of the gold nanoclusters revealed that, just after freezing, ordered…

原子与分子团簇 · 物理学 2009-11-07 H. -S. Nam , Nong M. Hwang , B. D. Yu , J. -K. Yoon

Molecular dynamics simulations were performed to understand the role of twin boundaries on deformation behaviour of body-centred cubic (BCC) iron (Fe) nanopillars. The twin boundaries varying from one to five providing twin boundary spacing…

材料科学 · 物理学 2016-11-18 G. Sainath , B. K. Choudhary

Twinning is an important mode of plastic deformation in metallic nanopillars. When twinning occurs on multiple systems, it is possible that twins belonging to different twin systems interact and forms a complex twin-twin junctions.…

材料科学 · 物理学 2020-08-04 G. Sainath , Sunil Goyal , A. Nagesha

There is growing interest in promoting deformation twinning for plasticity in advanced materials, as highly organized twin boundaries are beneficial to better strength-ductility combination in contrast to disordered grain boundaries.…

材料科学 · 物理学 2016-04-05 Peng Wang , Shaofeng Xu , Jiabin Liu , Xiaoyan Li , Yujie Wei , Hongtao Wang , Huajian Gao , Wei Yang

We report on the high-pressure optical and mechanical properties of penta-twinned gold nanoparticles (PT-AuNPs) of different geometries: decahedra, rods and bipyramids. Our results show that, unlike single-crystal (SC-AuNPs), PT-AuNPs…

A new mechanism for reactivity of multiply twinned gold nanoparticles resulting from their inherently strained structure provides a further explanation of the surprising catalytic activity of small gold nanoparticles. Atomic defect…

化学物理 · 物理学 2017-07-26 Michael Walsh , Kenta Yoshida , Akihide Kuwabara , Mungo Pay , Pratibha Gai , Edward Boyes

Molecular dynamics simulations performed on <110> Cu nanopillars revealed significant difference in deformation behavior of nanopillars with and without twin boundary. The plastic deformation in single crystal Cu nanopillar without twin…

材料科学 · 物理学 2016-11-07 G. Sainath , B. K. Choudhary

The influence of the physical mechanisms activated during deformation and annealing on the microstructure and texture evolution as well as on the mechanical properties in the equiatomic CoCrFeMnNi high-entropy alloy (HEA) were investigated.…

材料科学 · 物理学 2022-12-26 Christian Haase , Luis A Barrales-Mora

Stochastic geometry provides a powerful framework for modelling complex random structures, with applications in physics, materials science, biology, and other fields. The three-dimensional microstructure of polycrystalline materials is…

数学物理 · 物理学 2025-07-22 Oleksandr Kornijčuk , Luděk Heller , Zbyněk Pawlas , Viktor Beneš

Shape-controlled synthesis of multiply twinned nanostructures is heavily emphasized in nanoscience, in large part due to the desire to control the size, shape, and terminating facets of metal nanoparticles for applications in catalysis.…

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