相关论文: When Blinking Helps: Suppressed Biexciton Emission…
We investigated the influence of the photonic mode density (PMD) on the triplet dynamics of individual chromophores on a dielectric interface by comparing their response in the presence and absence of a nearby gold film. Lifetimes of the…
Single-photon sources based on neutral or charged excitons in a semiconductor quantum dot are attractive resources for photonic quantum computers and simulators. To obtain indistinguishable photons, the source is pumped on resonance with…
We report on a scheme for the creation of time-bin entangled states out of two subsequent single photons. Both photons arrive on the same input port of a beamsplitter and the situation in which the photons leave the beamsplitter on…
We report the first doping of crystalline methylammonium lead bromide (MAPbBr$_3$) perovskite thin-films with CdSe/CdZnS core/shell quantum dots (QDs), using a soft-chemistry method that preserves their high quantum yield and other…
Single-photon purity is one of the most important key metrics of many quantum states of light. For applications in photonic quantum technologies, e.g. quantum communication and linear optical quantum computing, a minimization of the…
Based on first-principles calculations, we show that chemically active metal ns2 lone pairs play an important role in exciton relaxation and dissociation in low-dimensional halide perovskites. We studied excited-state properties of several…
Unlike normal fluorescent methods that use the intensity as a direct measurement of the localized enhanced field, we use blinking statistics of quantum dots (QDs). We have already shown that blinking gives a more accurate characterization…
Among all excitonic complexes in transition-metal dichalcogenides (TMDs), dark and semi-dark trions are poised to play a stellar role in future quantum technologies due to their long lifetimes, about two orders of magnitude greater than…
Quantum degeneracy modifies light scattering and spontaneous emission. For fermions, Pauli blocking leads to a suppression of both processes. In contrast, in a weakly interacting Bose-Einstein condensate, we find spontaneous emission to be…
The desire to produce high-quality single photons for applications in quantum information science has lead to renewed interest in exploring solid-state emitters in the weak excitation regime. Under these conditions it is expected that…
Cooperative emission of photons from an ensemble of quantum dots (QDs) as superradiance can arise from the electronically coupled QDs with a coherent emitting excited state. This contrasts with superfluorescence (Dicke superradiance), where…
Perovskite quantum dots (PQDs) provide a robust solution-based approach to efficient solar cells, bright light-emitting devices, and quantum sources of light. Quantifying heterogeneity and understanding coupling between dots is critical for…
We demonstrate that the cycling between internal states of quantum dots during fluorescence blinking can be used to tune the near-field coupling with a sharp tip. In particular, the balance between tip-induced field enhancement and energy…
A detailed analysis of the electro-optical response of single as well as coupled semiconductor quantum dots is presented. This is based on a realistic ---i.e., fully tridimensional--- description of Coulomb-correlated few-electron states,…
We show that for the very same reason that excitons are bright, i.e. coupled to photons, they have a higher energy than dark excitons, even for electrons spatially separated from holes, such as in a double quantum well. Indeed, the same…
We propose using Quantum Dots as novel targets to probe sub-GeV dark matter-electron interactions. Quantum dots are nanocrystals of semiconducting material, which are commercially available, with gram-scale quantities suspended in…
We report the slow-light enhanced spin-resolved in-plane emission from a single quantum dot (QD) in a photonic crystal waveguide (PCW). The slow light dispersions in PCWs are designed to match the emission wavelengths of single QDs. The…
A rate equation model for the dark and bright excitons kinetics is proposed which explains the wide variation in the observed degree of circular polarization of the PL emission in different TMDs monolayers. Our work suggests that the dark…
The optical properties of transition metal dichalcogenide monolayers such as the two-dimensional semiconductors MoS$_2$ and WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. The light emission yield depends on whether…
We demonstrate experimentally an enhanced delayed fluorescence in tetracene single crystals strongly coupled to optical modes in open cavities formed by arrays of plasmonic nanoparticles. Hybridization of singlet excitons with collective…