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The newly identified field-induced up-up-down order in Ba$_3$CoSb$_2$O$_9$ etc. renewed attention on exotic phases in spin-1/2 triangular-lattice antiferromagnets. Here, we report a unique zero-field noncoplanar up,up,down, down,down,up…

强关联电子 · 物理学 2024-11-05 X. G. Zheng , M. Hagihala , I. Yamauchi , E. Nishibori , T. Honda , T. Yuasa , C. -N. Xu

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

强关联电子 · 物理学 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

Frustrated magnetism on the kagome lattice has been a fertile ground for rich and fascinating physics, ranging from experimental evidence of a spin liquid to theoretical predictions of exotic superconductivity. Among experimentally realized…

The ground state of the simple Heisenberg nearest-neighbor quantum kagome antiferromagnetic model is a magnetically disordered spin liquid, yet various perturbations may lead to fundamentally different states. Here we disclose the origin of…

The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of…

强关联电子 · 物理学 2011-03-16 Philippe Mendels , Fabrice Bert

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

The antiferromagnetism in $\alpha$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying…

强关联电子 · 物理学 2019-10-23 Yuan Wei , Zili Feng , Clarina dela Cruz , Wei Yi , Zi Yang Meng , Jia-Wei Mei , Youguo Shi , Shiliang Li

Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

强关联电子 · 物理学 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

强关联电子 · 物理学 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

We investigate the structural, electronic and magnetic properties of the newly synthesized mineral barlowite Cu4(OH)6FBr which contains Cu2+ ions in a perfect kagome arrangement. In contrast to the spin-liquid candidate herbertsmithite…

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

强关联电子 · 物理学 2009-11-13 R. Chitra , M. J. Rozenberg

The field of frustrated magnetism has been enriched significantly by the discovery of various kagome lattice compounds. These materials exhibit a great variety of macroscopic behaviours ranging from magnetic orders to quantum spin liquids.…

强关联电子 · 物理学 2015-08-10 Tsezar F. Seman , Cheng-Chien Chen , Rajiv R. P. Singh , Michel van Veenendaal

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

Recent discoveries in neutron scattering experiments for Kapellasite and Herbertsmithite as well as theoretical calculations of possible spin liquid phases have revived interest in magnetic phenomena on the kagome lattice. We study the…

强关联电子 · 物理学 2015-06-15 Raik Suttner , Christian Platt , Johannes Reuther , Ronny Thomale

We present the crystal structure and magnetic properties of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$, a stoichiometric frustrated quantum spin system with slightly distorted kagome layers. Single crystals of Y$_{3}$Cu$_{9}$(OH)$_{19}$Cl$_{8}$…

Herbertsmithite, ZnCu3(OH)6Cl2, is the prototype candidate for a spin liquid behavior on a geometrically perfect kagome lattice. Its discovery and the absence of any evidence for spin-freezing down to the lowest probed temperature to-date…

强关联电子 · 物理学 2015-05-28 P. Mendels , F. Bert

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

Quantum antiferromagnets based on the square-kagome lattice are proving to be a fertile platform for realizing nontrivial phenomena in frustrated magnetism. Recently, several decorated square-kagome compounds of the nabokoite family have…

强关联电子 · 物理学 2025-05-19 Matías G. Gonzalez , Yasir Iqbal , Johannes Reuther , Harald O. Jeschke

We present the hydrothermal synthesis, as well as structural and chemical analysis of single crystals on the compounds EuCu$_{3}$(OH)$_{6}$Cl$_{3}$, Zn$_{x}$Cu$_{4-x}$(OH)$_{6}$(NO$_{3}$)$_{2}$ and haydeeite, MgCu$_{3}$(OH)$_{6}$Cl$_{2}$…

强关联电子 · 物理学 2018-10-23 Pascal Puphal , Katharina M. Zoch , Joy Désor , Michael Bolte , Cornelius Krellner
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