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We report Zeeman infra-red spectroscopy of electronic-nuclear levels of $^5$I$_8 \rightarrow ^5$I$_7$ transitions of Ho$^{3+}$ in the C$_{\rm 4v}$(F$^-$) centre in CaF$_2$ with the magnetic field along the $\langle 111\rangle$ direction of…

材料科学 · 物理学 2025-10-20 Kieran M. Smith , Michael F. Reid , Jon-Paul R. Wells

Hyperfine interactions couple nuclear and electronic degrees of freedom. The present work explores how hyperfine coupling within the Tm ions in TmVO$_4$ single crystals affects an electronic ferroquadrupole ordered ground state and its…

强关联电子 · 物理学 2025-09-16 Mark P. Zic , Chao Huan , Nicolas Silva , Yuntian Li , Mark W. Meisel , Ian R. Fisher

In many important situations the dominant dephasing mechanism in cryogenic rare-earth-ion doped systems is due to magnetic field fluctuations from spins in the host crystal. Operating at a magnetic field where a transition has a zero…

原子物理 · 物理学 2015-06-03 D. L. McAuslan , J. G. Bartholomew , M. J. Sellars , J. J. Longdell

We study an infinite-range coupled electronic-quadrupole and nuclear-spin model for ferro-quadrupolar and nuclear-spin ordering in TmVO$_4$ in external magnetic and strain fields. This material is an experimental realization of a…

强关联电子 · 物理学 2026-03-24 Sayan Ghosh , Anirudha Menon , Manoranjan Kumar , Rajiv R. P. Singh

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…

We investigated electron-nuclear spin entanglement in the paramagnetic ground state of the Ho-based cubic compound HoCo2Zn20. From analyses of magnetization and specific heat data, we determined the cubic crystalline electric field (CEF)…

Rare-earth ions doped in crystals with low nuclear-spin densities are highly promising candidates for quantum technology applications. In this study, we investigated the spectroscopic properties of the 7F0 - 5 D0 optical and the hyperfine…

High-resolution Zeeman spectroscopy of electronic-nuclear hyperfine levels of ${^5\mathrm{I}_8}\rightarrow{^5\mathrm{I}_7}$ transitions in Ho$^{3+}$:Y$_2$SiO$_5$ is reported. Crystal-field parameters determined for the two $C_1$ symmetry…

Er-doped Si is a promising candidate for quantum information applications due to its telecom wavelength optical transition and its compatibility with Si nanofabrication technologies. Recent spectroscopic studies based on photoluminescence…

We analyze nuclear spin dynamics in quantum dots and defect centers with a bound electron under electron-mediated coupling between nuclear spins due to the hyperfine interaction ("J-coupling" in NMR). Our analysis shows that the Overhauser…

介观与纳米尺度物理 · 物理学 2008-11-04 D. Klauser , W. A. Coish , Daniel Loss

We characterize the Europium (Eu$^{3+}$) hyperfine interaction of the excited state ($^5$D$_0$) and determine its effective spin Hamiltonian parameters for the Zeeman and quadrupole tensors. An optical free induction decay method is used to…

Drawing inspiration from the recent breakthroughs in the \ce{Na_{2}BaCo(PO_{4})_{2}} quantum magnet, renowned for its spin supersolidity phase and its potential for revolutionary cooling applications, our study delves into the intricate…

We investigate the hyperfine energy levels and Zeeman splittings for homonuclear alkali-metal dimers in low-lying rotational and vibrational states, which are important for experiments designed to produce quantum gases of deeply bound…

原子物理 · 物理学 2010-03-09 J. Aldegunde , Jeremy M. Hutson

The invariant form of the hyperfine interaction between multipolar moments and the nuclear spin is derived, and applied to discuss possibilities to identify the antiferro-octupolar (AFO) moments by NMR experiments. The ordered phase of…

强关联电子 · 物理学 2009-11-10 Osamu Sakai , Ryousuke Shiina , Hiroyuki Shiba

We report the first observation of electromagnetically induced transparency (EIT) in an isotopically purified Nd$^{3+}$:YLiF$_4$ crystal. This crystal demonstrates inhomogeneous broadening of optical transitions of about 35 MHz. EIT is…

We describe the quantum phases of interacting three component fermions in the presence of spin-orbit coupling, as well as linear and quadratic Zeeman fields. We classify the emerging superfluid phases in terms of the loci of zeros of their…

量子气体 · 物理学 2016-12-08 Doga Murat Kurkcuoglu , C. A. R. Sa de Melo

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. We report the results of the calculations of the rate of laser-induced…

原子物理 · 物理学 2018-03-21 Vladimir I. Korobov , Petar Danev , Dimitar Bakalov , Stephan Schiller

Nuclear magnetic resonance (NMR) is particularly relevant for studies of internuclear spin coupling at zero and ultra-low fields (ZULF), where spin-spin interactions dominate over Zeeman ones. Here we report on ZULF NMR in CdTe. In this…

介观与纳米尺度物理 · 物理学 2024-03-27 V. M. Litvyak , P. Bazhin , R. André , M. Vladimirova , K. V. Kavokin

Erbium ions doped into crystals have unique properties for quantum information processing, because of their optical transition at 1.5 $\mu$m and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most…

The dependence of the magnetic fluctuations and the spin coherence time $T_2^{\rm hyp}$ of the lowest Stark states $^4I_{15/2}\ (Z_1)$ in $^{167}$Er$^{3+}$:Y$_2$SiO$_5$ under zero magnetic field on Er concentration is numerically…

量子物理 · 物理学 2026-02-20 K. Matsuura , S. Yasui , R. Kaji , H. Sasakura , T. Tawara , S. Adachi
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