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We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…

原子物理 · 物理学 2015-10-28 Woojun Lee , Hyosub Kim , Kyungtae Kim , Jaewook Ahn

We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…

We incorporate deep learning (DL) into coherent beam combining (CBC) systems for the first time, to the best of our knowledge. Using a well-trained convolutional neural network DL model, the phase error in CBC systems could be accurately…

We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon…

量子物理 · 物理学 2009-11-13 Matthew C. Stowe , Avi Pe'er , Jun Ye

We derive composite pulse sequences that achieve high-fidelity excitation of two-state systems in an optically dense, inhomogeneously broadened ensemble. The composite pulses are resistant to distortions due to the back-action of the medium…

量子物理 · 物理学 2016-02-24 Gabor Demeter

Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as…

量子物理 · 物理学 2023-11-17 Anatoly Shukhin , Inbar Hurvitz , Sivan Trajtenberg-Mills , Ady Arie , Hagai Eisenberg

Defects in solid-state materials play a central role in determining coherence, stability, and performance in quantum technologies. Although narrowband techniques can probe specific resonances with high precision, a broadband spectroscopic…

In multi-dimensional time-resolved spectroscopic experiments, multiple (more than two) short laser pulses with variable pulse delay times are employed for the time-resolved exploration of the photoinduced dynamics of molecular chromophores.…

化学物理 · 物理学 2026-03-25 Sebastian V. Pios , Maxim F. Gelin , Wolfgang Domcke , Lipeng Chen

Orthogonal frequency division multiplexing (OFDM) signals with rectangular pulses exhibit low spectral confinement. Shaping their power spectral density (PSD) is imperative in the increasingly overcrowded spectrum to benefit from the…

信号处理 · 电气工程与系统科学 2026-01-01 Javier Giménez , José A. Cortés , Luis Díez

Optical two-dimensional (2D) coherent spectroscopy excels in studying coupling and dynamics in complex systems. The dynamical information can be learned from lineshape analysis to extract the corresponding linewidth. However, it is usually…

光学 · 物理学 2020-06-24 Srikanth Namuduri , Michael Titze , Shekhar Bhansali , Hebin Li

We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities…

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

Coherent dual-comb spectroscopy (DCS) enables high-resolution measurements at high speeds without the trade-off between resolution and update rate inherent to mechanical delay scanning approaches. However, high system complexity and limited…

Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and…

光学 · 物理学 2020-10-21 Bachana Lomsadze , Steven T. Cundiff

Two- and multi-dimensional spectroscopy is used in physics and chemistry to obtain structural and dynamical information that would otherwise be invisible by the projection into a one-dimensional data set such as a single emission or…

We investigate how the quantum control of a two-level system (TLS) coupled to photons can modify and tune the TLS's photon absorption spectrum. Tuning and controlling the emission and the absorption is of much interest e.g.\ for the…

量子物理 · 物理学 2017-06-07 H. F. Fotso , V. V. Dobrovitski

Within the well-established optical response function formalism, a new strategy with the central idea of employing the forward-backward stochastic Schr\"{o}dinger equations in a segmented way to accurately obtain the two-dimensional (2D)…

化学物理 · 物理学 2018-08-08 Yaling Ke , Yi Zhao

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

光学 · 物理学 2023-12-01 Shicheng Jiang , Mahesh Gudem , Markus Kowalewski , Konstantin Dorfman

Multidimensional Coherent Optical Photocurrent Spectroscopy (MD-COPS) is implemented using unstabilized interferometers. Photocurrent from a semiconductor sample is generated using a sequence of four excitation pulses in a collinear…

光学 · 物理学 2013-11-14 Gaël Nardin , Travis M. Autry , Kevin L. Silverman , Steven T. Cundiff

The ability of scene understanding has sparked active research for panoramic image semantic segmentation. However, the performance is hampered by distortion of the equirectangular projection (ERP) and a lack of pixel-wise annotations. For…

计算机视觉与模式识别 · 计算机科学 2023-03-28 Xu Zheng , Jinjing Zhu , Yexin Liu , Zidong Cao , Chong Fu , Lin Wang