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Ultrafast demagnetization induced by femtosecond laser pulses in thin metallic layers is caused by the outflow of spin-polarized hot electron currents describable by the superdiffusive transport model. These laser-generated spin currents…

介观与纳米尺度物理 · 物理学 2023-05-24 Pavel Baláž , Maciej Zwierzycki , Francesco Cosco , Karel Carva , Pablo Maldonado , Peter M. Oppeneer

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

材料科学 · 物理学 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

材料科学 · 物理学 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

Demagnetization in ferromagnetic transition metals driven by a femtosecond laser pulse is a fundamental problem in solid state physics, and its understanding is essential to the development of spintronics devices. Ab initio calculation of…

材料科学 · 物理学 2024-01-02 Mitsuko Murakami , G. P. Zhang

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

材料科学 · 物理学 2010-07-06 Adrian Glaubitz

Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

强关联电子 · 物理学 2015-11-25 W. Töws , G. M. Pastor

Induced by an ultra-short laser pulse, the electronic structure of a material undergoes strong modifications leading to a fast demagnetization in magnetic materials. Induced spin-flip transitions are one of the reasons for demagnetization,…

材料科学 · 物理学 2024-04-29 Sergiy Mankovsky , Svitlana Polesya , Hubert Ebert

Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely-used three-temperature model (3TM). Here, we…

材料科学 · 物理学 2024-01-17 Markus Weißenhofer , Peter M. Oppeneer

Laser-induced terahertz spin transport (TST) and ultrafast demagnetization (UDM) are central but so far disconnected phenomena in femtomagnetism and terahertz spintronics. Here, we use broadband terahertz emission spectroscopy to reliably…

The discovery of femtosecond laser-induced ultrafast demagnetization in 1996 opened a new field, femtomagnetism, in which magnetic order can be quenched on timescales shorter than a picosecond. This seminal observation revealed that angular…

材料科学 · 物理学 2026-04-29 Quentin Remy , Stéphane Mangin

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

With the goal of pushing Spintronic devices towards faster and faster timescales, we demonstrate, using ab-intio time-dependent density functional theory simulations of bulk Heusler compounds subject to ultrashort intense laser pulses, that…

材料科学 · 物理学 2016-03-18 P. Elliott , T. Müller , J. K. Dewhurst , S. Sharma , E. K. U. Gross

The ultrafast demagnetization (UFD) dynamics of itinerant ferromagnets is theoretically investigated as a function of the characteristics of the initial laser excitation. A many-body pd-band Hamiltonian is considered which takes into…

强关联电子 · 物理学 2019-07-10 W. Töws , G. M. Pastor

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

材料科学 · 物理学 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

强关联电子 · 物理学 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

A systematic investigation of spin injection behavior in Au/FM (FM = Fe and Ni) multilayers is performed using the superdiffusive spin transport theory. By exciting the nonmagnetic layer, the laser-induced hot electrons may transfer spin…

介观与纳米尺度物理 · 物理学 2023-11-20 Wen-Tian Lu , Zhe Yuan , Xiaohong Xu

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

材料科学 · 物理学 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

The dynamics of ultrafast demagnetisation in 3$d$ magnets is complicated by the presence of both spin ${\v S}$ and orbital ${\v L}$ angular momentum, with the microscopic mechanism by which the magnetic moment is redistributed to the…

A major question in the field of femtosecond laser-induced demagnetization is whereto the angular momentum lost by the electrons is transferred. Recent ultrafast electron diffraction measurements [Tauchert \textit{et al.}, Nature {\bf 602},…

材料科学 · 物理学 2025-12-08 M. S. Mrudul , Markus Weißenhofer , Peter M. Oppeneer
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