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Living cells use phase separation and concentration gradients to organize chemical compartments in space. Here, we present a theoretical study of droplet dynamics in gradient systems. We derive the corresponding growth law of droplets and…

生物物理 · 物理学 2017-05-19 Christoph A. Weber , Chiu Fan Lee , Frank Jülicher

The mechanism of coalescence of aqueous droplet pairs under an electric field is quantitatively studied using microfluidics in quiescent conditions. We experimentally trap droplet pairs and apply electric fields with varying frequencies and…

软凝聚态物质 · 物理学 2024-11-27 David Van Assche , Thomas Beneyton , Alexandre Baron , Jean-Christophe Baret

Driven chemical reactions can control the macroscopic properties of droplets, like their size. Such active droplets are critical in structuring the interior of biological cells. Cells also need to control where and when droplets appear, so…

软凝聚态物质 · 物理学 2024-03-15 Noah Ziethen , Jan Kirschbaum , David Zwicker

Phase separation is the thermodynamic process that explains how droplets form in multicomponent fluids. These droplets can provide controlled compartments to localize chemical reactions, and reactions can also affect the droplets' dynamics.…

软凝聚态物质 · 物理学 2022-09-02 David Zwicker

New experimental results and their physical analysis are presented to clarify the behavior of a relatively stable self-arranged droplet cluster levitating over the locally heated water surface. An external electric field of both opposite…

We study the hydrodynamics and shape changes of chemically active droplets. In non-spherical droplets, surface tension generates hydrodynamic flows that drive liquid droplets into a spherical shape. Here we show that spherical droplets that…

生物物理 · 物理学 2018-11-12 Rabea Seyboldt , Frank Jülicher

In both biological and artificial systems, concentration gradients can serve as a convenient mechanism for manipulating particles and generating motility. Particles that interact with a solute will move along its gradient; if they…

软凝聚态物质 · 物理学 2011-07-21 Gareth P. Alexander , Andrea J. Liu

Using molecular dynamics simulations and scaling arguments, we investigate the coalescence preference dynamics of liquid droplets in a phase-segregating off-critical, single-component fluid. It is observed that the preferential distance of…

统计力学 · 物理学 2019-03-25 Sutapa Roy

When droplets are tightly packed in a 2D microchannel, coalescence of a pair of droplets can trigger an avalanche of coalescence events that propagate through the entire emulsion. This propagation is found to be stochastic, i.e. every…

软凝聚态物质 · 物理学 2023-09-25 Danny Raj Masila , Pavithra Sivakumar , Arshed Nabeel

The coalescence of liquid drops has conventionally been thought to have just two regimes when the drops are brought together slowly in vacuum or air: a viscous regime corresponding to the Stokes-flow limit and a later inertially-dominated…

流体动力学 · 物理学 2014-01-10 Joseph D. Paulsen

Three-dimensional, time-dependent direct simulations of step emulsification micro-devices highlight two essential mechanisms for droplet formation: first, the onset of an adverse pressure gradient driving a back-flow of the continuous phase…

计算物理 · 物理学 2020-06-22 Andrea Montessori , Marco Lauricella , Sauro Succi , Elad Stolovicki , David A. Weitz

By varying the oil volume fraction, the microscopic droplet size and the macroscopic rheology of emulsions are investigated in a Taylor-Couette (TC) turbulent shear flow. Although here oil and water in the emulsions have almost the same…

流体动力学 · 物理学 2022-11-23 Lei Yi , Cheng Wang , Thomas van Vuren , Detlef Lohse , Frederic Risso , Federico Toschi , Chao Sun

The mass and size distributions are the key characteristics of any astrophysical objects, including the densest clumps comprising the cold phase of multiphase environments. In our recent papers, we showed how individual clouds of various…

星系天体物理 · 物理学 2019-05-01 Tim Waters , Daniel Proga

Cloud droplets grow via vapor condensation and collisional aggregation. Upon reaching approximately $\approx 100~{\rm \mu m}$, their inertia allows them to capture smaller droplets during descent, initiating rain. Here, we show that…

流体动力学 · 物理学 2024-10-16 Florian Poydenot , Bruno Andreotti

The expected universal dynamics associated with the initial stage of droplet coalescence are difficult to study visually due to the rapid motion of the liquid and the awkward viewing geometry. Here we employ an electrical method to study…

软凝聚态物质 · 物理学 2009-11-13 Sarah C. Case , Sidney R. Nagel

These lecture notes describe a basic theory of chemically active droplets, which are droplets kept away from equilibrium by driven chemical reactions. The notes assume a basic familiarity with equilibrium thermodynamics of phase separation,…

软凝聚态物质 · 物理学 2024-07-16 David Zwicker

The stable configurations formed by two viscoelastic, ellipsoid-shaped droplets during their arrested coalescence has been investigated using micromanipulation experiments. Ellipsoidal droplets are produced by millifluidic emulsification of…

软凝聚态物质 · 物理学 2018-08-14 Chen Hao , Zhaoyu Xie , Timothy J. Atherton , Patrick T. Spicer

Liquid-liquid phase separation is an important mechanism for compartmentalizing the cell's cytoplasm, allowing the dynamic organization of the components necessary for survival. However, it is not clear how phase separation is affected by…

软凝聚态物质 · 物理学 2022-01-31 Estefania Vidal-Henriquez , David Zwicker

With most of the focus to date having been on the coalescence of freely suspended droplets, much less is known about the coalescence of sessile droplets, especially in the case of droplets laden with surfactant. Here, we employ large-scale…

软凝聚态物质 · 物理学 2024-03-19 S. Arbabi , P. Deuar , R. Bennacer , Z. Che , P. E. Theodorakis

Modification and control over the vaporization kinetics of microfluidic droplets may have strong utilitarian implications in several scientific and technological applications. The article reports the control over the vaporization kinetics…

流体动力学 · 物理学 2020-06-02 Purbarun Dhar , Vivek Jaiswal , Hanumant Chate , Lakshmi Sirisha Maganti