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Trains of ultrashort laser pulses separated by the time of rotational revival (typically, tens of picoseconds) have been exploited for creating ensembles of aligned molecules. In this work we introduce a chiral pulse train - a sequence of…

量子物理 · 物理学 2013-05-29 S. Zhdanovich , A. A. Milner , C. Bloomquist , J. Floß , I. Sh. Averbukh , J. W. Hepburn , V. Milner

We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

化学物理 · 物理学 2014-06-06 C T L Smeenk , P B Corkum

Polar active particles constitute a wide class of synthetic colloids that are able to propel along a preferential direction, given by their polar axis. Here, we demonstrate a generic self-phoretic mechanism that leads to their spontaneous…

软凝聚态物质 · 物理学 2021-10-27 Marco De Corato , Ignacio Pagonabarraga , Giovanniantonio Natale

Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…

Spontaneous orientation polarization (SOP) occurs when molecules with a finite permanent dipole moment are grown as thin films by physical vapor deposition and their alignment is such that a net non-zero polarization remains. We discuss how…

材料科学 · 物理学 2025-11-12 Albin Cakaj , Markus Schmid , Alexander Hofmann , Wolfgang Brütting

While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…

原子物理 · 物理学 2013-02-27 Felipe Herrera , Sabre Kais , K. Birgitta Whaley

We explore a pure optical method for enantioselective orientation of chiral molecules by means of laser fields with twisted polarization. Several field implementations are considered, including a pair of delayed cross-polarized laser…

化学物理 · 物理学 2018-03-23 I. Tutunnikov , E. Gershnabel , S. Gold , I. Sh. Averbukh

The propensity of molecules to spatially align along the polarization vector of intense, pulsed light fields is related to readily-accessible parameters (molecular polarizabilities, moment of inertia, peak intensity of the light and its…

原子物理 · 物理学 2009-11-06 S. Banerjee , D. Mathur , G. Ravindra Kumar

We show that it is possible to generate continuous-wave fields and pulses of polarization squeezed light by sending classical, linearly polarized laser light twice through an atomic sample which causes an optical Faraday rotation of the…

量子物理 · 物理学 2011-10-13 Jacob F. Sherson , Klaus Molmer

The induced polarization oscillations in a one-dimensional rectangular quantum well are modeled by a numerical solution of the time-dependent Schroedinger equation. The finite-difference discretization over time is realized in the framework…

介观与纳米尺度物理 · 物理学 2023-04-25 Pavel Belov , Rostislav Arkhipov

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

原子物理 · 物理学 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We show the approximate rotational controllability of a polar linear molecule by means of three nonresonant linear polarized laser fields. The result is based on a general approximate controllability result for the bilinear Schr\"odinger…

最优化与控制 · 数学 2013-02-14 Ugo Boscain , Marco Caponigro , Mario Sigalotti

The dynamics of short intense electromagnetic pulses propagating in a relativistic pair plasma with small temperature asymmetry is of current interest. Such pulses were shown to be governed by a nonlinear Schrodinger equation with a new…

偏微分方程分析 · 数学 2026-02-10 Luciano Medina

Using special capacitors our experiments discovered that the ground state K, Rb or Cs atom is polar atom with a large permanent electric dipole moment (EDM) of the order of eao (ao is Bohr radius) as excited state of hydrogen atom. But we…

原子物理 · 物理学 2009-01-12 Pei-Lin You

We report a theoretical study of the optical centrifuge acceleration of an asymmetric top molecule interacting with an electric static field by solving the time-dependent Schr\"odinger equation in the rigid rotor approximation. A detailed…

化学物理 · 物理学 2018-02-14 Juan J. Omiste

We present a theoretical study of the impact of an electrostatic field combined with non-resonant linearly polarized laser pulses on the rotational dynamics of linear molecules. Within the rigid rotor approximation, we solve the…

原子物理 · 物理学 2015-06-05 Juan J. Omiste , Rosario González-Férez

We investigate rotational state changes in a single collision of diatomic molecular ions, polar or apolar, with an atomic ion. Rotational state changes may occur since the angular degree of freedom of the molecular ions interacts with the…

量子物理 · 物理学 2026-04-20 J. Martin Berglund , Michael Drewsen , Christiane P. Koch

We analyze the alignment of molecules generated by a pair of crossed ultra-short pump pulses of different polarizations by a technique based on the induced time-dependent gratings. Parallel polarizations yield an intensity grating, while…

量子物理 · 物理学 2009-11-13 Arnaud Rouzee , Vincent Renard , Stephane Guerin , Olivier Faucher , Bruno Lavorel

Short laser pulses are widely used for controlling molecular rotational degrees of freedom and inducing molecular alignment, orientation, unidirectional rotation and other types of coherent rotational motion. To follow the ultra-fast…

The photon-induced process of electron-positron pair creation in a strong homogeneous magnetic field, provided that the polarization of particles is arbitrary, has been considered. The polarization of a photon is described in terms of the…

高能物理 - 唯象学 · 物理学 2010-02-08 O. P. Novak , R. I. Kholodov