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Many nanoelectronic devices rely on thin dielectric barriers through which electrons tunnel. For instance, aluminium oxide barriers are used as Josephson junctions in superconducting electronics. The reproducibility and drift of circuit…

介观与纳米尺度物理 · 物理学 2020-02-05 M. J. Cyster , J. S. Smith , J. A. Vaitkus , N. Vogt , S. P. Russo , J. H. Cole

Many phenomena in condensed matter are thought to result from competition between different ordered phases. Palladium is a paramagnetic metal close to both ferromagnetism and superconductivity, and is therefore a potentially interesting…

介观与纳米尺度物理 · 物理学 2010-05-14 Gavin D. Scott , Juan J. Palacios , Douglas Natelson

First principle calculations of the conductance of gold wires containing 3-8 atoms each with 2.39 {\AA} bond length were performed using density functional theory. Three different configuration of wire/electrodes were used. For zigzag wire…

We study theoretically the length dependence of both conductance and thermopower in metal-molecule-metal junctions made up of dithiolated oligophenylenes contacted to gold electrodes. We find that while the conductance decays exponentially…

介观与纳米尺度物理 · 物理学 2009-05-24 F. Pauly , J. K. Viljas , J. C. Cuevas

Metallic atomic junctions pose the ultimate limit to the scaling of electrical contacts. They serve as model systems to probe electrical and thermal transport down to the atomic level as well as quantum effects occurring in one-dimensional…

介观与纳米尺度物理 · 物理学 2017-05-24 Nico Mosso , Ute Drechsler , Fabian Menges , Peter Nirmalraj , Siegfried Karg , Heike Riel , Bernd Gotsmann

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the…

介观与纳米尺度物理 · 物理学 2016-08-31 R. Gutierrez , G. Fagas , K. Richter , F. Grossmann , R. Schmidt

Suspended chains consisting of single noble metal and oxygen atoms have been formed. We provide evidence that oxygen can react with and be incorporated into metallic one-dimensional atomic chains. Oxygen incorporation reinforces the linear…

介观与纳米尺度物理 · 物理学 2017-12-11 W. H. A. Thijssen , M. Strange , J. M. J. aan de Brugh , J. M. van Ruitenbeek

Using benzene sandwiched between two Au leads as a model system, we investigate from first principles the change in molecular conductance caused by different atomic structures around the metal-molecule contact. Our motivation is the…

材料科学 · 物理学 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

Despite many similarities between electronics and optics, the hopping of the electron on a discrete atomic lattice gives rise to energy band nonparabolicity and anisotropy. The crucial influences of this effect on material properties and…

介观与纳米尺度物理 · 物理学 2019-04-30 Shu-Hui Zhang , Wen Yang , Kai Chang

Despite extensive investigations of dissipation and deformation processes in micro- and nano- sized metallic samples, the mechanisms at play during deformation of systems with ultimate, molecular size remain elusive. While metallic…

介观与纳米尺度物理 · 物理学 2021-02-08 Jean Comtet , Antoine Lainé , Antoine Niguès , Lydéric Bocquet , Alessandro Siria

In organic semiconductors charge transport typically takes place via slow hopping processes. Molecular aggregation can lead to enhanced exciton and charge transport through coupling of the transition dipole moments. In this work, we…

Electrical resistivity in good metals, particularly noble metals such as gold (Au), silver (Ag), or copper, increases linearly with temperature ($T$) for $T > \Theta_{\mathrm{D}}$, where $\Theta_{\mathrm{D}}$ is the Debye temperature. This…

One of the salient features of graphene is the very high carrier mobility that implies tremendous potential for use in electronic devices. Unfortunately, transport measurements find the expected high mobility only in freely suspended…

介观与纳米尺度物理 · 物理学 2015-06-04 Søren Ulstrup , Marco Bianchi , Richard Hatch , Dandan Guan , Alessandro Baraldi , Dario Alfè , Liv Hornekær , Philip Hofmann

Designing molecular organic semiconductors with distinct frontier orbitals is key for the development of devices with desirable properties. Generating defined organic nanostructures with atomic precision can be accomplished by on-surface…

Understanding of the energy exchange between electrons and phonons in metals is important for micro- and nano-manufacturing and system design. The electron-phonon (e-ph) coupling constant is to describe such exchange strength, yet its…

介观与纳米尺度物理 · 物理学 2021-03-17 Wuli Miao , Moran Wang

Quantum aspects, such as electron tunneling between closely separated metallic nanoparticles, are crucial for understanding the plasmonic response of nanoscale systems. We explore quantum effects on the response of the conductively coupled…

材料科学 · 物理学 2015-12-08 Tuomas P. Rossi , Asier Zugarramurdi , Martti J. Puska , Risto M. Nieminen

We achieve, at room temperature, conductance enhancements over two orders of magnitude in single molecule circuits formed with polycyclic benzoquinoidal (BQn) diradicals upon increasing molecular length by ~0.5 nm. We find that this extreme…

介观与纳米尺度物理 · 物理学 2024-03-11 Brent Lawson , Efrain Vidal , Michael M. Haley , Maria Kamenetska

We adapt existing phonon heat transport methods to compute the phononic thermal conductance of metallic atomic contacts during a stretching process. Nonequilibrium molecular dynamics (NEMD) simulations are used to generate atomic…

介观与纳米尺度物理 · 物理学 2019-10-08 D. O. Möhrle , F. Müller , M. Matt , P. Nielaba , F. Pauly

The tunneling spectra of small metallic grains shows an unusual structure of the differential conductance peaks. Namely, resonance peaks appear in clusters, or develop substructure as the the gate voltage is changed. These features are…

凝聚态物理 · 物理学 2007-05-23 Oded Agam

We uncover two anomalous features in the nonlocal transport behavior of two-dimensional metallic materials with spin-orbit coupling. Firstly, the nonlocal resistance can have negative values and oscillate with distance, even in the absence…

介观与纳米尺度物理 · 物理学 2017-10-04 Chunli Huang , Y. D Chong , Miguel A. Cazalilla