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We investigate the resonant two-magnon Raman scattering in two-dimensional (2D) Mott insulators by using a half-filled 2D Hubbard model in the strong coupling limit. By performing numerical diagonalization calculations for small clusters,…

强关联电子 · 物理学 2007-05-23 T. Tohyama , H. Onodera , K. Tsutsui , S. Maekawa

The optical properties of the two-dimensional (2D) crystals are dominated by tightly bound electron-hole pairs (excitons) and lattice vibration modes (phonons). The exciton-phonon interaction is fundamentally important to understand the…

材料科学 · 物理学 2021-02-09 Qing-Hai Tan , Yu-Jia Sun , Xue-Lu Liu , Yanyuan Zhao , Qihua Xiong , Ping-Heng Tan , Jun Zhang

The weakly screened electron-hole interactions in an atomically thin semiconductor not only downshift its excitation spectrum from a quasiparticle one, but also redistribute excitation energies and wavefunction characters with profound…

介观与纳米尺度物理 · 物理学 2018-10-24 Yuanxi Wang , Bruno R. Carvalho , Vincent H. Crespi

Raman spectra of few-layer WS2 have been measured with up to seven excitation energies, and peculiar resonance effects are observed. The two-phonon acoustic phonon scattering signal close to the main E2g1 peak is stronger than the main…

介观与纳米尺度物理 · 物理学 2017-06-07 Jinho Yang , Jae-Ung Lee , Hyeonsik Cheong

We investigate the resonant two-magnon Raman scattering in the two-dimensional (2D) and ladder-type Mott insulators by using a half-filled Hubbard model in the strong coupling limit. By performing numerical diagonalization calculations for…

强关联电子 · 物理学 2009-11-07 Hiroaki Onodera , Takami Tohyama , Sadamichi Maekawa

ReS$_2$ has recently emerged as a new member in the rapidly growing family of two-dimensional materials. Unlike MoS$_2$ or WSe$_2$, the optical and electrical properties of ReS$_2$ are not isotropic due to the reduced symmetry of the…

介观与纳米尺度物理 · 物理学 2016-02-17 Philipp Nagler , Gerd Plechinger , Christian Schüller , Tobias Korn

Monolayers of ReS2 were grown by a chemical vapor deposition technique on SiO2/Si substrates and investigated at room temperature by using micro-Raman, micro-photoluminescence (PL) and absorbance spectroscopies. The Raman scattering…

材料科学 · 物理学 2024-04-23 Solomon Ojo , Juwon Onasanya , Morad Benamara , Bothina Hamad , M. O. Manasreh

Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…

光学 · 物理学 2024-08-13 Minhaeng Cho

Resonant Raman scattering is investigated in monolayer WS$_2$ at low temperature with the aid of an unconventional spectroscopy technique, $i.e.$, Raman scattering excitation (RSE). The RSE spectrum is made up by sweeping the excitation…

介观与纳米尺度物理 · 物理学 2017-07-13 Maciej R. Molas , Karol Nogajewski , Marek Potemski , Adam Babinski

Using resonant Raman scattering spectroscopy with 25 different laser lines, we describe the Raman scattering spectra of mono- and multi-layers 2H-molybdenum diselenide (MoSe$_2$) as well as the different resonances affecting the most…

介观与纳米尺度物理 · 物理学 2016-04-19 P. Soubelet , A. E. Bruchhausen , A. Fainstein , K. Nogajewski , C. Faugeras

We present an ab initio computational approach for the calculation of resonant Raman intensities, including both excitonic and non-adiabatic effects. Our diagrammatic approach, which we apply to two prototype, semiconducting layered…

介观与纳米尺度物理 · 物理学 2020-10-01 Sven Reichardt , Ludger Wirtz

Controlling resonant Raman scattering in two-dimensional semiconductors typically requires tuning the excitation energy to match excitonic transitions. Here we show that mechanical deformation can achieve the same effect without changing…

材料科学 · 物理学 2026-03-27 Álvaro Rodríguez , Carmen Munuera , Andres Castellanos-Gomez

A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…

介观与纳米尺度物理 · 物理学 2009-10-31 E. Menendez-Proupin , C. Trallero-Giner , A. Garcia-Cristobal

We studied the intensity of resonant Raman scattering due to optical phonons in a planar II-VI-type semiconductor microcavity in the regime of strong coupling between light and matter. Two different sets of independent experiments were…

强关联电子 · 物理学 2009-10-20 A. Bruchhausen , L. M. Leon Hilario , A. A. Aligia , A. M. Lobos , A. Fainstein , B. Jusserand , R. Andre

Two-dimensional semiconducting materials have a wide range of applications in various fields due to their excellent properties and rich physics. Here, we report a detailed investigation of the temperature dependent Raman and…

材料科学 · 物理学 2025-05-05 Atul G. Chakkar , Deepu Kumar , Ashok Kumar , Mahesh Kumar , Pradeep Kumar

Unidirectional in-plane structural anisotropy in Rhenium-based transition metal dichalcogenides (TMDs) introduces a new class of 2-D materials, exhibiting anisotropic optical properties. In this work, we perform temperature dependent,…

介观与纳米尺度物理 · 物理学 2020-10-21 Avijit Dhara , Devarshi Chakrabarty , Pritam Das , Aswini K. Pattanayak , Shreya Paul , Shreyashi Mukherjee , Sajal Dhara

We investigate the ultralow-frequency Raman response of atomically thin ReS2, a special type of two-dimensional (2D) semiconductors with unique distorted 1T structure. Bilayer and few-layer ReS2 exhibit rich Raman spectra at frequencies…

介观与纳米尺度物理 · 物理学 2016-02-16 Rui He , Jia-An Yan , Zongyon Yin , Zhipeng Ye , Gaihua Ye , Jason Cheng , Ju Li , C. H. Lui

Under homogeneous uniaxial strains, the Raman 2D band of graphene involving two-phonon double-resonance scattering processes splits into two peaks and they altogether redshift strongly depending on the direction and magnitude of the strain.…

介观与纳米尺度物理 · 物理学 2015-03-19 Duhee Yoon , Young-Woo Son , Hyeonsik Cheong

The discovery of in-plane anisotropic excitons in two-dimensional layered semiconductors enables state-of-the-art nanophotonic applications. A fundamental yet unknown parameter of these quasiparticles is the coherence time (T_2 ), which…

Inelastic light (Raman) scattering has been used to study electronic excitations and phonon anomalies in detwinned, slightly overdoped YBa$_2$Cu$_3$O$_{6.95}$ and moderately overdoped Y$_{0.85}$Ca$_{0.15}$Ba$_2$Cu$_3$O$_{6.95}$ single…

超导电性 · 物理学 2015-05-13 M. Bakr , A. P. Schnyder , L. Klam , D. Manske , C. T. Lin , B. Keimer , M. Cardona , C. Ulrich
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