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High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…

High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…

光学 · 物理学 2025-10-20 Marcelo F. Ciappina

High-order harmonic generation (HHG) is a fundamental process which can be simplified as the production of high energetic photons from a material subjected to a strong driving laser field. This highly nonlinear optical process contains rich…

光学 · 物理学 2021-12-21 Dasol Kim , Yeon Lee , Alexis Chacón , Dong Eon Kim

In transition metal dichalcogenides (TMDCs), charge carriers have spin, pseudospin, and valley degrees of freedom associated with magnetic moments. The monolayers and bilayers of the TMDCs, in particular, MoS$_2$, lead strong couplings…

材料科学 · 物理学 2021-11-29 Yeon Lee , Dasol Kim , Dong Eon Kim , Alexis Chacón

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

材料科学 · 物理学 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…

High-harmonic generation (HHG) in the two topological phases of a finite, one-dimensional, periodic structure is investigated using a self-consistent time-dependent density functional theory (TDDFT) approach. For harmonic photon energies…

光学 · 物理学 2018-04-26 Dieter Bauer , Kenneth K. Hansen

High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

计算物理 · 物理学 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

In this paper we explore the capabilities of MoS2 and WS2 2D monolayers to produce radiation in the terahertz range by generation of high-order harmonics. This phenomenon, which is a result of the non-linear response of the electronic…

应用物理 · 物理学 2024-02-13 Jose Manuel Iglesias , Elena Pascual , Maria J. Martin , Raul Rengel

We theoretically investigate the orientation dependence of high-harmonic generation (HHG) in monolayer transition metal dichalcogenides (TMDCs). We find that, unlike conventional solid-state and atomic layered materials such as graphene,…

材料科学 · 物理学 2017-06-05 Tomohiro Tamaya , Satoru Konabe , Shiro Kawabata

Two-dimensional materials offer a versatile platform to study high-harmonic generation (HHG), encompassing as limiting cases bulk-like and atomic-like harmonic generation [Tancogne-Dejean and Rubio, Science Advance \textbf{4}, eaao5207…

材料科学 · 物理学 2018-10-31 Guillaume Le Breton , Angel Rubio , Nicolas Tancogne-Dejean

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

光学 · 物理学 2018-10-23 Guang-Rui Jia , Xin-Qiang Wang , Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

材料科学 · 物理学 2020-12-23 G. P. Zhang , Y. H. Bai

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far…

材料科学 · 物理学 2018-09-12 G. P. Zhang , M. S. Si , M. Murakami , Y. H. Bai , Thomas F. George

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

原子物理 · 物理学 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

We theoretically investigated the dependence of higher-order harmonic generation (HHG) in solid-state materials on the ellipticity of the electric field. We found that in the multiphoton absorption and ac Zener regimes, the intensity of HHG…

材料科学 · 物理学 2016-12-28 T. Tamaya , A. Ishikawa , T. Ogawa , K. Tanaka

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

材料科学 · 物理学 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

We report a coherent layer-by-layer high-order harmonic generation (HHG) build-up in artificially stacked transition metal dichalcogenides (TMDC) crystals in their various stacking configurations. In the experiments, millimeter-sized single…

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