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Motivated by the recent experimental discovery of superconductivity in the infinite-layer nickelate Nd0.8Sr0.2NiO2 [Li et al., Nature 572, 624 (2019)], we study how the correlated Ni 3dx2-y2 electrons in the NiO2 layer interact with the…

Recent discovery of superconductivity in the doped infinite-layer nickelates has renewed interest in understanding the nature of high-temperature superconductivity more generally. The low-energy electronic structure of the parent compound…

Recently, superconductivity was discovered in the infinite layer of hole-doped nickelates NdNiO$_{2}$. Contrary to this, superconductivity in LaNiO$_{2}$ is still under debate. This indicates the crucial role played by the $f$ electrons on…

强关联电子 · 物理学 2023-02-09 Andrzej Ptok , Surajit Basak , Przemysław Piekarz , Andrzej M. Oleś

After the significant discovery of the hole-doped nickelate compound Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, an analysis of the electronic structure, orbital components, Fermi surfaces and band topology could be helpful to understand the mechanism of…

材料科学 · 物理学 2021-03-18 Jiacheng Gao , Zhijun Wang , Chen Fang , Hongming Weng

We demonstrate in this paper that the recently discovered infinite-layer (IL) nickelates have much in common with a class of materials known as electrides. Oxide based electrides are compounds in which topotactic removal of loosely bound…

超导电性 · 物理学 2023-11-30 Kateryna Foyevtsova , Ilya Elfimov , George A. Sawatzky

The recent discovery of Sr-doped infinite-layer nickelate $\textrm{NdNiO}_2$ [D. Li et al. Nature 572, 624 (2019)] offers an exciting platform for investigating unconventional superconductivity in nickelatebased compounds. In this work, we…

强关联电子 · 物理学 2020-05-19 Zhao Liu , Zhi Ren , W. Zhu , Z. F. Wang , Jinlong Yang

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in…

Recent experiments have shown that the reduced multilayer rare-earth (RE) nickel oxides of form RE$_{p+1}$Ni$_p$O$_{2p+2}$ may belong to the novel family of superconducting lanthanide nickelates. Here, the correlated electronic structure of…

强关联电子 · 物理学 2022-04-07 Frank Lechermann

The superconducting infinite-layer (IL) nickelates offer a new platform for investigating the long-standing problem of high-temperature superconductivity. Many models were proposed to understand its superconducting mechanisms based on the…

Significant magnetic exchange interactions have been observed in infinite-layer nickelates RNiO2 (R = La, Pr, Nd), which exhibit unconventional superconductivity upon hole doping. Despite their structural and Fermi surface similarities to…

超导电性 · 物理学 2025-05-15 Yanbing Zhou , Dan Zhao , Boyun Zeng , Chengliang Xia , Yu Wang , Hanghui Chen , Tao Wu , Xianhui Chen

The discovery of superconductivity in the infinite-layer nickelates has opened new perspectives in the context of quantum materials. We analyze, via first-principles calculations, the electronic properties of La$_2$NiO$_3$F -- the first…

超导电性 · 物理学 2021-06-10 F. Bernardini , A. Demourgues , A. Cano

We analyze the electronic structure of different surface terminations for infinite-layer nickelates. Surface NiO$_2$ layers are found to be buckled, in contrast to planar bulk layers. While the rare-earth terminated surface fermiology is…

We report a determinant quantum Monte Carlo study of a two-band model, inspired by infinite-layer nickelates, focusing on the influence of interlayer hybridization between $3d_{x^2-y^2}$ orbitals derived from Ni (or Ni and O) in one layer…

强关联电子 · 物理学 2024-06-10 Fangze Liu , Cheng Peng , Edwin W. Huang , Brian Moritz , Chunjing Jia , Thomas P. Devereaux

Motivated by the recent discovery of superconductivity in the Sr-doped layered nickelate NdNiO$_2$, we perform a systematic computational materials design of layered nickelates that are dynamically stable and whose electronic structure…

超导电性 · 物理学 2020-02-12 Motoaki Hirayama , Terumasa Tadano , Yusuke Nomura , Ryotaro Arita

The recent discovery of superconductivity in infinite-layer nickelates has drawn considerable attention; however, a consensus on the fundamental building blocks and common ingredients necessary to understand and describe their ground states…

强关联电子 · 物理学 2023-12-07 Cheng Peng , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux , Chunjing Jia

The demonstration of superconductivity in nickelate analogues of high $T_c$ cuprates provides new perspectives on the physics of correlated electron materials. The degree to which the nickelate electronic structure is similar to that of…

强关联电子 · 物理学 2020-10-02 Jonathan Karp , Antia S. Botana , Michael R. Norman , Hyowon Park , Manuel Zingl , Andrew Millis

The recent observation of superconductivity in an infinite-layer and quintuple-layer nickelate within the same $R_{n+1}$Ni$_{n}$O$_{2n+2}$ series ($R$ = rare-earth, $n=2-\infty$, with $n$ indicating the number of NiO$_{2}$ layers along the…

强关联电子 · 物理学 2022-10-05 Harrison LaBollita , Myung-Chul Jung , Antia S. Botana

Motivated by recent photoemission measurements on the La$_{0.8}$Sr$_{0.2}$NiO$_2$, we carry out a systematic study of the infinite-layer nickelate using both dynamical mean-field theory and density matrix embedding theory. The renormalized…

强关联电子 · 物理学 2024-11-07 Ziyan Chen , Yuxin Wang , Kun Jiang , Jiangping Hu

Employing first-principles density functional theory calculations and Wannierization of the low energy band structure, we analyze the electronic structure of undoped, infinite-layer nickelate compounds, NdNiO$_2$, PrNiO$_2$ and LaNiO$_2$.…

Revealing the momentum-resolved electronic structure of infinite-layer nickelates is essential for understanding this new class of unconventional superconductors, but has been hindered by the formidable challenges in improving the sample…

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