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Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

材料科学 · 物理学 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby

Identifying an efficient pathway to change the order parameter via a subtle excitation of the coupled high-frequency mode is the ultimate goal of the field of ultrafast phase transitions. This is an especially interesting research direction…

Processes involving ultrafast laser driven electron-phonon dynamics play a fundamental role in the response of quantum systems in a growing number of situations of interest, as evidenced by phenomena such as strongly driven phase…

材料科学 · 物理学 2024-03-01 Kevin Lively , Shunsuke A. Sato , Guillermo Albareda , Angel Rubio , Aaron Kelly

We investigate generation of exchange magnons by ultrashort, picosecond acoustic pulses propagating through ferromagnetic thin films. Using the Landau-Lifshitz-Gilbert equations we derive the dispersion relation for exchange magnons for an…

介观与纳米尺度物理 · 物理学 2020-03-17 V. Besse , A. V. Golov , V. S. Vlasov , A. Alekhin , D. Kuzmin , I. V. Bychkov , L. N. Kotov , V. V. Temnov

We investigate spin angular momentum transfer in the Einstein-de Haas effect within prototypical magnetic crystals, focusing on its partition between phonons and rigid-body rotation. Using the Eckart frame to decouple local vibrations…

介观与纳米尺度物理 · 物理学 2026-01-30 Xin Nie , Wenhao Luo , Kun Cao , Dao-Xin Yao

The role of photon angular momentum in laser-induced demagnetization of Nickel thin films is investigated by means of pump-probe time-resolved magneto-optical Kerr effect in the polar geometry. The recorded data display a strong dependency…

材料科学 · 物理学 2009-11-11 F. Dalla Longa , J. T. Kohlhepp , W. J. M. de Jonge , B. Koopmans

The angular momentum interconversion between electron spin and other type of angular momenta is useful to develop new spintronic functionalities. The conversions from the angular momentum of photon and mechanical rotation to ferromagnetic…

介观与纳米尺度物理 · 物理学 2021-06-09 R. Sasaki , Y. Nii , Y. Onose

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

材料科学 · 物理学 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Ultrafast spectroscopies can access the dynamics of electrons and nuclei at short timescales, shedding light on nonequilibrium phenomena in materials. However, development of accurate calculations to interpret these experiments has lagged…

材料科学 · 物理学 2021-05-05 Xiao Tong , Marco Bernardi

We show that electron drag by nonequilibrium phonons describes the actual waveform and spectrum of terahertz pulses generated during femtosecond laser irradiation of metals. In contrast to previous models, there is a picosecond delay in the…

其他凝聚态物理 · 物理学 2026-04-16 Ivan Oladyshkin

We develop a kinetic theory for twisted density waves (phonons), carrying a finite amount of orbital angular momentum, in large magneto optical traps, where the collective processes due to the exchange of scattered photons are considered.…

量子气体 · 物理学 2016-02-17 J. D. Rodrigues , H. Terças , J. T. Mendonça

For nearly a decade, it has been a mystery why the small average number of photons absorbed per atom from an ultrashort laser pulse is able to induce a strong magnetization within a few hundred femtoseconds. Here we resolve this mystery by…

光学 · 物理学 2015-05-18 M. S. Si , G. P. Zhang

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

材料科学 · 物理学 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

The magnetization response of bulk ferromagnets after excitation by an ultrashort optical pulse is calculated using a dynamical model of the Elliott-Yafet type that includes the effects of the spin-orbit interaction in the ab-initio…

材料科学 · 物理学 2015-06-03 Sven Essert , Hans Christian Schneider

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

强关联电子 · 物理学 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

We report a computational theoretical investigation of electron spin-flip scattering induced by the electron-phonon interaction in the transition-metal ferromagnets bcc Fe, fcc Co and fcc Ni. The Elliott-Yafet electron-phonon spin-flip…

介观与纳米尺度物理 · 物理学 2015-06-15 K. Carva , M. Battiato , D. Legut , P. M. Oppeneer

In crystals with time-reversal symmetry but without inversion symmetry, the phonon angular momentum can be generated by the temperature gradient, and it is called phonon thermal Edelstein effect. On the other hand, when both symmetries are…

介观与纳米尺度物理 · 物理学 2020-06-02 Masato Hamada , Shuichi Murakami

We investigate ultrafast demagnetization due to electron-phonon interaction in a model band-ferromagnet. We show that the microscopic mechanism behind the spin dynamics due to electron-phonon interaction is the interplay of scattering and…

材料科学 · 物理学 2017-10-25 Kai Leckron , Svenja Vollmar , Hans Christian Schneider

The ultrafast control of materials has opened the possibility to investigate non-equilibrium states of matter with striking properties, such as transient superconductivity and ferroelectricity, ultrafast magnetization and demagnetization,…

材料科学 · 物理学 2023-11-23 Lorenzo Caprini , Hartmut Löwen , R. Matthias Geilhufe