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Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of non-thermal electrons, a material's dominant…

Time and angular resolved photoelectron spectroscopy is a powerful technique to measure electron dynamics in solids. Recent advances in this technique have facilitated band and energy resolved observations of the effect that excited…

材料科学 · 物理学 2020-09-30 Umberto De Giovannini , Hannes Hübener , Shunsuke A. Sato , Angel Rubio

In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency…

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

介观与纳米尺度物理 · 物理学 2019-03-27 Avinash Rustagi , Alexander F. Kemper

We use time- and angle-resolved photoemission spectroscopy (tr-ARPES) in the Extreme Ultraviolet (EUV) to measure the time- and momentum-dependent electronic structure of photo-excited K0.3MoO3. Prompt depletion of the Charge Density Wave…

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

材料科学 · 物理学 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective…

强关联电子 · 物理学 2019-11-18 Mattia Udina , Tommaso Cea , Lara Benfatto

This treatise reviews latest results obtained from angle-resolved photoemission spectroscopy (ARPES) on cuprate superconductors, with a special focus on the electron-phonon interaction. What has emerged is rich information about the…

强关联电子 · 物理学 2009-09-29 X. J. Zhou , T. Cuk , T. Devereaux , N. Nagaosa , Z. -X. Shen

Angle-resolved photoemission spectroscopy (ARPES) -- with its exceptional sensitivity to both the binding energy and momentum of valence electrons in solids -- provides unparalleled insights into the electronic structure of quantum…

强关联电子 · 物理学 2024-09-06 Fabio Boschini , Marta Zonno , Andrea Damascelli

Nonequilibrium pump-probe time domain spectroscopies can become an important tool to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Here, using the time-resolved solution of a model…

其他凝聚态物理 · 物理学 2014-01-07 Michael Sentef , Alexander F. Kemper , Brian Moritz , James K. Freericks , Zhi-Xun Shen , Thomas P. Devereaux

Time- and angle-resolved photoemission spectroscopy (trARPES) is a powerful spectroscopic method to measure the ultrafast electron dynamics directly in momentum-space. However, band gap materials with exceptional strong Coulomb interaction…

介观与纳米尺度物理 · 物理学 2019-12-09 Dominik Christiansen , Malte Selig , Ermin Malic , Ralph Ernstorfer , Andreas Knorr

Numerous angle resolved photoemission spectroscopy (ARPES) studies of a wide class of low-density metallic systems, ranging from doped transition metal oxides to quasi two-dimensional interfaces between insulators, exhibit phonon sidebands…

强关联电子 · 物理学 2020-10-29 J. Krsnik , V. N. Strocov , N. Nagaosa , O. S. Barišić , Z. Rukelj , S. M. Yakubenya , A. S. Mishchenko

Time-resolved angle-resolved photoemission spectroscopy is one of the most powerful pump-probe measurements of materials driven far from equilibrium. Unlike the linear-response regime, where the frequency-dependent response function is…

强关联电子 · 物理学 2021-09-29 J. K. Freericks , Alexander F. Kemper

We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron and electron-phonon interactions, and captures exciton formation as well as the transition…

材料科学 · 物理学 2025-02-13 Zhenlin Zhang , Wei Hu , Enrico Perfetto , Gianluca Stefanucci

Recently there has been an accumulation of experimental evidence in the high temperature superconductors suggesting the relevance of electron-phonon coupling in these materials. These findings challenge some well-held beliefs of what…

超导电性 · 物理学 2007-05-23 T. P. Devereaux , T. Cuk , Z. -X. Shen , N. Nagaosa

Photo-induced phase transitions have been intensively studied owing to the ability to control a material of interest in the ultrafast manner, which can induce exotic phases unable to be attained at equilibrium. However, the key mechanisms…

The electron-phonon coupling (EPC) is a ubiquitous interaction in condensed systems and plays a vital role in shaping the electronic properties of materials. Yet, achieving coherent manipulation of electron-phonon coupling has posed a…

材料科学 · 物理学 2024-05-13 Jicai Zhang , Tien-Dat Tran , Ziwen Wang , Wenhao Yu , Chong Zhang , Marcus Lo , Wenqi Xu , Tran Trung Luu

Recent developments in the techniques of ultrafast pump-probe photoemission have made possible the search for collective modes in strongly correlated systems out of equilibrium. Including inelastic scattering processes and a retarded…

超导电性 · 物理学 2017-11-29 B. Nosarzewski , B. Moritz , J. K. Freericks , A. F. Kemper , T. P. Devereaux

Time and angle-resolved photoemission spectroscopy (trARPES) allows direct mapping of the electronic band structure and its dynamic response on femtosecond timescales. Here, we present a new ARPES system, powered by a new fiber-based…

We discuss the potential creation and measurement of coherences in both dispersive solids and qubit-like single levels using current generation time- and angle-resolved photoemission technology. We show that in both cases, when both the…

介观与纳米尺度物理 · 物理学 2020-05-22 Alexander F. Kemper , Avinash Rustagi
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