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We present a system for molecular spectroscopy using a broadband mid-infrared laser with near infrared detection. Difference frequency generation of a Yb:fiber femtosecond laser produced a mid-infrared (MIR) source tunable from 2100-3700…
The mid-infrared (mid-IR) spectral region holds great promise for new laser-based sensing technologies, based on measuring strong mid-IR molecular absorption features. Practical applications have been limited to date, however, by current…
Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously…
Fourier transform infrared (FTIR) spectrometers have been the dominant technology in the field of mid-infrared (MIR)spectroscopy for decades. Supercontinuum laser sources operating in the MIR spectral region now offer the potential to…
Broadband mid-infrared (MIR) molecular spectroscopy demands a bright and broadband light source in the molecular fingerprint region. To this end, intra-pulse difference frequency generation (IDFG) has shown excellent properties among…
Plasma-based mid-infrared (MIR) laser generation has garnered significant interest owing to its advantage of high output power, continuous wavelength tunability, and ultrashort pulse durations. However, existing methodologies predominantly…
Tunable mid-infrared lasers are essential for optical sensing and imaging. Existing technologies, however, face challenges in simultaneously achieving broadband spectral tunability and ultra-rapid scan rates, limiting their utility in…
Optical frequency combs have revolutionized high-precision spectroscopy, yet an intrinsic trade-off between spectroscopic signal-to-noise ratio (sSNR) and measurement bandwidth ($B$) fundamentally constrains sensitive, broadband…
Spectral imaging in the mid-infrared (MIR) range provides simultaneous morphological and chemical information of a wide variety of samples. However, current MIR technologies struggle to produce high-definition images over a broad spectral…
Sensitive mid-infrared (MIR) spectroscopy plays an indispensable role in various photon-starved conditions. However, the detection sensitivity of conventional MIR spectrometers is severely limited by excessive noises of the involved…
We demonstrate mid-infrared (MIR) frequency combs at 10 GHz repetition rate via intra-pulse difference-frequency generation (DFG) in quasi-phase-matched nonlinear media. Few-cycle pump pulses ($\mathbf{\lesssim}$15 fs, 100 pJ) from a…
We present an experimental implementation of a chirped mid-infrared (mid-IR) high-power laser source with variable center frequency between 4 THz to 30 THz and continuously tunable frequency sweep of up to 20 % within one pulse, with a…
Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…
Spectral red-shifting of high power laser pulses propagating through underdense plasma can be a source of ultrashort mid-infrared (MIR) radiation. During propagation, a high power laser pulse drives large amplitude plasma waves, depleting…
A real-time ranging lidar with 0.1 Mega Hertz update rate and few-micrometer resolution incorporating dispersive Fourier transformation and instantaneous microwave frequency measurement is proposed and demonstrated. As time-stretched…
We demonstrate the measurement of single-shot spectra of temporally selected micropulses from a mid-infrared (MIR) free-electron laser (FEL) by upconversion. We achieve the upconversion of FEL pulses at 11 \mu m using externally…
The dream of physico-chemists to control molecular reactions with light beyond electronic excitations pushes the development of laser pulse shaping capabilities in the mid-infrared (MIR) spectral range. Here, we present a compact optical…
Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…
High-speed mid-infrared (MIR) videography constitutes an enabling tool to monitor and analyze various dynamics in scientific research and industrial applications, such as combustion diagnostics, explosion reactions, photosynthetic tracking,…
Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…