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We demonstrate dynamic control of the lattice by THz light by exploiting the coupling of phonon modes. The low-energy sliding phonon modes in the spin-ladder system, Sr$_{14}$Cu$_{24}$O$_{41}$, are excited using THz radiation with high…

Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

Lead halide perovskites (LHPs) have emerged as an excellent class of semiconductors for next-generation solar cells and optoelectronic devices. Tailoring physical properties by fine-tuning the lattice structures has been explored in these…

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

Coherent manipulation of magnetism through the lattice provides unprecedented opportunities for controlling spintronic functionalities on the ultrafast timescale. Such nonthermal control conventionally involves nonlinear excitation of…

Terahertz (THz) frequency range holds immense potential for high-speed data processing and signal manipulation. However, a fundamental challenge remains: the efficient and tunable control of THz electromagnetic fields. One promising…

光学 · 物理学 2025-07-28 Chao Shen , Carla Verdi , Serafim Babkin , Maksym Serbyn , Zhanybek Alpichshev

Excitation of coherent optical phonons in solids provides a pathway for ultrafast modulation of light on a sub-ps timescale. Here, we report on efficient 3.6 THz modulation of light reflected from hybrid metal/semiconductor plasmonic…

Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…

强关联电子 · 物理学 2016-08-22 Daniele Nicoletti , Andrea Cavalleri

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high frequency vibrational mode is driven resonantly by…

Terahertz near fields of gold metamaterials resonant at a frequency of $0.88\,\rm THz$ allow us to enter an extreme limit of non-perturbative ultrafast THz electronics: Fields reaching a ponderomotive energy in the keV range are exploited…

Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…

介观与纳米尺度物理 · 物理学 2021-11-29 Ziqi Li , Bo Peng , Miao-Ling Lin , Yu-Chen Leng , Bin Zhang , Chi Pang , Ping-Heng Tan , Bartomeu Monserrat , Feng Chen

Coherent control of quantum materials has progressed along two major fronts: nonlinear phononics, which reshapes lattices to induce emergent states, and Floquet engineering, which tailors electronic band reconstruction via time-periodic…

Active control of optical nonlinearity is essential for advancing next-generation electronics and photonics, including high-speed wireless communications, optical information processing, and nonlinear signal manipulation. However, achieving…

光学 · 物理学 2025-12-01 Chen Wang , Yong Tan , Yongzheng Wen , Shiqiang Zhao , Kaixin Yu , Renfei Zhang , Jingbo Sun , Ji Zhou

Coherent phonons describe the collective, ultrafast motion of atoms and play a central role in light-induced structural dynamics. Here, we employ terahertz scanning tunneling microscopy (THz-STM) to excite and detect coherent phonons in…

Tailored light excitation and nonlinear control of lattice vibrations have emerged as powerful strategies to manipulate the properties of quantum materials out of equilibrium. Generalizing the use of coherent phonon-phonon interactions to…

The nature of electronic motion and structural information of atoms and molecules is encoded into strong-field induced radiations ranging from terahertz (THz) to extreme ultraviolet wavelength. The dependence of THz yields in bi-chromatic…

原子物理 · 物理学 2024-05-31 Ziyang Gan , Kaixuan Zhang , Yuan Gao , Ahai Chen , Yizhu Zhang , Tian-Min Yan , Thomas Pfeifer , Yuhai Jiang

The interaction of a single-cycle THz electric field with the topological insulator $\mathrm{MnBi}_2\mathrm{Te}_4$ triggers strongly anharmonic lattice dynamics, promoting fully coherent energy transfer between the otherwise non-interacting…

We develop the microscopic theory of a terahertz (THz) laser based on the effects of resonant tunneling in a double quantum well heterostructure embedded in both optical and THz cavities. In the strong coupling regime the system hosts…

介观与纳米尺度物理 · 物理学 2014-02-26 K. Kristinsson , O. Kyriienko , I. A. Shelykh

We present a direct comparison between resonant terahertz (THz) and nonresonant impulsive stimulated Raman scattering (ISRS) excitation of phonon-polaritons in ferroelectric lithium niobate. THz excitation offers advantages of selectively…

材料科学 · 物理学 2017-02-01 Blake S. Dastrup , Jacob R. Hall , Jeremy A. Johnson

Modification of surface and volume of sapphire is shown to affect reflected and transmitted light at THz spectral range. Structural modifications were made using ultra-short 230 fs laser pulses at 1030 nm and 257.5 nm wavelengths forming…

介观与纳米尺度物理 · 物理学 2016-05-17 X. W. Wang , G. Seniutinas , A. Balcytis , I. Kasalynas , V. Jakstas , V. Janonis , R. Venckevicius , R. Buividas , D. Appadoo , G. Valusis , S. Juodkazis
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