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相关论文: Disorder-Induced Spectral Splitting versus Rabi Sp…

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The vacuum Rabi splitting (VRS) in molecular polaritons stands as a fundamental measure of collective light-matter coupling. Despite its significance, the impact of molecular disorder on VRS is not fully understood yet. This study delves…

化学物理 · 物理学 2024-04-18 Kai Schwennicke , Noel C. Giebink , Joel Yuen-Zhou

The strong coupling between two subsystems consisting of quantum emitters and photonic modes, at which the level splitting of mixed quantum states occurs, has been a central subject of quantum physics and nanophotonics due to various…

光学 · 物理学 2021-06-30 Renming Liu , Yi-Cong Yu , Xue-Hua Wang

Strong light-matter interactions between molecules and quantized electromagnetic fields inside an optical cavity open up novel possibilities, though inevitably influenced by disorder, an inherent attribute of realistic molecular systems.…

化学物理 · 物理学 2025-05-29 Robert F. Catuto , Hsing-Ta Chen

Exciton polaritons, arising from the interaction of electronic transitions with confined electromagnetic fields, have emerged as a powerful tool to manipulate the properties of organic materials. However, standard experimental and…

Polaritons are usually described within single-mode cavity QED models. However, nanophotonic environments typically involve several modes that spectrally overlap and interfere, giving rise to sharp dip features such as Fano profiles in the…

Semiconductor nanoparticles and nanostructures in the strong coupling regime exhibit an intriguing energy scale in the optical frequencies, which is specified by the Rabi splitting between the upper and lower exciton-polariton states.…

光学 · 物理学 2019-11-19 Burak Gerislioglu , Arash Ahmadivand

We provide a simple method that enables readily acquired experimental data to be used to predict whether or not a candidate molecular material may exhibit strong coupling. Specifically, we explore the relationship between the hybrid…

Strong light-matter coupling gives rise to polaritons - hybrid excitations whose mixed photonic and matter character enables control over optical, electronic and chemical properties. This Feature Article surveys the main architectures…

Multilayer assemblies of metal nanoparticles can act as photonic structures, where collective plasmon resonances hybridize with cavity modes to create plasmon-polariton states. For sufficiently strong coupling, plasmon polaritons…

光学 · 物理学 2026-05-28 Tanay Paul , Allison M. Green , Delia J. Milliron , Thomas M. Truskett

We study the interplay between disorder and light-matter coupling by considering a disordered one-dimensional chain of lossy dipoles coupled to a multimode optical cavity, through a microscopically derived Hamiltonian. Such a system,…

介观与纳米尺度物理 · 物理学 2023-01-04 Thomas F. Allard , Guillaume Weick

Strong light-matter interactions in both the single-emitter and collective strong coupling regimes attract significant attention due to emerging quantum and nonlinear optics applications, as well as opportunities for modifying…

介观与纳米尺度物理 · 物理学 2019-09-11 Tuomas P. Rossi , Timur Shegai , Paul Erhart , Tomasz J. Antosiewicz

The effect of disorder in the intensity of the driving laser on a coupled array of cavities described by a Bose-Hubbard Hamiltonian for dark-state polaritons is investigated. A canonically-transformed Gutzwiller wave function is used to…

其他凝聚态物理 · 物理学 2020-05-15 Abuenameh Aiyejina , Roger Andrews

Light-matter interactions can occur when an ensemble of molecular resonators is placed in a confined electromagnetic field. In the strong coupling regime the rapid exchange of energy between the molecules and the electromagnetic field…

介观与纳米尺度物理 · 物理学 2020-08-10 Philip A. Thomas , Wai Jue Tan , Henry A. Fernandez , William L. Barnes

From the high vibrational dipolar strength offered by molecular liquids, we demonstrate that a molecular vibration can be ultra-strongly coupled to multiple IR cavity modes, with Rabi splittings reaching $24\%$ of the vibration frequencies.…

The strong coupling between molecules and photonic modes in a Fabry-P\'{e}rot optical cavity, which forms hybrid light-matter states called polaritons, has been demonstrated as a promising route to control the rates of chemical reactions.…

量子物理 · 物理学 2025-05-22 Kunyang Sun , Matthew Du , Joel Yuen-Zhou

Cavity quantum electrodynamics advances the coherent control of a single quantum emitter with a quantized radiation field mode, typically piecewise engineered for the highest finesse and confinement in the cavity field. This enables the…

The strong coupling regime is observed in a system of two-dimensional electrons whose cyclotron motion is coupled to an electro-magnetic mode in a Fabry-Perot cavity resonator. The Rabi splitting of eigenfrequencies of coupled motion is…

介观与纳米尺度物理 · 物理学 2016-07-28 L. V. Abdurakhimov , R. Yamashiro , A. O. Badrutdinov , D. Konstantinov

Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition…

Strong coupling in the conventional sense requires that the Rabi cycling process between two interacting states is faster than other dissipation rates. Some recent experimental findings show intriguing properties that were attributed to…

材料科学 · 物理学 2026-03-09 Ben Johns , Nitin Yadav , Anand Vinod , Kuljeet Kaur , Jino George

Plasmonic structures interacting with light provide electromagnetic resonances which result in a high degree of local field confinement enabling the enhancement of light-matter interaction. Plasmonic structures typically consist of metals…

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