相关论文: Specular reflection of polar molecules from a simp…
A full density-matrix simulation is performed for optical deflection of a barium monofluoride (BaF) beam. Pairs of counter-propagating laser pulses are used for stimulated absorption followed by stimulated emission. The scheme produces a…
A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We…
Focusing optics for neutral molecules finds application in shaping and steering molecular beams. Here we present an electrostatic elliptical mirror for polar molecules consisting of an array of microstructured gold electrodes deposited on a…
A cryogenic neon solid doped with barium monofluoride (BaF) is created on a cryogenic substrate using a stream of Ne gas and a high-intensity beam of BaF molecules produced in a cryogenic helium-buffer-gas laser-ablation source. The…
We demonstrate one-dimensional Doppler cooling of a beam of buffer-gas cooled Barium monofluoride (BaF) molecules. The dependences of the cooling efficiency with the laser detuning, the bias filed and the laser intensity are carefully…
We describe a simple experimental apparatus for laser ablation of barium monohydride (BaH) molecules and the study of their rovibrational spectra that are relevant to direct laser cooling. We present a detailed analysis of the properties of…
Currently, there is great interest in laser cooling of barium monofluoride (BaF) molecules for precision tests of fundamental symmetries. We use high-resolution absorption spectroscopy to characterize several as yet imprecisely known…
Polarization is well known for its ability to decompose diffuse and specular reflections. However, the existing decomposition methods only focus on direct reflection and overlook multiple reflections, especially specular inter-reflection.…
Precision measurements of the electron's electric dipole moment (eEDM) are critical for testing fundamental symmetries in particle physics, and heavy polar molecules-such as barium monofluoride (BaF)-have emerged as promising candidates for…
Direct laser cooling of molecules has made significant progress in recent years. However, the selective cooling and manipulation of molecules based on their isotopic composition, which is ubiquitous in atomic laser cooling, has not yet been…
We present a mechanism for cooling atoms by a laser beam reflected from a single mirror. The cooling relies on the dipole force and thus in principle applies to arbitrary refractive particles including atoms, molecules, or dielectric…
We use two-dimensional transverse laser cooling to produce an ultracold beam of YbF molecules. Through experiments and numerical simulations, we study how the cooling is influenced by the polarization configuration, laser intensity, laser…
A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…
We present a significantly different reflection process from an optically thin flat metallic or dielectric layer and propose a strikingly simple method to form approximately unipolar half-cycle optical pulses via reflection of a…
Optical pumping of barium monofluoride (BaF) within a cryogenic neon matrix is demonstrated. Interestingly, with an applied magnetic field of 2~G, optical pumping is found to be considerably more efficient for a laser beam with…
A novel deflection effect of an intense laser beam with spin angular momentum is revealed theoretically by an analytical modeling using radiation pressure and momentum balance of laser plasma interaction in the relativistic regime, as a…
Electric deflection measurements on liquid helium nanodroplets doped with individual polar molecules demonstrate that the cold superfluid matrix enables full orientation of the molecular dipole along the external field. This translates into…
An electrostatic hexapole lens is used to manipulate the transverse properties of a beam of barium fluoride molecules from a cryogenic buffer gas source. The spatial distribution of the beam is measured by recording state-selective…
As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. The precision of such measurements can be significantly enhanced by utilizing a cold molecular sample.…
Dielectric mirrors comprising thin-film multilayers are widely used in optical experiments because they can achieve substantially higher reflectance compared to metal mirrors. Here we investigate potential problems that can arise when…