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This is the first quantitative analysis of mechanical reliability of all-solid state batteries. Mechanical degradation of the solid electrolyte (SE) is caused by intercalation-induced expansion of the electrode particles, within the…

材料科学 · 物理学 2017-03-16 Giovanna Bucci , Tushar Swamy , Yet-Ming Chiang , W. Craig Carter

Ageing of lithium-ion batteries results in irreversible reduction in performance. Intrinsic variability between cells, caused by manufacturing differences, occurs throughout life and increases with age. Researchers need to know the minimum…

Lithium metal batteries are seen as a critical piece towards electrifying aviation. During charging, plating of lithium metal, a critical failure mechanism, has been studied and mitigation strategies have been proposed. For electric…

化学物理 · 物理学 2021-03-09 Victor Venturi , Venkatasubramanian Viswanathan

Currently, the characterization of electric energy storage units used for power system operation and planning models relies on two major assumptions: charge and discharge efficiencies, and power limits are constant and independent of the…

系统与控制 · 电气工程与系统科学 2024-12-20 Alvaro Gonzalez-Castellanos , David Pozo , Aldo Bischi

Using a novel electrochemical phase-field model, we question the common belief that LixFePO4 nanoparticles separate into Li-rich and Li-poor phases during battery discharge. For small currents, spinodal decomposition or nucleation leads to…

材料科学 · 物理学 2015-03-13 Peng Bai , Daniel A. Cogswell , Martin Z. Bazant

This paper is the second part of a series of papers about empirical approaches to open circuit voltage (OCV) modeling and its performance comparison in lithium-ion batteries. The first part of the series introduced various sources of…

系统与控制 · 电气工程与系统科学 2023-06-30 Prarthana Pillai , James Nguyen , Balakumar Balasingam

We study the linear stability of transient electrodeposition in a charged random porous medium, whose pore surface charges can be of any sign, flanked by a pair of planar metal electrodes. Discretization of the linear stability problem…

化学物理 · 物理学 2019-07-09 Edwin Khoo , Hongbo Zhao , Martin Z. Bazant

Cathode particle fracture is widely recognised as a major degradation mechanism in lithium-ion batteries, yet cracking also permits electrolyte wetting of newly exposed internal surfaces, modifying interfacial reaction pathways. The…

计算工程、金融与科学 · 计算机科学 2026-05-05 S. Luza-Vega , Y. Zhao , E. Martínez-Pañeda

As the core determinant of lithium-ion battery performance, electrode materials play a crucial role in defining the battery's capacity, cycling stability, and durability. During charging and discharging, electrode materials undergo complex…

材料科学 · 物理学 2025-08-15 Liqi Wang , Ruijuan Xiao , Hong Li

In the present work we study the well-known Two Capacitor Problem from a new perspective. Although this problem has been thoroughly investigated, as far as we know there are no studies of the thermodynamic aspects of the discharge process.…

经典物理 · 物理学 2012-06-12 Vitor Lara , Alexandre P. Lima , Antônio T. Costa

This work proposes a semi-empirical model for the SEI growth process during the early stages of lithium-ion battery formation cycling and aging. By combining a full-cell model which tracks half-cell equilibrium potentials, a…

材料科学 · 物理学 2023-07-25 Andrew Weng , Everardo Olide , Iaroslav Kovalchuk , Jason B. Siegel , Anna Stefanopoulou

We present a porous electrode model for lithium-ion batteries using Butler--Volmer reaction kinetics. We model lithium concentration in both the solid and fluid phase along with solid and liquid electric potential. Through asymptotic…

应用物理 · 物理学 2019-06-03 Iain R. Moyles , Matthew G. Hennessy , Timothy G. Myers , Brian R. Wetton

Recently, we have experimentally demonstrated a continuous loading mechanism for an optical dipole trap from a guided atomic beam [1]. The observed evolution of the number of atoms and temperature in the trap are consequences of the unusual…

Accurate parameter dependent electro-chemical numerical models for lithium-ion batteries are essential in industrial application. The exact parameters of each battery cell are unknown and a process of estimation is necessary to infer them.…

统计理论 · 数学 2024-04-25 Andrea Petrocchi , Matthias K. Scharrer , Franz Pichler , Stefan Volkwein

Passivating solid-electrolyte interphase (SEI) films arising from electrolyte decomposition on low-voltage lithium ion battery anode surfaces are critical for battery operations. We review the recent theoretical literature on electrolyte…

化学物理 · 物理学 2013-07-12 Kevin Leung

In this work a 1D finite volume based model using coupled meshes is introduced to capture potential and species distribution throughout the discharge process in a lithium bismuth liquid metal battery while neglecting hydrodynamic effects,…

化学物理 · 物理学 2023-05-30 Carolina Duczek , Norbert Weber , Omar E. Godinez-Brizuela , Tom Weier

Nickel-based layered oxides offer an attractive platform for the development of energy-dense cobalt-free cathodes for lithium-ion batteries but suffer from degradation via oxygen gas release during electrochemical cycling. While such…

材料科学 · 物理学 2022-04-29 Xinhao Li , Qian Wang , Haoyue Guo , Nongnuch Artrith , Alexander Urban

This paper presents the current state of mathematical modelling of the electrochemical behaviour of lithium-ion batteries as they are charged and discharged. It reviews the models developed by Newman and co-workers, both in the cases of…

化学物理 · 物理学 2020-02-04 Giles W Richardson , Jamie M Foster , Rahifa Ranom , Colin P Please , Angel M Ramos

Parasitic extraction is a powerful tool in the design process of electromechanical devices, specifically as part of workflows that check electromagnetic compatibility. A novel scheme to extract impedances from CAD device models, suitable…

计算工程、金融与科学 · 计算机科学 2021-07-07 Jonathan Stysch , Andreas Klaedtke , Herbert De Gersem

Batteries are playing an increasingly central role as distributed energy resources in the shift toward power systems dominated by renewable energy sources. However, existing battery models must invariably rely on complementarity constraints…

最优化与控制 · 数学 2025-06-27 Juan M. Morales
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