相关论文: Nanocavities for Molecular Optomechanics: their fu…
This is a tutorial-style introduction to the field of molecular polaritons. We describe the basic physical principles and consequences of strong light-matter coupling common to molecular ensembles embedded in UV-visible or infrared…
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…
We propose a theoretical scheme to generate nonreciprocal bipartite entanglement between a cavity mode and vibrational modes in a molecular cavity optomechanical system. Our system consists of $\mathcal{N}$ molecules placed inside a…
Accessing the terahertz (THz) spectral domain through surface-enhanced Raman spectroscopy (SERS) is challenging and opens up the study of low-frequency molecular and electronic excitations. Compared to direct THz probing of heterogenous…
The purpose of this work is to calculate the vibrational modes of an elastically anisotropic sphere embedded in an isotropic matrix. This has important application to understanding the spectra of low-frequency Raman scattering from…
We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by…
Optical cavities are a foundational technology for controlling light-matter interactions. While interfacing a single cavity to either an atom or ensemble has become a standard tool, the advent of single atom control in large atomic arrays…
State-of-the-art microscopes use intense lasers that can severely disturb biological processes, function and viability. This introduces hard limits on performance that only quantum photon correlations can overcome. Here we demonstrate this…
We present an integrated optomechanical and electromechanical nanocavity, in which a common mechanical degree of freedom is coupled to an ultrahigh-Q photonic crystal defect cavity and an electrical circuit. The sys- tem allows for…
Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often…
Cavity-enhanced radiation pressure coupling between optical and mechanical degrees of freedom allows quantum-limited position measurements and gives rise to dynamical backaction enabling amplification and cooling of mechanical motion. Here…
Today's cutting-edge optical spectroscopic exploratory tools, such as Raman or infrared spectroscopy, rely on methods of signal enhancement as a route for their development. These methods are indispensable for substance identification and…
Raman phonons are quantized molecular motions that arise from the inelastic scattering of light and mediate a wide range of spectroscopic and nonlinear optical phenomena. These can play a major role in frequency-conversion processes, but…
Electromagnetic cavity modes in photonic and plasmonic resonators offer rich and attractive regimes for tailoring the properties of light-matter interactions. Yet there is a disturbing lack of a precise definition for what constitutes a…
We present a method to locally probe spatially varying chemical composition of soft matter systems by use of optically controlled and elastically self-assembled plasmonic nanoantennae. Disc-shaped metal particles with sharp irregular edges…
We present, for the first time, the quantum mechanical description of light-matter interaction in the presence of optical cavities that are characterized by radiative losses. Unique to radiative losses is the unitary evolution and their…
Light is extensively used to steer the motion of atoms in free space, enabling cooling and trapping of matter waves through ponderomotive forces and Doppler-mediated photon scattering. Likewise, light interaction with free electrons has…
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers strongly…
We use a method based on optical coherent transients to study the vibrational coherence lifetimes of atoms trapped in the potential wells of a near-resonant optical lattice in the oscillating regime. The dependence of the positions and…
The rigorous resource framework of quantum coherence has been set up recently and excited a wide variety of interests. Here we show that a quantum cavity optomechanical system, as an emerging platform, can behave with a certain value of…