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The pressure-driven insulator-metal transition is a crucial topic in condensed matter physics. However, even for the prototypical strongly correlated system, NiO, the critical pressure for transition remains debated. In this work, we…

强关联电子 · 物理学 2025-05-30 Bei-Lei Liu , Yue-Chao Wang , Yuan-Ji Xu , Xingyu Gao , Hai-Feng Liu , Hai-Feng Song

We explore the interplay of electron-electron correlations and surface effects in the prototypical correlated insulating material, NiO. In particular, we compute the electronic structure, magnetic properties, and surface energies of the…

强关联电子 · 物理学 2021-04-09 I. Leonov , S. Biermann

We have calculated magnetic properties and the electronic structure of NiO both in the paramagnetic and in magnetically-ordered state as well as zero-temperature properties and thermodynamics within the strongly-correlated crystal-field…

强关联电子 · 物理学 2008-10-08 R. J. Radwanski , Z. Ropka

The thermodynamics of the antiferromagnetic ordering transition in NiO and the photoelectron spectra in the antiferromagnetic phase are studied by the Variational Cluster Approximation. Using realistic Racah parameters to describe the…

强关联电子 · 物理学 2015-04-01 R. Eder

We report a detail theoretical study of the electronic structure and phase stability of transition metal oxides MnO, FeO, CoO, and NiO in their paramagnetic cubic B1 structure by employing dynamical mean-field theory of correlated electrons…

强关联电子 · 物理学 2016-10-26 I. Leonov , L. Pourovskii , A. Georges , I. A. Abrikosov

We report a theoretical study of the effects of electron correlations and structural confinement on the electronic properties and magnetic state of LaNiO3 (LNO) thin films epitaxially deposited on the (001) LaAlO3 (LAO) substrate. Using the…

强关联电子 · 物理学 2024-02-01 N. O. Vambold , G. A. Sazhaev , I. V. Leonov

We perform a comprehensive theoretical study of the pressure-induced evolution of the electronic structure, magnetic state, and phase stability of the late transition metal monoxides MnO, FeO, CoO, and NiO using a fully charge…

强关联电子 · 物理学 2020-06-22 I. Leonov , A. O. Shorikov , V. I. Anisimov , I. A. Abrikosov

Strong electron correlations underlie a plethora of electronic and magnetic components and devices and are often used to identify and probe novel ground states in quantum materials. Herein we report a magnetic phase crossover in EuMn2P2, an…

The charge transfer antiferromagnetic (T$_{N}$ =220 K) insulator EuNiO$_{3}$ undergoes, at ambient pressure, a temperature-induced metal insulator MI transition at T$_{MI}$=463 K. We have investigated the effect of pressure (up to p~20 GPa)…

强关联电子 · 物理学 2009-11-11 R. Lengsdorf , A. Barla , J. A. Alonso , M. J. Martinez-Lope , H. Micklitz , M. M. Abd-Elmeguid

Electron correlation and long-range magnetic ordering have a significant impact on the electronic structure and physical properties of solids. Here, we investigate the electronic structure of ilmenite MnTiO$_{3}$ using room temperature…

强关联电子 · 物理学 2025-06-13 Asif Ali , R. K. Maurya , Sakshi Bansal , B. H. Reddy , Ravi Shankar Singh

Ultrashort x-ray pulses can be used to disentangle magnetic and structural dynamics and are accordingly utilized here to study the photoexcitation of NdNiO$_3$ (NNO), a model nickelate exhibiting structural and magnetic dynamics that…

Accurate high-energy electron diffraction measurements of structure factors of NiO have been carried out to investigate how strong correlations in the Ni 3d shell affect electron charge density in the interior area of nickel ions and…

强关联电子 · 物理学 2009-10-31 S. L. Dudarev , L. -M. Peng , S. Y. Savrasov , J. -M. Zuo

We use a combination of optical spectra, first principles calculations, and energy dependent magneto-optical measurements to elucidate the electronic structure and to study the phase diagram of Ni$_3$V$_2$O$_8$. We find a remarkable…

强关联电子 · 物理学 2007-05-23 R. C. Rai , J. Cao , S. Brown , J. L. Musfeldt , D. Kasinathan , D. J. Singh , G. Lawes , N. Rogado , R. J. Cava , X. Wei

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

Using \emph{ab initio} band structure and DFT+dynamical mean-field theory methods we examine the effects of electron-electron interactions on the electronic structure, magnetic state, and structural phase stability of the recently…

强关联电子 · 物理学 2026-01-26 I. V. Leonov

Magnetic correlations in all four phases of pure and doped vanadium sesquioxide V_2O_3 have been examined by magnetic thermal neutron scattering. While the antiferromagnetic insulator can be accounted for by a Heisenberg localized spin…

强关联电子 · 物理学 2009-10-31 Wei Bao , C. Broholm , G. Aeppli , S. A. Carter , P. Dai , T. F. Rosenbaum , J. M. Honig , P. Metcalf , S. F. Trevino

The YNiO$_3$ nickelate is a paradigm d-electron oxide that manifests the intriguing temperature-mediated sequence of three phases transitions from (i) magnetically ordered insulator to (ii) paramagnetic (PM) insulator and then to (iii) PM…

材料科学 · 物理学 2023-03-16 Oleksandr I. Malyi , Alex Zunger

It has been recently shown that under pressure trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ (LNO) becomes superconducting below a critical temperature $\sim$20 K, in addition to the infinite-layer and bilayer systems. Motivated…

强关联电子 · 物理学 2024-06-12 I. V. Leonov

Using DFT+DMFT we study the normal-state electronic structure and magnetic correlations of the recently discovered alternating single-layer bilayer Raddlesden-Popper nickelate La$_5$Ni$_3$O$_{11}$ (1212-LNO). Our results exhibit qualitative…

强关联电子 · 物理学 2026-04-30 I. V. Leonov

A non-trivial balance between Coulomb repulsion and kinematic effects determines the electronic structure of correlated electron materials. The use electromagnetic fields strong enough to rival these native microscopic interactions allows…

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