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Polyelectrolyte (PE) hydrogels can dynamically respond to external stimuli, such as changes in pH and temperature, which benefits their use for smart materials and nanodevices with tunable properties. We investigate equilibrium…

软凝聚态物质 · 物理学 2026-04-07 Jiaxing Yuan , Tine Curk

Dynamic structuring of water is a key player in a large class of processes underlying biochemical and technological developments today, the latter often involving electric fields. However, the anisotropic coupling between the water…

软凝聚态物质 · 物理学 2019-05-29 Andreas Baer , Zoran Miličević , David M. Smith , Ana-Sunčana Smith

We introduce a three-dimensional model for polyelectrolyte hydrogel filaments operating in a fluid environment under an electric field. The formulation builds on a morphoelastic framework for inextensible and unshearable rods, such that the…

The behavior of polyelectrolytes between charged surfaces immersed in semi-dilute solutions is investigated theoretically. A continuum mean field approach is used for calculating numerically concentration profiles between two electrodes…

软凝聚态物质 · 物理学 2007-05-23 I. Borukhov , D. Andelman , H. Orland

Stretching dynamics of polymers in microfluidics is of particular interest for polymer scientists. As a charged polymer, a polyelectrolyte can be deformed from its coiled equilibrium configuration to an extended chain by applying uniform or…

软凝聚态物质 · 物理学 2014-11-18 Farnoush Farahpour , Fathollah Varnik , Mohammad Reza Ejtehadi

In this study we use non-equilibrium thermodynamics to systematically derive a phase-field model of a polyelectrolyte gel coupled to a hydrodynamic model for a salt solution surrounding the gel. The governing equations for the gel account…

软凝聚态物质 · 物理学 2022-03-02 Giulia L. Celora , Matthew G. Hennessy , Andreas Münch , Barbara Wagner , Sarah L. Waters

Colloidal magnetic particles embedded in an elastic polymer matrix constitute a smart material called ferrogel. It responds to an applied external magnetic field by changes in elastic properties, which can be exploited for various…

软凝聚态物质 · 物理学 2016-10-07 Peet Cremer , Hartmut Löwen , Andreas M. Menzel

Biological systems achieve adaptive mechanical responses through reaction-diffusion processes that couple chemical wave propagation to structural transitions. Although synthetic hydrogels with enzymatic reactions offer a platform for…

软凝聚态物质 · 物理学 2026-03-31 Natascha Gray , Zoe Grämiger , André R. Studart , Rafael Libanori

Contraction assay based on surface measurement have been widely used to evaluate cell contractility in 3D models. This method is straightforward and requires no specific equipment, but it does not provide quantitative data about contraction…

Nonlinear elastic responses of short and stiff polyelectrolytes are investigated by dynamic simulations on a single molecule level. When a polyelectrolyte condensate undergoes a mechanical unfolding, two types of force-extension curves,…

软凝聚态物质 · 物理学 2009-11-10 Hirofumi Wada , Yoshihiro Murayama , Masaki Sano

Since the discovery of polar topological textures, achieving efficient control and manipulation of them has emerged as a significant challenge for their integration into nanoelectronic devices. In this study, we use second principles…

材料科学 · 物理学 2025-08-01 Fernando Gómez-Ortiz , Louis Bastogne , He Xu , Philippe Ghosez

Two types of high-strength composite hydrogels possessing the structure of interpenetrating polymer networks were synthesized via free-radical polymerization of acrylamide carried out straight within the matrix of plant or bacterial…

化学物理 · 物理学 2019-04-02 Alexander Buyanov , Iosif Gofman , Natalya Saprykina

We use a coarse-grained molecular dynamics model to study the electrophoretic behaviour of flexible polyelectrolyte chains. We first characterize the static properties of the model with respect to the chain length, the polyelectrolyte…

软凝聚态物质 · 物理学 2008-12-16 Kai Grass , Christian Holm

Computer simulations are used to investigate the response of a charged colloid and its surrounding microion cloud to an external electric field. Both static fields (DC) and alternating fields (AC) are considered. A mesoscopic simulation…

软凝聚态物质 · 物理学 2013-07-19 Jiajia Zhou , Roman Schmitz , Burkard Duenweg , Friederike Schmid

We study the behavior of single linear polyelectrolytes condensed by trivalent salt under the action of electric fields through computer simulations. The chain is unfolded when the strength of the electric field is stronger than a critical…

软凝聚态物质 · 物理学 2011-08-26 Yu-Fu Wei , Pai-Yi Hsiao

In this work, we perform experiments with spherical polyacrylamide (PAAm) hydrogel drops/spheres, spanning a broad range of shear moduli and impact velocities on hydrophilic (plasma-treated glass) and hydrophobic (silane-coated) substrates,…

软凝聚态物质 · 物理学 2026-04-21 Akash Chowdhury , Surjyasish Mitra , Sushanta K. Mitra

Based on a coordinate transformation approach, Pendry {\it et al.} have reported electromagnetically anisotropic and inhomogeneous shells that, in theory, completely shield an interior structure of arbitrary size from electromagnetic fields…

Implantable hydrogels should ideally possess mechanical properties matched to the surrounding tissues to enable adequate mechanical function while regeneration occurs. This can be challenging, especially when degradable systems with high…

组织与器官 · 定量生物学 2024-03-19 Michael Phillips , Giuseppe Tronci , Christopher M. Pask , Stephen J. Russell

Simulation of extracellular fields is one of the substantial methods used in the area of computational neuroscience. Its most common usage is validation of experimental methods as EEG and extracellular spike recordings or modeling of…

神经元与认知 · 定量生物学 2013-01-22 Pavol Bauer , Sanja Mikulovic , Stefan Engblom , Katarina E. Leão , Frank Rattay , Richardson N. Leão

High-strength composite hydrogels cellulose-polyacrylamide were synthesized by free-radical polymerization of acrylamide conducted inside the previously formed physical network of regenerated plant cellulose. Partial hydrolysis of the amide…

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