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Two-dimensional (2D) layered hybrid perovskites provide an ideal platform for studying the properties of excitons. Here, we report on a strong triplet-exciton and longitudinal-optical (LO) phonon coupling in 2D (C6H5CH2CH2NH3, PEA)2PbBr4…

介观与纳米尺度物理 · 物理学 2021-02-26 Yunuan Wang , Feilong Song , Yu Yuan , Jianchen Dang , Xin Xie , Sibai Sun , Sai Yan , Yanbing Hou Zhidong Lou , Xiulai Xu

Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…

Lead-halide perovskite nanocrystals (PNCs) exhibit unique optoelectronic properties, many of which originate from a purported bright-triplet exciton fine-structure. A major impediment to measuring this fine-structure is inhomogeneous…

介观与纳米尺度物理 · 物理学 2022-03-09 Albert Liu

Two-dimensional (2D) materials have attracted considerable attention due to their unique physicochemical properties and significant potential in energy-related applications. Polymeric carbon nitrides (PCNs) with 2D stacked architecture show…

To assess the potential optoelectronic applications of metal-halide perovskites, it is critical to have a detailed understanding of the nature, strength, and dynamics of the interactions between carriers and the polar lattices. Here, we…

材料科学 · 物理学 2022-10-28 Xing He , Naveen Kumar Tailor , Soumitra Satapathi , Jakoah Brgoch , Ding-Shyue Yang

Our ability to efficiently detect and generate far-infrared (i.e., terahertz) radiation is vital in areas spanning from biomedical imaging to interstellar spectroscopy. Despite decades of intense research, bridging the terahertz gap between…

材料科学 · 物理学 2023-07-24 Zhao Tang , Greis J. Cruz , Fanhao Jia , Yabei Wu , Weiyi Xia , Peihong Zhang

Two-dimensional (2D) perovskites or Ruddleson Popper (RP) perovskites have emerged as a class of material inheriting the superior optoelectronic properties of two different materials: perovskites and 2D materials. The large exciton binding…

Reducing the dimensionality of metal-halide perovskites enhances quantum and dielectric confinement, enabling tunable excitonic properties. In one dimension, the arrangement of metal-halide octahedra in chains with corner-, edge-, or…

材料科学 · 物理学 2025-09-05 Kostas Fykouras , Linn Leppert

Stable excitons in semiconductor monolayers such as transition-metal dichalcogenides (TMDCs) enable and motivate fundamental research as well as the development of room-temperature optoelectronics applications. The newly discovered layered…

材料科学 · 物理学 2021-03-17 Magdalena Birowska , Paulo E. Faria Junior , Jaroslav Fabian , Jens Kunstmann

Active optical waveguides combine light source and waveguides together in an individual component, which are essential for the integrated photonic chips. Although 1D luminescent materials based optical waveguides were extensively…

Exciton-polaritons (EPs) arising from strong light-matter coupling offer new pathways for controlling optoelectronic properties. While typically requiring closed optical cavities for strong coupling, we demonstrate that 2D metal-organic…

光学 · 物理学 2025-12-11 Bongjun Choi , Adam D. Alfieri , Wangleong Chen , Deep Jariwala

Mixed-halide based hybrid perovskite semiconductors have attracted tremendous attention as a promising candidate for high efficient photovoltaic and light-emitting devices. However, these advanced perovskite materials may undergo phase…

Semiconductor heterostructures are backbones for solid state based optoelectronic devices. Recent advances in assembly techniques for van der Waals heterostructures has enabled the band engineering of semiconductor heterojunctions for…

Hybrid Perovskites have shown a great potential for applications in photovoltaics and light-emitting devices with high efficiency. Interaction between defect-induced trapped excitons and phonons plays an important role in understanding the…

Development of advanced optical data storage, information encryption, and security labeling technologies requires low-cost materials exhibiting local, pronounced, and diverse modification of their structure-dependent optical properties…

Halide perovskite solar cells have demonstrated a rapid increase in power conversion efficiencies. Understanding and mitigating remaining carrier losses in halide perovskites is now crucial to enable further increases to approach their…

There is a variety of possible ways to tune the optical properties of 2D perovskites, though the mutual dependence between different tuning parameters hinders our fundamental understanding of their properties. In this work we attempt to…

Perovskite-based nanoscintillators, such as CsPbBr3 nanocrystals (NCs), are emerging as promising candidates for ionizing radiation detection, thanks to their high emission efficiency, rapid response, and facile synthesis. However, their…

Photogenerated carrier transport and recombination in metal halide perovskites are critical to device performance. Despite considerable efforts, sample quality issues and measurement techniques have limited the access to their intrinsic…

Due to their exceptional photovoltaic properties, metal halide perovskites (MHPs) are extensively studied for their potential applications in solar cells. In recent years, the power conversion efficiencies of MHPs-based solar cells rapidly…

材料科学 · 物理学 2022-08-12 A. Bojtor , S. Kollarics , B. G. Markus , A. Sienkiewicz , M. Kollar , L. Forro , F. Simon