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Mechanical deformations, either spontaneously occurring during sample preparation or purposely induced in their nanoscale manipulation, drastically affect the electronic and optical properties of transition metal dichalcogenide monolayers.…

材料科学 · 物理学 2024-02-16 Stefan Velja , Jannis Krumland , Caterina Cocchi

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

材料科学 · 物理学 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

材料科学 · 物理学 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

Semiconducting 2D materials, such as transition metal dichalcogenides (TMDs), are emerging in nanomechanics, optoelectronics, and thermal transport. In each of these fields, perfect control over 2D material properties including strain,…

Layered materials such as graphite and transition metal dichalcogenides have extremely anisotropic mechanical properties owing to orders of magnitude difference between in-plane and out-of-plane interatomic interaction strengths. Although…

材料科学 · 物理学 2017-11-10 Jae-Ung Lee , Sungjong Woo , Jaesung Park , Hee Chul Park , Young-Woo Son , Hyeonsik Cheong

Large area MoS2 and WS2 van der Waals epitaxial thin films with complete control over number of layers including monolayer is grown by pulsed laser deposition utilizing slower growth kinetics. The films grown on c-plane sapphire show…

Van der Waals stacking presents new opportunities for nonlinear optics with its remarkable tunability and scalability. However, the fundamental role of interlayer interactions in modifying the overall nonlinear optical susceptibilities…

We demonstrate a method to induce tensile and compressive strain into two-dimensional transition metal dichalcogenide (TMDC) MoS$_{2}$ via the deposition of stressed thin films to encapsulate exfoliated flakes. With this technique we can…

介观与纳米尺度物理 · 物理学 2021-07-15 Tara Peña , Shoieb A. Chowdhury , Ahmad Azizimanesh , Arfan Sewaket , Hesam Askari , Stephen M. Wu

Geometrical confinement effect in exfoliated sheets of layered materials leads to significant evolution of energy dispersion with decreasing layer thickness. Molybdenum disulphide (MoS2) was recently found to exhibit indirect to direct gap…

Transition metal dichalcogenides are 2D structures with remarkable electronic, chemical, optical and mechanical properties. Monolayer and crystal properties of these structures have been extensively investigated, but a detailed…

介观与纳米尺度物理 · 物理学 2018-01-18 Y. M. Jaques , P. Manimunda , Y. Nakanishi , S. Susarla , C. F. Woellner , S. Bhowmick , S. A. S. Asif , D. S. Galvão , C. S. Tiwary , P. M. Ajayan

We characterize the electronic structure and elasticity of monolayer transition-metal dichalcogenides MX2 (M=Mo, W, Sn, Hf and X=S, Se, Te) with 2H and 1T structures using fully relativistic first principles calculations based on density…

材料科学 · 物理学 2015-06-18 David M. Guzman , Alejandro Strachan

Emergence of topological states in strongly correlated systems, particularly two-dimensional (2D) transition-metal dichalcogenides, offers a platform for manipulating electronic properties in quantum materials. However, a comprehensive…

Many classes of two-dimensional (2D) materials have emerged as potential platforms for novel electronic and optical devices. However, the physical properties are strongly influenced by nanoscale heterogeneities in the form of edges, grain…

Two-dimensional transition metal dichalcogenides show great potential as promising thermoelectric materials due to their lower dimensionality, the unique density of states and quantum confinement of carriers. The effect of mechanical strain…

计算物理 · 物理学 2019-05-28 Jayanta Bera , Satyajit Sahu

The discovery of two dimensional (2D) magnetic materials has brought great research value for spintronics and data storage devices. However, their air-stability as well as the oxidation mechanism has not been unveiled, which limits their…

材料科学 · 物理学 2022-04-06 Jun Chen , Linwei Zhou , Nanshu Liu , Jingsi Qiao , Xieyu Zhou , Cong Wang , Wei Ji

Second harmonic generation (SHG) is prohibited in centrosymmetric crystals such as silicon or germanium due to the presence of inversion symmetry. However, the structuring of such materials makes it possible to break the inversion symmetry,…

The new generation of two-dimensional (2D) materials has shown a broad range of applications for optical and electronic devices. Understanding the properties of these materials when integrated with the more traditional three-dimensional…

First-principles calculations are used to probe the effects of mechanical strain on the magnetic and optical properties of monolayer (ML) 2H-TaSe$_2$. A complex dependence of these physical properties on strain results in unexpected…

材料科学 · 物理学 2019-08-21 Sugata Chowdhury , Jeffrey R. Simpson , T. L. Einstein , Angela R. Hight Walker

We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is…

光学 · 物理学 2018-08-20 Yu Song , Siqi Hu , Miao-Ling Lin , Xuetao Gan , Ping-Heng Tan , Jianlin Zhao

Magnetic doping of 2D materials such as Transition Metal Dichalcogenides is promising for the enhancement of magneto-optical properties, as it was previously observed for 3D diluted magnetic semiconductors. To maximize the effect of…

材料科学 · 物理学 2023-09-15 Julia Kucharek , Rafał Bożek , Wojciech Pacuski