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Momentum-indirect excitons composed of electrons and holes in different valleys define optoelectronic properties of many semiconductors, but are challenging to detect due to their weak coupling to light. The identification of an excitons'…

Artificial moir\'e superlattices in 2d van der Waals heterostructure is a new venue for realizing and controlling correlated electronic phenomena. Recently, twisted bilayer WSe$_2$ emerged as a new robust moir\'e system hosting a correlated…

强关联电子 · 物理学 2020-12-02 Zhen Bi , Liang Fu

Collective excitations presenting nonlinear dynamics are fundamental phenomena with broad applications. A prime example is nonlinear optics, where diverse frequency mixing processes are central to communication, sensing, wavelength…

We present a theoretical analysis of valley pseudospin control in the transition metal dichalcogenide (TMD) monolayer by utilizing the magnetic proximity effect of 2D magnetic layer and, propose self-consistent analysis of photoluminescence…

介观与纳米尺度物理 · 物理学 2026-05-20 V. N. Mantsevich

We investigate the confinement of neutral excitons in a one-dimensional (1D) potential, engineered by proximizing hBN-encapsulated monolayer MoSe$_2$ to ferroelectric domain walls (DW) in periodically poled LiNbO$_3$. Our device exploits…

介观与纳米尺度物理 · 物理学 2025-03-21 Pedro Soubelet , Yao Tong , Asier Astaburuaga Hernandez , Peirui Ji , Katia Gallo , Andreas V. Stier , Jonathan J. Finley

Spin-flip dark excitons are optical-dipole-forbidden quasiparticles with remarkable potential in optoelectronics, especially when they are realized within cleavable van der Waals materials. Despite this potential, dark excitons have not yet…

We report the experimental observation of quadrupolar exciton states in the reflectance contrast spectrum of 2$H$-stacked bilayer MoSe$_2$. The application of a vertical electric field results in a quadratic energy redshift of these…

In superlattices of twisted semiconductor monolayers, tunable moir\'e potentials emerge, trapping excitons into periodic arrays. In particular, spatially separated interlayer excitons are subject to a deep potential landscape and they…

介观与纳米尺度物理 · 物理学 2023-06-02 Samuel Brem , Ermin Malic

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and…

The polarization analysis of optical transitions in monolayer and bilayer transition-metal dichalcogenides provides invaluable information on the spin and valley (pseudospin) degrees of freedom. To explain optical properties of a given…

材料科学 · 物理学 2015-10-06 Hanan Dery , Yang Song

Valley selective hybridization and residual coupling of electronic states in commensurate van der Waals heterobilayers enable the control of the orbital character of interlayer excitons. We demonstrate electric field control of layer index,…

Controlling magnetic order via external fields or heterostructures enables precise manipulation and tracking of spin and exciton information, facilitating the development of high-performance optical spin valves. However, the weak…

材料科学 · 物理学 2024-09-30 Jia Shi , Dan Wang , Nai Jiang , Ziqian Xin , Houzhi Zheng , Chao Shen , Xinping Zhang , Xinfeng Liu

Moir\'e patterns with angular mismatch in van der Waals heterostructures composed of atomically thin semiconducting materials are a fascinating platform to engineer the optically generated excitonic properties towards novel quantum…

介观与纳米尺度物理 · 物理学 2020-12-17 Keisuke Shinokita , Yuhei Miyauchi , Kenji Watanabe , Takashi Taniguchi , Kazunari Matsuda

Vertically stacked van der Waals heterostructures constitute a promising platform for providing tailored band alignment with enhanced excitonic systems. Here we report observations of neutral and charged interlayer excitons in trilayer…

The moire potential, induced by stacking two monolayer semiconductors with slightly different lattice mismatches, acts as periodic quantum confinement for optically generated excitons, resulting in spatially ordered zero-dimensional quantum…

Squeezing bubbles and impurities out of interlayer spaces by applying force through a few-layer graphene capping layer leads to van der Waals heterostructures with ultra-flat structure free from random electrostatic potential arising from…

介观与纳米尺度物理 · 物理学 2020-12-29 T. Hotta , A. Ueda , S. Higuchi , M. Okada , T. Shimizu , T. Kubo , K. Ueno , T. Taniguchi , K. Watanabe , R. Kitaura

Interlayer valley excitons in bilayer MoS2 feature concurrently large oscillator strength and long lifetime, and hence represent an advantageous scenario for valleytronic applications. However, control of valley pseudospin of interlayer…

We investigate the excitonic spectrum of MoS$_2$ monolayers and calculate its optical absorption properties over a wide range of energies. Our approach takes into account the anomalous screening in two dimensions and the presence of a…

介观与纳米尺度物理 · 物理学 2018-05-28 Emilia Ridolfi , Caio H. Lewenkopf , Vitor M. Pereira

Transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform to explore unique excitonic physics via properties of the constituent TMDs and external stimuli. Interlayer excitons (IXs) can form in TMD heterobilayers as…

介观与纳米尺度物理 · 物理学 2023-11-02 Hanlin Fang , Qiaoling Lin , Yi Zhang , Joshua Thompson , Sanshui Xiao , Zhipei Sun , Ermin Malic , Saroj Dash , Witlef Wieczorek

Moir\'e superlattices in atomically thin van-der-Waals heterostructures hold great promise for an extended control of electronic and valleytronic lifetimes, the confinement of excitons in artificial moir\'e lattices, and the formation of…