相关论文: Utilizing frustration in Gd- and Yb-based oxides f…
Generation of very low temperatures has been crucially important for applications and fundamental research, as low-temperature quantum coherence enables operation of quantum computers and formation of exotic quantum states, such as…
Attaining milli-Kelvin temperatures is often a prerequisite for the study of novel quantum phenomena and the operation of quantum devices. Adiabatic demagnetization refrigeration (ADR) is an effective, easy and sustainable alternative to…
We report the synthesis, characterization, low-temperature magnetic, and thermodynamic measurements of the novel milli-Kelvin adiabatic demagnetization refrigeration (mK-ADR) candidate material NaYbGeO$_4$ which exhibits a distorted square…
Adiabatic demagnetization refrigeration (ADR) is regaining relevance for the refrigeration to temperatures below 1 K as global helium-3 supply is increasingly strained. While ADR at these temperatures is long established with paramagnetic…
Crystal structure, thermodynamic properties, and adiabatic demagnetization refrigeration (ADR) effect in the spin-7/2 triangular antiferromagnet KBaGd(BO3)2 are reported. With the average nearest-neighbor exchange coupling of 44 mK, this…
We present a comprehensive study of the structural, magnetic, and thermodynamic properties, as well as the adiabatic demagnetization refrigeration (ADR) performance of NaGdP$_2$O$_7$. Although NaGdP$_2$O$_7$ exhibits antiferromagnetic…
With the aim of improving the performance of classical paramagnetic salts for adiabatic refrigeration processes at the sub-Kelvin range, relevant thermodynamic parameters of some new Yb-based intermetallic compounds are analyzed and…
We report the effect of exchange frustration on the magnetocaloric properties of GdCrTiO$_5$ compound. Due to the highly exchange-frustrated nature of magnetic interaction, in GdCrTiO$_5$, the long-range antiferromagnetic ordering occurs at…
Rare-earth (RE) based frustrated magnets have attracted great attention as excellent candidates for magnetic refrigeration at sub-Kelvin temperatures, while the experimental identification on systems exhibiting both large volumetric cooling…
Frustrated magnets provide a platform for exploring exotic phases beyond conventional ordering, with potential relevance to functional materials and information technologies. In this work, we use Monte Carlo simulations to map the…
A tiny adiabatic-demagnetization refrigerator (T-ADR) has been developed for a commercial superconducting quantum interference device magnetometer [Magnetic Property Measurement System (MPMS) from Quantum Design]. The whole T-ADR system is…
An adiabatic demagnetization process is studied in Gd2Ti2O7, a geometrically frustrated antiferromagnet on a pyrochlore lattice. In contrast to conventional paramagnetic salts, this compound can exhibit a temperature decrease by a factor of…
We develop a general framework, which combines exact diagonalization in small clusters with a density matrix variational principle, to study frustrated magnets at finite temperature. This thermodynamic hierarchical mean-field technique is…
The magnetothermodynamics of strongly frustrated classical Heisenberg antiferromagnets on kagome, garnet, and pyrochlore lattices is examined. The field induced adiabatic temperature change (dT/dH)_S is significantly larger for such systems…
Many laboratories routinely cool samples to 10 mK, but relatively few can cool condensed matter below 1 mK. Easy access to the microkelvin range would propel fields such as quantum sensors and quantum materials. Such temperatures are…
Motivated by recent experiments on BaCuSi2O6, we investigate magnetic excitations and quantum phase transitions of layered dimer magnets with inter-layer frustration. We consider two scenarios, (A) a lattice with one dimer per unit cell and…
Geometric magnetic frustration (GMF) has attracted substantial interest due to the exotic physics and rich phase diagrams revealed by the cancellation of normally-dominant magnetic interactions, giving impetus for the search for novel…
Thermodynamic properties of cubic Heisenberg ferromagnets with competing exchange interactions are considered near the frustration point where the coefficient $D$ in the spin-wave spectrum $E_{\mathbf{k}}\sim D k^{2}$ vanishes. Within the…
The intermetallic compound Nd$_2$Co$_{0.85}$Si$_{2.88}$ having a triangular lattice could be synthesized in single-phase only with defect crystal structure. Investigation through different experimental techniques indicate the presence of…
As materials with suppressed ordering temperatures and enhanced ground state entropies, frustrated magnetic oxides are ideal candidates for cryogenic magnetocaloric refrigeration. While previous materials design has focused on tuning the…